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We examine the robustness of single-molecule tunneling diodes to thermal-environmental effects. The diode comprises three fragments: two different conjugated chemical groups at the boundaries, and a saturated moiety in between, breaking…

Mesoscale and Nanoscale Physics · Physics 2015-12-29 Michael Kilgour , Dvira Segal

We have investigated the effect of a difference in the tunnelling resistances of the individual normal metal-insulator-superconductor (NIS) tunnel junctions in a double junction SINIS device, with particular emphasis on the impact on the…

Mesoscale and Nanoscale Physics · Physics 2012-02-01 S. Chaudhuri , I. J. Maasilta

Molecular conduction operating in dielectric solvent environments are often described using kinetic rates based on Marcus theory of electron transfer at a molecule-metal electrode interface. However, the successive nature of charge transfer…

Chemical Physics · Physics 2020-02-18 Henning Kirchberg , Michael Thorwart , Abraham Nitzan

We develop a theory of thermal transport of weakly interacting electrons in quantum wires. Unlike higher-dimensional systems, a one-dimensional electron gas requires three-particle collisions for energy relaxation. The fastest relaxation is…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Alex Levchenko , Tobias Micklitz , Zoran Ristivojevic , K. A. Matveev

Heating and heat conduction in molecular junctions are considered within a general NEGF formalism. We obtain a unified description of heating in current carrying molecular junctions as well as the electron and phonon contributions to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Mark A. Ratner , Abraham Nitzan

The translational motion of molecular ions can be effectively cooled sympathetically to translational temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The ro-vibrational degrees of freedom,…

Atomic Physics · Physics 2009-11-10 I. S. Vogelius , L. B. Madsen , M. Drewsen

It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on…

Quantum Physics · Physics 2009-11-10 S. Schiller , C. Laemmerzahl

The study of cold and controlled molecular ions is pivotal for fundamental research in modern physics and chemistry. Investigations into cooling molecular anions, in particular, have proven to be of key consequence for the production of…

We show that the vibrations of a nanomechanical resonator can be cooled to near its quantum ground state by tunnelling injection of electrons from an STM tip. The interplay between two mechanisms for coupling the electronic and mechanical…

Mesoscale and Nanoscale Physics · Physics 2011-05-12 F. Santandrea , L. Y. Gorelik , R. I. Shekhter , M. Jonson

We study the phenomenon of absorption refrigeration, where refrigeration is achieved by heating instead of work, in two different setups: a minimal set up based on coupled qubits, and two non-linearly coupled resonators. Considering ZZ…

Quantum Physics · Physics 2021-09-01 Bibek Bhandari , Andrew N. Jordan

Recent experiments demonstrate a temperature control of the electric conduction through a ferrocene-based molecular junction. Here we examine the results in view of determining means to distinguish between transport through single-particle…

Mesoscale and Nanoscale Physics · Physics 2018-02-23 Miguel A. Sierra , David Sánchez , Alvar R. Garrigues , Enrique del Barco , Lejia Wang , Christian A. Nijhuis

A self-consistent method for calculating electron transport through a molecular device is proposed. It is based on density functional theory electronic structure calculations under periodic boundary conditions and implemented in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

We consider bosonic transport through one-dimensional spin systems. Transport is induced by coupling the spin systems to bosonic reservoirs kept at different temperatures. In the limit of weak-coupling between spins and bosons we apply the…

Statistical Mechanics · Physics 2014-05-26 Gernot Schaller , Malte Vogl , Tobias Brandes

Using a model comprising a 2-level bridge connecting free electron reservoirs we show that coupling of a molecular bridge to electron-hole excitations in the leads can markedly effect the source-drain current through a molecular junction.In…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

We demonstrate electronic cooling of a suspended AuPd island using superconductor-insulator-normal metal tunnel junctions. This was achieved by developing a simple fabrication method for reliably releasing narrow submicron sized metal…

Mesoscale and Nanoscale Physics · Physics 2009-02-25 J. T. Muhonen , A. O. Niskanen , M. Meschke , Yu. A. Pashkin , J. S. Tsai , L. Sainiemi , S. Franssila , J. P. Pekola

We present a microscopic laser model for many atoms coupled to a single cavity mode, including the light forces resulting from atom-field momentum exchange. Within a semiclassical description, we solve the equations for atomic motion and…

Quantum Physics · Physics 2007-12-18 Thomas Salzburger Helmut Ritsch

This brief review presents the emerging field of mesoscopic physics with cold atoms, with an emphasis on thermal and 'thermoelectric' transport, i.e. coupled transport of particle and entropy. We review in particular the comparison between…

Quantum Gases · Physics 2016-12-21 Charles Grenier , Corinna Kollath , Antoine Georges

We investigate nonlinear thermal transport properties of a single interacting quantum dot with two energy levels tunnel-coupled to two electrodes using nonequilibrium Green function method and Hartree-Fock decoupling approximation. In the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Chen Xue-Ou , Bing Dong , X. L. Lei

We consider resonant transmission through a finite-length quantum wire connected to leads via finite transparency junctions. The coherent electron transport is strongly modified by the Coulomb interaction. The low-temperature…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 N. B. Kopnin , Y. M. Galperin , V. M. Vinokur

Atomic and single-molecule junctions represent the ultimate limit to the miniaturization of electrical circuits. They are also ideal platforms to test quantum transport theories that are required to describe charge and energy transfer in…

Mesoscale and Nanoscale Physics · Physics 2013-08-01 Woochul Lee , Kyeongtae Kim , Wonho Jeong , Linda Angela Zotti , Fabian Pauly , Juan Carlos Cuevas , Pramod Reddy