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We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…

Atomic Physics · Physics 2017-09-13 Chien-Yu Lien , Scott R. Williams , Brian Odom

The process of nonlinear electron emission from a metal surface under the action of femtosecond laser pulse with moderate intensity $\sim10^{11}$~W/cm$^2$ is considered. One-dimensional model is formulated, taking into account the advantage…

Mesoscale and Nanoscale Physics · Physics 2016-11-24 P. A. Golovinski , E. A. Mikhin

We present some approaches to the computation of ultra-fast laser pulses capable of selectively breaking molecular bonds. The calculations are based on a mixed quantum-classical description: The electrons are treated quantum mechanically…

Atomic and Molecular Clusters · Physics 2015-05-27 Kevin Krieger , Alberto Castro , E. K. U. Gross

The possibility of achieving highly selective excitation of low metastable states of hydrogen and helium atoms by using short laser pulses with reasonable parameters is demonstrated theoretically. Interactions of atoms with the laser field…

Atomic Physics · Physics 2007-05-23 A. D. Kondorskiy , L. P. Presnyakov , Yu. Ralchenko

We study laser-driven isomerization reactions through an excited electronic state using the recently developed Geometrical Optimization procedure [J. Phys. Chem. Lett. 6, 1724 (2015)]. The goal is to analyze whether an initial wave packet…

Chemical Physics · Physics 2018-02-07 Bo Y. Chang , Seokmin Shin , Volker Engel , Ignacio R. Sola

The parametric amplification of ultrashort (femtosecond) laser pulses in crystals with a regular domain structure (RDS) of the 5%Mg : PPLN type has been investigated theoretically. The focus was on the formation of a signal pulse in…

Optics · Physics 2024-05-07 O. I. Sobirov , D. B. Yusupov , N. A. Akbarova , U. K. Sapaev

We present a detailed study of the ionisation probability of H and H$_{2}^{+}$ induced by a short intense laser pulse. Starting from a Coulomb-Volkov description of the process we derive a multipole-like expansion where each term is…

Atomic Physics · Physics 2013-07-11 Renata Della Picca , Juan Fiol , Pablo Daniel Fainstein

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

Optimal control techniques combined with femtosecond laser pulse shaping are applied to steer and enhance the strong-field induced emission of highly charged atomic ions from silver clusters embedded in helium nanodroplets. With light…

The temporal dynamics of double ionization of H2 has been investigated both experimentally and theoretically with few-cycle laser pulses. The main observables are the proton spectra associated to the H^+ + H^+ fragmentation channel. The…

Quantum Physics · Physics 2008-09-23 Sébastien Saugout , Eric Charron , Christian Cornaggia

We derive the analytical theory describing the process of sub-femtosecond pulse formation from a quasi-monochromatic seeding extreme ultraviolet (XUV) radiation, which propagates in active medium of a hydrogen-like plasma-based X-ray laser…

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

Atomic Physics · Physics 2014-05-19 Armin Scrinzi , Bernard Piraux

Advances of high intensity lasers have opened up the field of strong field physics and led to a broad range of technological applications. Recent x ray laser sources and optics development makes it possible to obtain extremely high…

We experimentally investigate the impact of pulse shape on the dynamics of laser-generated plasma in rare gases. Fast-rising triangular pulses with a slower decay lead to early ionization of the air and depose energy more efficiently than…

We optimize the pulse shape and polarization of time-dependent electric fields to maximize the production of electron-positron pairs via strong field quantum electrodynamics processes. The pulse is parametrized in Fourier space by a…

High Energy Physics - Phenomenology · Physics 2017-08-02 François Fillion-Gourdeau , Florian Hebenstreit , Denis Gagnon , Steve MacLean

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

We discuss double ionization of atoms in strong laser pulses using a reduced dimensionality model. Following the insights obtained from an analysis of the classical mechanics of the process, we confine each electron to move along the lines…

Atomic Physics · Physics 2008-08-06 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Collision of laser-driven subrelativistic high density ion flows provides a way to create extremely compressed ion conglomerates and study their properties. This paper presents a theoretical study of the electrodynamic implosion of ions…

Plasma Physics · Physics 2025-12-03 S. Yu. Guskov , Ph. Korneev , M. Murakami