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The first X-ray magnetic circular dichroism (XMCD) spectra on the title compounds are presented. In Mn12 the Mn(III) and Mn(IV) contributions are clearly apparent and evidence the opposite spin arrangement of the two ions. For Fe8 the…

Solid solutions of the magnetic insulators Ba3Cr2O8 and Sr3Cr2O8 (Ba3-xSrxCr2O8) have been prepared in polycrystalline form for the first time. Single crys- talline material was obtained using a mirror image floating zone technique. X-ray…

Strongly Correlated Electrons · Physics 2013-04-18 Henrik Grundmann , Andreas Schilling , Casey A. Marjerrison , Hanna A. Dabkowska , Bruce D. Gaulin

Magnetization and neutron diffraction measurements indicate long-range antiferromagnetic ordering below TN=4 K in the 2D, S=1/2 Heisenberg antiferromagnet K2V3O8. The ordered state exhibits ``weak ferromagnetism'' and novel, field-induced…

Strongly Correlated Electrons · Physics 2009-10-31 M. D. Lumsden , B. C. Sales , D. Mandrus , S. E. Nagler , J. R. Thompson

The mixed-valent iridate Ba3InIr2O9 has been discussed as a promising candidate for quantum spin-liquid behavior. The compound exhibits Ir$^{4.5+}$ ions in face-sharing IrO6 octahedra forming Ir2O9 dimers with three t2g holes per dimer. Our…

We report the synthesis and measurements of magnetic, transport, and thermal properties of polycrystalline Nb0.18Re0.82, which has a superconducting transition at Tc ~ 8.8 K. The non-centrosymmetric alpha-Mn structure of the compound is…

The spin dimer system $\mathrm{Ba}_{3-x}\mathrm{Sr}_x\mathrm{Cr_2O_8}$ is a solid solution of the triplon Bose-Einstein condensation candidates $\mathrm{Ba_3Cr_2O_8}$ and $\mathrm{Sr_3Cr_2O_8}$. The magnetic intradimer interaction constant…

Strongly Correlated Electrons · Physics 2015-06-19 Henrik Grundmann , Marisa Medarde , Denis Sheptyakov , Andreas Schilling

We study the ground state and spin excitations in Ba3MnSb2O9, an easy-plane S = 5/2 triangular lattice antiferromagnet. By combining single-crystal neutron scattering, electric spin resonance (ESR), and spin wave calculations, we determine…

BaCo2(AsO4)2 (BCAO) has seen extensive study since its initial identification as a proximate Kitaev quantum spin liquid candidate. Thought to be described by the highly anisotropic XXZ-J_1-J_3 model, the ease with which magnetic order is…

A bulk diluted magnetic semiconductor was found in the K and Mn co-doped BaCd2As2 system. Different from recently reported tetragonal ThCr2Si2-structured II-II-V based(Ba,K)(Zn,Mn)2As2, the Ba1-yKyCd2-xMnxAs2 system has a hexagonal…

Strongly Correlated Electrons · Physics 2014-01-06 Xiaojun Yang , Yuke Li , Pan Zhang , Hao Jiang , Yongkang Luo , Qian Chen , Chunmu Feng , Chao Cao , Jianhui Dai , Qian Tao , Guanghan Cao , Zhu-an Xu

Molecular based spin-1/2 triangular lattice systems such as LiZn$_2$Mo$_3$O$_8$ have attracted research interest. Distortions, defects, and intersite disorder are suppressed in such molecular-based magnets, and intrinsic geometrical…

Strongly Correlated Electrons · Physics 2019-02-19 K. Iida , H. Yoshida , H. Okabe , N. Katayama , Y. Ishii , A. Koda , Y. Inamura , N. Murai , M. Ishikado , R. Kadono , R. Kajimoto

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

Electrical resistivity, specific heat and NMR measurements classify non-centrosymmetric $\rm Mo_3Al_2C$ ($\beta$-Mn type, space group $P4_132$) as a strong-coupled superconductor with $T_c = 9$~K deviating notably from BCS-like behaviour.…

We present inelastic neutron scattering and thermodynamic measurements characterizing the magnetic excitations in a disordered non-magnetic substituted spin-liquid antiferromagnet. The parent compound Ba3Mn2O8 is a dimerized,…

Strongly Correlated Electrons · Physics 2015-05-20 M. B. Stone , A. Podlesnyak , G. Ehlers , A. Huq , E. C. Samulon , M. C. Shapiro , I. R. Fisher

Dimethylammonium copper (II) chloride (also known as DMACuCl3 or MCCL) is a low dimensional S=1/2 quantum spin system proposed to be an alternating ferro-antiferromagnetic chain with similar magnitude ferromagnetic (FM) and…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , W. Tian , G. E. Granroth , M. D. Lumsdena , J-H. Chung , D. G. Mandrusa , S. E. Nagler

We present a model of equal spin $s_1$ dimer single molecule magnets. The spins within each dimer interact via the Heisenberg and the most general set of four quadratic anisotropic spin interactions with respective strengths $J$ and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dmitri V. Efremov , Richard A. Klemm

The magnetic properties and the electronic excitations of the new diluted magnetic semiconductor Ba$_{1-x}$K$_{x}$(Zn$_{1-y}$Mn$_{y}$)$_{2}$As$_{2}$ have been studied by x-ray magnetic circular dichroism (XMCD) and resonant inelastic x-ray…

We investigated the static and dynamic magnetic properties of the polar ferrimagnet Mn$_2$Mo$_3$O$_8$ in three magnetically ordered phases via magnetization, magnetic torque, and THz absorption spectroscopy measurements. The observed…

The presence of spin-orbit (SO) interaction in a noncentrosymmetric superconductor, La2C3 (T_c~11 K) is demonstrated by muon spin rotation (muSR) in its normal state, where muSR spectra exhibit field-induced weak depolarization due to van…

Superconductivity · Physics 2009-11-13 R. Kadono , M. Hiraishi , M. Miyazaki , K. H. Satoh , S. Takeshita , S. Kuroiwa , S. Saura , J. Akimitsu

The dimerized quantum magnet BaCuSi$_2$O$_6$ was proposed as an example of "dimensional reduction" arising near the magnetic-field-induced quantum critical point (QCP) due to perfect geometrical frustration of its inter-bilayer…

Strongly Correlated Electrons · Physics 2020-05-08 S. Allenspach , A. Biffin , U. Stuhr , G. S. Tucker , S. Ohira-Kawamura , M. Kofu , D. J. Voneshen , M. Boehm , B. Normand , N. Laflorencie , F. Mila , Ch. Rüegg

We present a numerical study of the spin-1/2 bilayer Heisenberg antiferromagnet with random interlayer dimer dilution. From the temperature dependence of the uniform susceptibility and a scaling analysis of the spin correlation length we…

Disordered Systems and Neural Networks · Physics 2009-11-07 O. P. Vajk , M. Greven