Related papers: Auger decay in krypton induced by attosecond pulse…
Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…
The surface effect and quantum confinement render nanomaterials the optoelectronic properties more susceptible to nonradiative processes than their bulk counterparts. These nonradiative processes usually contain a series of interwoven and…
In this study, we discovered that the energy gap above the vacuum level in the projected bulk band structure of Ag(100) prevents electrons in the first-order field emission resonance (FER) from inducing the surface plasmons. This mechanism…
We discuss a new strategy to compute partial Auger decay widths with equation-of-motion ionisation-potential coupled-cluster (EOMIP-CCSD) wave functions in the framework of non-Hermitian quantum mechanics, where the decaying character of…
In the field of chemistry, where nuclear motion has traditionally been a focal point, we now explore the ultra-rapid electronic motion spanning attoseconds to femtoseconds, demonstrating that it is equally integral and relevant to the…
We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…
High harmonic light sources make it possible to access attosecond time-scales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics,…
Nuclear orbiting resonances have been revealed at the sub-barrier energies as an atomic phenomenon by means of x-ray spectroscopy experiments. This interpretation is supported by several phenomenological models and theoretical estimates of…
Preliminary results are presented from a new positron beam system currently under development at the University of Texas at Arlington for the coincident energy measurement of Doppler-shifted annihilation quanta and positron-induced Auger…
In semiconductor nanostructures nonradiative Auger recombination is enhanced by the presence of boundaries which relax the momentum conservation and thereby removes the threshold reduction for these processes. We propose a method to…
The peculiar electron dispersion in Dirac materials makes lowest-order Auger processes prohibited or marginally prohibited by energy and momentum conservation laws. Thus, Auger recombination (AR) in these materials is very sensitive to…
We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…
In a recent publication [B. Schuette, S. Bauch et al., accepted for publication in Phys. Rev. Lett. 2012] it was demonstrated both, experimentally and theoretically, that Auger electrons are subject to an energetic chirp if a…
We describe a new instrument, the Argonne Auger Radioisotope Microscope (ARM), capable of characterizing the Auger electron emission of radionuclides, including candidates relevant in nuclear medicine. Our approach relies on event-by-event…
We investigate the \alpha-decay of a spherical nucleus under the influence of an ultra-intense laser field for the case when the radius vector joining the center-of-masses of the \alpha-particle and the daughter is aligned with the…
Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…
We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…
A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…
We experimentally investigate the impact of pulse shape on the dynamics of laser-generated plasma in rare gases. Fast-rising triangular pulses with a slower decay lead to early ionization of the air and depose energy more efficiently than…
An interaction of a pseudoscalar particle with two photons induced by an external electromagnetic field is used to study the photon decay $\gamma \to \gamma a$ where a is a pseudoscalar particle associated with the Peccei-Quinn U(1)…