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We develop the strong-field approximation for high-order harmonic generation in hydrogen molecules, including the vibrational motion and the laser-induced coupling of the lowest two Born-Oppenheimer states in the molecular ion that is…

Atomic Physics · Physics 2009-11-13 C. C. Chirila , M. Lein

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Optically excited electron-hole pairs, driven by a strong terahertz (THz) field, create high-sidebands in the optical spectrum. The sideband spectrum exhibits a 'plateau' up to a cutoff of 3.17Up, where Up is the ponderomotive energy. This…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 J. A. Crosse , Ren-Bao Liu

We present the generation of high order harmonics in crystalline silicon subjected to intense near-infrared 30fs laser pulse. The harmonic spectrum extends from the near infrared to the extreme ultraviolet spectral region. Depending on the…

Atomic Physics · Physics 2020-08-10 Boyan Obreshkov , Tzveta Apostolova

We present a model for quasi-phase matching (QPM) in high-order harmonic generation (HHG). Using a one-dimensional description, we analyze the time-dependent, ultrafast wave-vector balance to calculate the on-axis harmonic output versus…

The classical approach to linking lattice dynamics properties to continuum equations of motion, the "method of long waves," is extended to include higher order terms. The additional terms account for non-local and non-linear effects. In the…

Computational Physics · Physics 2018-09-05 Zhijie Xu , R. C. Picu , J. Fish

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

The nonlinear saturation of the tearing mode is revisited in slab geometry by taking into account higher-order harmonics in the outer solution. The general formalism for tackling this problem in the case of a vanishing current gradient at…

Plasma Physics · Physics 2009-11-13 N. Arcis , N. F. Loureiro , F. Militello

The extreme nonlinear optical process of high-harmonic generation (HHG) makes it possible to map the properties of a laser beam onto a radiating electron wavefunction, and in turn, onto the emitted x-ray light. Bright HHG beams typically…

We explore with ab-initio theory high harmonic generation (HHG) from a series of gas-phase fullerenes (from C$_{20}$ to C$_{60}$, including isomers) under varying laser conditions (different ellipticities, angular orientations, intensities…

Optics · Physics 2026-02-27 Km Akanksha Dubey , Ofer Neufeld

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

High-order harmonic generation in the presence of a chirped THz pulse is investigated numerically with a complete 3D non-adiabatic model. The assisting THz pulse illuminates the HHG gas cell laterally inducing quasi-phase-matching. We…

The mechanism of harmonic generation in both O and X-mode configurations for a magnetized plasma has been explored here in detail with the help of Particle-In-Cell (PIC) simulations. A detailed characterization of both the reflected and…

Plasma Physics · Physics 2021-10-27 Srimanta Maity , Devshree Mandal , Ayushi Vashistha , Laxman Prasad Goswami , Amita Das

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

We present a classical model for high harmonic generation during the propagation of an intense laser pulse through an atomic gas. Numerical simulations of the model show excellent quantitative agreement with the corresponding quantum model…

Atomic Physics · Physics 2018-07-04 S. A. Berman , J. Dubois , C. Chandre , M. Perin , T. Uzer

We present a novel method for multi-color wavefront measurement of high-order harmonic generation beams using the Talbot effect, validated both theoretically and experimentally for the first time. Each harmonic maintains a unique wavefront…

Optics · Physics 2024-02-07 Yang Du , Kui Li , Jin Niu , Angyi Lin , Jie Li , Zhongwei Fan , Guorong Wu , Xiaoshi Zhang , Fucai Zhang

We study nonlinear optical response of Landau quantized graphene to an intense electromagnetic wave. In particular, we consider high harmonic generation process. It is shown that one can achieve efficient generation of high harmonics with…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 H. K. Avetissian , A. G. Ghazaryan , G. F. Mkrtchian , Kh. V. Sedrakian

Waveform shaping and frequency synthesis based on waveform modulation is ubiquitous in electronics, telecommunication technology, and optics. For optical waveforms, the carrier frequency is on the order of several hundred THz, while the…

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We studied the multi-plateau high-order harmonic generation (HHG) from solids numerically. It is found that the HHG spectrum in the second or higher plateau is redshifted in short laser pulses due to the nonadiabatic effect. The…

Optics · Physics 2017-09-20 Guang-Rui Jia , Xue-Bin Bian