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A versatile semiclassical approximation for intense laser-atom processes is presented. This uniform approximation is no more complicated than the frequently-used multi-dimensional saddle-point approximation and far superior, since it…

Atomic Physics · Physics 2016-09-08 C. Figueira de Morisson Faria , H. Schomerus , W. Becker

Manipulating at will the propagation dynamics of high power laser pulses is a long-standing dream whose accomplishment would lead to the control of a plethora of fascinating physical phenomena emerging from laser-matter interaction. The…

Optics · Physics 2015-11-18 P. Béjot , G. Karras , F. Billard , J. Doussot , E. Hertz , B. Lavorel , O. Faucher

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

We demonstrate sub-cycle control of frustrated double ionization (FDI) in the two-electron triatomic molecule D$_3^+$ when driven by two orthogonally polarized two-color laser fields. We employ a three-dimensional semi-classical model that…

Atomic Physics · Physics 2018-05-22 A. Vilà , G. P. Katsoulis , A. Emmanouilidou

In any atomic species, the spherically symmetric potential originating from the charged nucleus results in fundamental symmetry properties governing the structure of atomic states and transition rules between them. If atoms are exposed to…

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

We investigate the role of hyperfine structure in resonant-dipole interactions between two atoms cotrapped in an optical tweezer. Two-body loss rates from light-assisted collisions (LACs) are measured across the $^{87}$Rb hyperfine spectrum…

Atomic Physics · Physics 2025-01-14 Steven K. Pampel , Matteo Marinelli , Mark O. Brown , José P. D'Incao , Cindy A. Regal

A theory for the many-electron multi-photon process is presented. It is shown that after single-electron excitation into some level in the continuum (ATI) an inelastic collision of the excited electron with the parent atomic particle can…

atom-ph · Physics 2009-10-28 M. Yu. Kuchiev

Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show…

Atomic Physics · Physics 2015-08-20 Ncamiso B. Khanyile , Gang Shu , Kenneth R. Brown

We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…

Atomic Physics · Physics 2020-08-05 Benjamin L. Augenbraun , John M. Doyle , Tanya Zelevinsky , Ivan Kozyryev

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

Atomic Physics · Physics 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

We analyze two-particle binding factors of H2, LiH, and HeH+ molecules/ions with the help of our original exact diagonalization ab intio (EDABI) approach. The interelectronic correlations are taken into account rigorously within the second…

Strongly Correlated Electrons · Physics 2022-08-24 M. Hendzel , M. Fidrysiak , J. Spałek

In the present work we propose a novel quantum material concept, which enables super- and/or ultrastrong interaction of two-level systems with the photonic field in a complex network. Within the mean field approximation we examine phase…

Quantum Physics · Physics 2025-07-23 A. Yu. Bazhenov , M. Nikitina , Alexander Alodjants

The relativistic theory of above-threshold ionization (ATI) of hydrogen-like atoms in ultrastrong radiation fields, taking into account the photoelectron induced rescattering in the continuum spectrum is developed. It is shown that the…

Quantum Physics · Physics 2007-05-23 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

A new scheme based on (i) upcoming brilliant X-ray Free Electron Laser (FEL) sources, (ii) novel energy and angular dispersive, large-area electron imagers and (iii) the well-known photoelectron holography is elaborated that provides…

Atomic Physics · Physics 2015-05-14 F. Krasniqi , B. Najjari , L. Strüder , D. Rolles , A. Voitkiv , J. Ullrich

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

Nonadiabatic dynamics around an avoid crossing or a conical intersection play a crucial role in the photoinduced processes of most polyatomic molecules. The present work shows that the topological phase in conical intersection makes the…

Optics · Physics 2022-11-01 Guanglu Yuan , Ruifeng Lu , Shicheng Jiang , Konstantin Dorfman

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

Rapid development of topological concepts in photonics unveils exotic phenomena such as unidirectional propagation of electromagnetic waves resilient to backscattering at sharp bends and disorder-immune localization of light at stable…