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One- and multi-phonon excitations of the single crystalline LaCoO3 were studied using Raman spectroscopy in the temperature region of 5 K - 300 K. First-order Raman spectra show a larger number of phonon modes than allowed for the…

Strongly Correlated Electrons · Physics 2022-05-31 V. Gnezdilov , K. -Y. Choi , Yu. Pashkevich , P. Lemmens , S. Shiryaev , G. Bychkov , S. Barilo , V. Fomin , A. V. Yeremenko

We report an inelastic light scattering study of single-crystalline NaCu$_2$O$_2$, a spin-chain compound known to exhibit a phase with helical magnetic order at low temperatures. Phonon excitations were studied as a function of temperature…

Strongly Correlated Electrons · Physics 2009-11-11 K. -Y. Choi , V. P. Gnezdilov , P. Lemmens , L. Capogna , M. R. Johnson , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

The magnetic susceptibility between 1.5 and 800 K, the infrared reflectivity at room temperature and the temperature dependence of the dielectric constant at mm-wavelengths are reported for single crystalline BiFeO3. A well developed…

Strongly Correlated Electrons · Physics 2010-07-22 Jun Lu , M Schmidt , P Lunkenheimer , A Pimenov , A A Mukhin , V D Travkin , A Loidl

The sequence of phase transitions in PbHf0.83Sn0.17O3 has been studied by THz, far infrared and Raman spectroscopies, revealing the complementary behaviour of both, polar and non-polar phonons and their impact on the transition lattice…

The spin-driven polarizations of type-I multiferroics are veiled by the preexisting ferroelectric (FE) polarization. Using first-principles calculations combined with a spin model, we uncover two hidden but huge spin-driven polarizations in…

Strongly Correlated Electrons · Physics 2015-04-28 Jun Hee Lee , Randy S. Fishman

Resonant and non-resonant X-ray scattering studies on HoFe3(BO3)O4 reveal competing magnetic ordering of Ho and Fe moments. Temperature and X-ray polarization dependent measurements employed at the Ho L3 edge directly reveal a spiral spin…

Strongly Correlated Electrons · Physics 2013-04-05 D. K. Shukla , S. Francoual , A. Skaugen , M. v. Zimmermann , H. C. Walker , L. N. Bezmaternykh , I. A. Gudim , V. L. Temerov , J. Strempfer

We have investigated the temperature evolution of the magnetic structures of HoFeO$_3$ by single crystal neutron diffraction. The three different magnetic structures found as a function of temperature for \hfo\ are described by the magnetic…

Materials Science · Physics 2016-04-29 T. Chatterji , M. Meven , P. J. Brown

We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…

Materials Science · Physics 2007-10-16 R. Tackett , G. Lawes , B. C. Melot , M. Grossman , E. S. Toberer , R. Seshadri

In metals in the vicinity of a polar transition, interactions between electrons and soft phonon modes remain to be determined. Here we explore the consequences of spin-orbit assisted electron-phonon coupling on the collective modes of such…

Strongly Correlated Electrons · Physics 2023-12-27 Abhishek Kumar , Premala Chandra , Pavel A. Volkov

EuTiO3 (ETO) has recently experienced an enormous revival of interest because of its possible multiferroic properties which are currently in the focus of research. Unfortunately ETO is an unlikely candidate for enlarged multifunctionality…

Materials Science · Physics 2015-06-05 A. Bussmann-Holder , Z. Guguchia , J. Köhler , H. Keller , A. Shengelaya , A. R. Bishop

We report on bifurcations effect mediated by the electron-phonon coupling in a concentrated rare-earth-containing antiferromagnet, observed in the spectra of coupled $4f$-electron-phonon modes under the influence of an external magnetic…

We report a comprehensive study of the low-level substitution of Mn$^{3+}$ by Fe$^{3+}$ effect on the static and dynamic magnetoelectric coupling in TbMn$_{1-x}$Fe$_x$O$_3$ ($x=0$, 0.02 and 0.04). The cationic substitution has a large…

Materials Science · Physics 2023-03-14 A. Maia , R. Vilarinho , C. Kadlec , M. Lebeda , M. Mihalik, , M. Zentková , M. Mihalik , J. Agostinho Moreira , S. Kamba

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

Exciton dynamics can be strongly affected by lattice vibrations through electron-phonon coupling. This is rarely explored in two-dimensional magnetic semiconductors. Focusing on bilayer CrI3, we first show the presence of strong…

Bismuth ferrite, BiFeO3, is the only known room-temperature 'multiferroic' material. We demonstrate here, using neutron scattering measurements in high quality single crystals, that the antiferromagnetic and ferroelectric orders are…

Materials Science · Physics 2009-11-13 D. Lebeugle , D. Colson , A. Forget , M. Viret , A. M. Bataille , A. Gukasov

We have performed Raman measurements on TbMnO3 single crystal under magnetic field along the three crystallographic directions. The flip of the spin spiral plane creates an electromagnon excitation. In addition to the electromagnons induced…

Strongly Correlated Electrons · Physics 2015-06-05 P. Rovillain , J. Liu , M. Cazayous , Y. Gallais , M. -A. Measson , H. Sakata , A. Sacuto

Low-energy magnon excitations in multiferroic BiFeO$_3$ were measured in detail as a function of temperature around several Brillouin zone centers by inelastic neutron scattering experiments on single crystals. Unique features around 1 meV…

Materials Science · Physics 2014-09-15 Jaehong Jeong , Manh Duc Le , P. Bourges , S. Petit , S. Furukawa , Shin-Ae Kim , Seongsu Lee , S-W. Cheong , Je-Geun Park

We used Raman and terahertz spectroscopies to investigate lattice and magnetic excitations and their cross-coupling in the hexagonal YMnO3 multiferroic. Two phonon modes are strongly affected by the magnetic order. Magnon excitations have…