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A model subspace configuration interaction method is developed to obtain chemically accurate electron correlations by diagonalising a very compact effective Hamiltonian of realistic molecule. The construction of the effective Hamiltonian is…

Chemical Physics · Physics 2022-10-18 Jiasheng Li , Jun Yang

An accurate determination of the electron correlation energy is essential for describing the structure, stability, and function in a wide variety of systems, ranging from gas-phase molecular assemblies to condensed matter and…

Chemical Physics · Physics 2014-03-05 Alberto Ambrosetti , Anthony M. Reilly , Robert A. DiStasio , Alexandre Tkatchenko

We theoretically characterize interactions, energetics, and chemical reaction paths in ionic two-body and three-body systems of alkali-metal and alkaline-earth-metal atoms in the context of modern experiments with cold hybrid ion-atom…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

We report the implementation of equation-of-motion coupled-cluster (EOMCC) method in the four-component relativistic framework with the spherical atomic potential to generate the excited states from a closed-shell atomic configuration. This…

Atomic Physics · Physics 2015-06-19 D. K. Nandy , Yashpal Singh , B. K. Sahoo

We calculate excitation energies for low states of nobelium, including states with open $5f$ subshell. An efficient version of the many-electron configuration-interaction method for treating the atom as a sixteen external electrons system…

Atomic Physics · Physics 2019-03-13 V. A. Dzuba , V. V. Flambaum , M. G. Kozlov

Atomic high-precision measurements have become a competitive and essential technique for tests of fundamental physics, the Standard Model, and our theory of gravity. It is therefore self-evident that such measurements call for a consistent…

Quantum Physics · Physics 2024-05-24 Tobias Asano , Enno Giese , Fabio Di Pumpo

The beginning of the application of the method of interacting configurations in the complex number representation to the compound atomic systems has been presented. The spectroscopic characteristics of the Be atom in the problem of the…

Atomic Physics · Physics 2016-08-16 V. M. Simulik , T. M. Zajac , R. V. Tymchyk

A new relativistic method for calculation of positron binding to atoms is presented. The method combines a configuration interaction treatment of the valence electron and the positron with a many-body perturbation theory description of…

Atomic Physics · Physics 2009-10-31 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin , C. Harabati

We use all-order relativistic many-body perturbation theory to study 5s^2 nl configurations of In I and Sn II. Energies, E1-amplitudes, and hyperfine constants are calculated using all-order method, which accounts for single and double…

Atomic Physics · Physics 2015-05-13 U. I. Safronova , M. S. Safronova , M. G. Kozlov

Recently, a method was developed for implementing arbitrary short-range nucleon-nucleon correlations in Monte Carlo sampled nuclei (as well as deformations of the 1-body nuclear density). We use this method to implement realistic 2-body…

Nuclear Theory · Physics 2023-12-19 Matthew Luzum , João Paulo Picchetti , Mauricio Hippert , Jean-Yves Ollitrault

We study the effects of higher-order electronic correlations in the systems with particle-hole excited states using a relativistic hybrid method that combines configuration interaction and linearized coupled-cluster approaches. We find the…

Atomic Physics · Physics 2018-01-31 M. S. Safronova , U. I. Safronova , M. G. Kozlov

We present and analyze results of the relativistic coupled-cluster calculation of energies, hyperfine constants, and dipole matrix elements for the $2s$, $2p_{1/2}$, and $2p_{3/2}$ states of Li atom. The calculations are complete through…

Atomic Physics · Physics 2011-07-13 A. Derevianko , S. G. Porsev , K. Beloy

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo

Correlations play a crucial role in the nuclear many-body problem. We give an overview of recent developments in nuclear structure theory aiming at the description of these interaction-induced correlations by unitary transformations. We…

Nuclear Theory · Physics 2010-06-08 Robert Roth , Thomas Neff , Hans Feldmeier

Relativistic third-order MBPT is applied to obtain energies of ions with two valence electrons in the no virtual-pair approximation (NVPA). A total of 302 third-order Goldstone diagrams are organized into 12 one-body and 23 two-body terms.…

Atomic Physics · Physics 2009-11-11 H. C. Ho , W. R. Johnson , S. A. Blundell , M. S. Safronova

Relativistic Hartree-Fock method together with many-body perturbation theory and configuration interaction techniques are used to calculate relativistic energy shifts for frequencies of the strong electric dipole transitions of C III, C IV,…

Atomic Physics · Physics 2007-10-26 I. M. Savukov , V. A. Dzuba

Accurate atomic structure calculations of complicated atoms with 4 or more valence electrons begin to push the memory and time limits of supercomputers. This paper presents a robust method of decreasing the size of \textit{ab initio}…

Atomic Physics · Physics 2018-10-24 A. J. Geddes , D. A. Czapski , E. V. Kahl , J. C. Berengut

The many-body Coulomb repulsive energy of strictly correlated electrons provides direct information of the exact Hohenberg-Kohn exchange-correlation functional in the strong interaction limit. Until now the treatment of strictly correlated…

Chemical Physics · Physics 2013-03-13 Christian B. Mendl , Lin Lin

We present a mathematically rigorous method suitable for solving three-body bound state and scattering problems when the inter-particle interaction is of a hard-core nature. The proposed method is a variant of the Boundary Condition Model…

Chemical Physics · Physics 2008-02-03 E. A. Kolganova , A. K. Motovilov , S. A. Sofianos

Fully relativistic approach to evaluate the correlation effects in highly charged ions is presented. The interelectronic-interaction contributions of first and second orders in $1/Z$ are treated rigorously within the framework of…

Atomic Physics · Physics 2019-12-18 Y. S. Kozhedub , A. V. Malyshev , D. A. Glazov , V. M. Shabaev , I. I. Tupitsyn