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The advent of ultrafast pulsed X-ray free-electron lasers with very high brightness has enabled the determination of transient molecular structures of small and medium-sized organic molecules in excited states and undergoing chemical…

Chemical Physics · Physics 2025-10-07 Peter M. Weber , Brian Stankus , Adam Kirrander

X-ray scattering has been an indispensable tool in advancing our understanding of matter, from the first evidence of the crystal lattice to recent discoveries of nuclei's fastest dynamics. In addition to the lattice, ultrafast resonant…

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic…

Chemical Physics · Physics 2024-03-19 Antonia Freibert , David Mendive-Tapia , Oriol Vendrell , Nils Huse

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitations of these materials hold great promise for understanding and…

Strongly Correlated Electrons · Physics 2019-04-02 Y. Cao , D. G. Mazzone , D. Meyers , J. P. Hill , X. Liu , S. Wall , M. P. M. Dean

The study of elementary bosonic excitations is essential toward a complete description of quantum electronic solids. In this context, resonant inelastic X-ray scattering (RIXS) has recently risen to becoming a versatile probe of electronic…

Strongly Correlated Electrons · Physics 2019-01-23 M. Kang , J. Pelliciari , Y. Krockenberger , J. Li , D. E. McNally , E. Paris , R. Liang , W. N. Hardy , D. A. Bonn , H. Yamamoto , T. Schmitt , R. Comin

This paper is concerned with the inverse time-harmonic elastic scattering problem of recovering unbounded rough surfaces in two dimensions. We assume that elastic plane waves with different directions are incident onto a rigid rough surface…

Numerical Analysis · Mathematics 2018-04-09 Guanghui Hu , Xiaoli Liu , Bo Zhang , Haiwen Zhang

We propose a scheme for imaging periodic surfaces using a superlens. By employing an inverse scattering model and the transformed field expansion method, we derive an approximate reconstruction formula for the surface profile, assuming…

Numerical Analysis · Mathematics 2024-03-05 Peijun Li , Yuliang Wang

High-energy X-ray diffraction methods can non-destructively map the 3D microstructure and associated attributes of metallic polycrystalline engineering materials in their bulk form. These methods are often combined with external stimuli…

The development of medium-energy inelastic X-ray scattering (IXS) optics with meV and sub-meV resolution has attracted considerable efforts in recent years. Meanwhile, there are also concerns or debates about the fundamental and feasibility…

Optics · Physics 2011-09-12 Xian-Rong Huang

Many applications require recovering the geometry information of multiple elastic particles based on the scattering information. In this paper, we consider the inverse time-harmonic elastic scattering of multiple rigid particles in three…

Mathematical Physics · Physics 2022-09-21 Jun Lai , Jinrui Zhang

In indirect resonant inelastic X-ray scattering (RIXS) an intermediate state is created with a core-hole that has a ultrashort lifetime. The core-hole potential therefore acts as a femtosecond pulse on the valence electrons. We show that…

Strongly Correlated Electrons · Physics 2009-11-11 Luuk J. P. Ament , Filomena Forte , Jeroen van den Brink

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it…

Strongly Correlated Electrons · Physics 2015-06-25 Jeroen van den Brink

Recent seminal experiments have utilized time-resolved X-ray absorption spectroscopy (XAS) to investigate the ultrafast photo-induced renormalization of the electron interaction (''Hubbard $U$'') in Mott and charge transfer insulators. In…

Strongly Correlated Electrons · Physics 2025-08-19 Denis Golez , Eva Paprotzki , Philipp Werner , Martin Eckstein

A rigorous mathematical model and an efficient computational method are proposed to solving the inverse elastic surface scattering problem which arises from the near-field imaging of periodic structures. We demonstrate how an enhanced…

Analysis of PDEs · Mathematics 2017-12-08 Huaian Diao , Peijun Li , Xiaokai Yuan

The detection of inelastically scattered soft X-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of X-rays (PAX) has been rediscovered for modern spectroscopy…

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš