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Bianisotropy is a powerful concept enabling asymmetric optical response, including asymmetric reflection, absorption, optical forces, light trapping, and lasing. The physical origin of these asymmetric effects can be understood from…

Optics · Physics 2021-07-07 Ehsan Mobini , Rasoul Alaee , Robert W. Boyd , Ksenia Dolgaleva

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…

We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…

Optical-field sampling using second-harmonic generation (SHG) from strong-field ionization enables ultrabroadband terahertz detection, but the microscopic origin of the SHG signal and its ultrabroadband response have been unclear. Here we…

Recently Second Harmonic Generation (SHG) for the yellow exciton series in cuprous oxide has been demonstrated [J. Mund et al., Phys. Rev. B 98, 085203 (2018)]. Assuming perfect $O_{\mathrm{h}}$ symmetry, SHG is forbidden along certain…

We report on time-resolved ultrafast optical spectroscopy study of the topological insulator (TI) Bi$_2$Se$_3$. We unravel that a net spin polarization can not only be generated using circularly polarized light via interband transitions…

Materials Science · Physics 2016-01-26 M. C. Wang , S. Qiao , Z. Jiang , S. N. Luo , J. Qi

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion sym-metry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally small. We…

We report optical second-harmonic generation (SHG) in reflection from GaSe crystals of 1 to more than 100 layers using a fundamental picosecond pulsed pump at 1.58 eV and a supercontinuum white light pulsed laser with energies ranging from…

Mesoscale and Nanoscale Physics · Physics 2017-10-10 Yanhao Tang , Krishna C. Mandal , John A. McGuire , Chih Wei Lai

High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

Optics · Physics 2023-09-08 Akira Kofuji , Robert Peters

Under infrared ultrashort pulse laser stimulation, we investigated temperature-dependent second-harmonic generation (SHG) from nitrogen-vacancy (NV)-introduced bulk diamond. The SHG intensity decreases in the temperature range of 20-300…

Optics · Physics 2022-04-05 Aizitiaili Abulikemu , Yuta Kainuma , Toshu An , Muneaki Hase

Surfaces and interfaces of magnetic nanostructures can reveal rather interesting and unusual properties that differ substantially from those of bulky materials. Here we apply the surface-sensitive method of optical second harmonic…

Mesoscale and Nanoscale Physics · Physics 2018-12-13 T. V. Murzina , K. A. Lazareva , E. E. Shalygina , I. A. Kolmychek , E. A. Karashtin , N. S. Gusev , A. A. Fraerman

The magnetic spin dynamics and optical properties of EuZn$_2$P$_2$ are studied. Single crystals grown by the Sn-flux method crystallize in the $P\overline{3}m1$ (No.~164) space group and order antiferromagnetically at $T_N=23.5$~K.…

Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…

We combined a spin-resolved photoemission spectrometer with a high-harmonic generation (HHG) laser source in order to perform spin-, time- and angle-resolved photoemission spectroscopy (STARPES) experiments on the transition metal…

We present both static and time-resolved second harmonic generation (SHG) measurements on polar antiferromagnet Fe$_2$Mo$_3$O$_8$ to monitor the evolution of the electric polarization change and its coupling to magnetic order. We find that…

Strongly Correlated Electrons · Physics 2021-08-29 L. Y. Shi , D. Wu , T. Lin , S. J. Zhang , Q. M. Liu , Z. X. Wang , T. C. Hu , T. Dong , N. L. Wang

In a thin strip of a two-dimensional semiconductor electronic system, spin-orbit coupling may be induced near both edges of the strip due to the substantial spatial variation of the confining potential in the boundary regions. In this paper…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yongjin Jiang , Liangbin Hu

The anisotropic dispersion and inherent nonlinearity of magnetostatic spin waves in thin films and confined structures provide unique opportunities for implementation in next-generation magnonic devices for data and signal processing. A…

Materials Science · Physics 2026-05-19 Stephanie R. Lake , Marc Eger , Philipp Geyer , Rouven Dreyer , Seth W. Kurfman , Georg Schmidt

We have studied second harmonic generation (SHG) in a polar ferrimagnet GaFeO_3, employing a FeO_6 cluster model in which the Fe atom is slightly shifted from the center of the octahedron. The electric-dipole transition could take place…

Strongly Correlated Electrons · Physics 2015-05-19 Jun-ichi Igarashi , Tatsuya Nagao

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

Optics · Physics 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen