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We demonstrate a left-right asymmetry control of the photo\-electron angular distribution in multi\-photon ionization of Li atoms by a bichromatic laser field. By delaying the fundamental (780 nm) and its second harmonic relative to each…

Atomic Physics · Physics 2024-05-20 Silva Mezinska , Alexander Dorn , Thomas Pfeifer , Klaus Bartschat

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

We calculate angle-resolved above-threshold ionization spectra for diatomic molecules in linearly polarized laser fields, employing the strong-field approximation. The interference structure resulting from the individual contributions of…

Atomic Physics · Physics 2009-11-13 H. Hetzheim , C. Figueira de Morisson Faria , W. Becker

The development of fast numerical methods for multilevel radiative transfer (RT) applications often leads to important breakthroughs in astrophysics, because they allow the investigation of problems that could not be properly tackled using…

Astrophysics · Physics 2009-11-11 A. Asensio Ramos , J. Trujillo Bueno

Resonant light interacting with matter can support different phases of a polarizable medium, and optical bistability where two such phases coexist. Here we identify signatures of optical phase transitions and optical bistability mapped onto…

Atomic Physics · Physics 2020-11-10 C. D. Parmee , J. Ruostekoski

We propose a new scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created…

Atomic Physics · Physics 2025-07-01 T. Bayer , K. Eickhoff , D. Köhnke , M. Wollenhaupt

Holography is a cornerstone characterisation and imaging technique that can be applied to the full electromagnetic spectrum, from X-rays to radio waves or even particles such as neutrons. The key property in all these holographic approaches…

Quantum Physics · Physics 2021-01-12 Hugo Defienne , Bienvenu Ndagano , Ashley Lyons , Daniele Faccio

Optical imaging plays a critical role in advancing our understanding of three dimensional dynamics of biological systems. Coherent imaging (CI) methods exploit spatial phase information, encoded through propagation of coherent signal light…

Optics · Physics 2015-07-24 Jeffrey J. Field , David G. Winters , Randy A. Bartels

Accessing coherences is key to fully understand and control ultrafast dynamics of complex quantum systems like molecules. Most photochemical processes are mediated by conical intersections (CIs), which generate coherences between electronic…

This study aims to assess the composition of scattered particles generated in proton therapy for tumours situated proximal to titanium dental implants. The investigation involves decomposing the mixed field and recording Linear Energy…

Conical intersections (CI) between molecular potential energy surfaces with non-vanishing non-adiabatic couplings generally occur in any molecule consisting of at least three atoms. They play a fundamental role in describing the molecular…

The discovery of topological phases has recently led to a paradigm shift in condensed matter physics, and facilitated breakthroughs in engineered photonics and acoustic metamaterials. Topological insulators (TIs) enable the generation of…

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

A double-index atomic partitioning of the molecular first-order density matrix is proposed. Contributions diagonal in the atomic indices correspond to atomic density matrices, whereas off-diagonal contributions carry information about the…

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

We have measured hyperfine structure in the first-excited $P$ state ($D$ lines) of all the naturally-occurring alkali atoms. We use high-resolution laser spectroscopy to resolve hyperfine transitions, and measure intervals by locking the…

Atomic Physics · Physics 2010-08-20 Dipankar Das , Vasant Natarajan

We provide approximate analytic expressions for above-threshold ionization (ATI) transition probabilities and photoelectron angular distributions (PADs). These analytic expressions are more general than those existing in the literature and…

Atomic Physics · Physics 2018-02-14 A. S. Maxwell , A. Al-Jawahiry , X. Y. Lai , C. Figueira de Morisson Faria

An approach using topology reveals a new understanding and knowledge of laser particle acceleration. Laser pulse irradiation on a thin-foil target is examined using two-dimensional particle-in-cell simulations. Through topology, laser ion…

Plasma Physics · Physics 2019-05-29 Toshimasa Morita

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek