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Magnetometry, electrical transport, and neutron scattering measurements were performed on single crystals of the Fe^{4+}-containing perovskite-related phase Sr_3Fe_2O_7-x as a function of oxygen content. Although both the crystal structure…

Strongly Correlated Electrons · Physics 2013-06-12 D. C. Peets , J. -H. Kim , P. Dosanjh , M. Reehuis , A. Maljuk , N. Aliouane , C. Ulrich , B. Keimer

The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (\textit{e.g.} Pb, I) makes these materials interesting for applications in spintronics. Due to a lack of inversion symmetry…

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central…

The synergistic interplay of different interactions in materials leads to the emergence of novel quantum phenomena. Spin-orbit and vibronic couplings usually counteract each other, however, in cubic $d^1$ double perovskites they coexist and…

Strongly Correlated Electrons · Physics 2023-06-21 Naoya Iwahara , Liviu F. Chibotaru

We report a thorough study of Y$_{0.7}$La$_{0.3}$VO$_3$ single crystals by measuring magnetic properties, specific heat, thermal conductivity, x-ray and neutron diffraction with the motivation of revealing the lattice response to the…

Strongly Correlated Electrons · Physics 2019-12-04 J. -Q. Yan , W. Tian , H. B. Cao , S. Chi , F. Ye , A. Llobet , Q. Chen , J. Ma , Y. Ren , J. -G. Cheng , J. -S. Zhou , M. A. McGuire , R. J. McQueeney

Compounds with distorted perovskite structure of the 4-f and 3-d transition metals with the common formula LnTO3 (where Ln is rare-earth element, T is an element from the Fe group) are the most multifold binary oxides of these two groups…

Strongly Correlated Electrons · Physics 2007-05-23 D. Dimitrov , I. Radulov , V. Lovchinov , A. Apostolov

We investigated the electronic properties of epitaxially stabilized perovskite SrIrO3 and demonstrated the effective strain-control on its electronic structure. Comprehensive transport measurements showed that the strong spin-orbit coupling…

We investigated the electronic structures of the perovskite-type 4$d$ transition metal oxides Sr$M$O$_3$ ($M$ = Zr, Mo, Ru, and Rh) using their optical conductivity spectra $\sigma (\omega)$. The interband transitions in $\sigma (\omega)$…

Strongly Correlated Electrons · Physics 2009-11-07 Y. S. Lee , J. S. Lee , T. W. Noh , Douck-Young Byun , Kwang Soo Yoo , K. Yamaura , E. Takayama-Muromachi

Using density functional theory plus Hubbard $U$ calculations, we show that the ground state of (Mg,Fe)(Si,Fe)O$_3$ perovskite, a major mineral phase in the Earth's lower mantle, has high-spin ferric iron ($S=5/2$) at both the dodecahedral…

Geophysics · Physics 2015-05-27 Han Hsu , Peter Blaha , Matteo Cococcioni , Renata M. Wentzcovitch

We report time-of-flight neutron spectroscopic and diffraction studies of the 5$d^2$ cubic double pervoskite magnets, Ba$_2$MOsO$_6$ ($M$ = Zn, Mg, Ca). These cubic materials are all described by antiferromagnetically-coupled 5$d^2$…

Dislocations in perovskite oxides have important impacts on their physical and chemical properties, which are determined by their unique atomic environments. In the present study, the structure of dislocations in a 10{\deg} low-angle grain…

Materials Science · Physics 2020-01-08 Xujing Li , Shulin Chen , Mingqiang Li , Jingmin Zhang , Xiumei Ma , Kaihui Liu , Xuedong Bai , Peng Gao

A comparative density functional plus dynamical mean field theory study of the pseudocubic ruthenate materials CaRuO$_3$ and SrRuO$_3$ is presented. Phase diagrams are determined for both materials as a function of Hubbard repulsion $U$ and…

Strongly Correlated Electrons · Physics 2015-06-02 Hung T. Dang , Jernej Mravlje , Antoine Georges , Andrew J. Millis

Using inelastic magnetic neutron scattering we have discovered a localized spin resonance at 4.5 meV in the ordered phase of the geometrically frustrated cubic antiferromagnet $\rm ZnCr_2O_4$. The resonance develops abruptly from quantum…

Strongly Correlated Electrons · Physics 2009-10-31 S. -H. Lee , C. Broholm , T. H. Kim , W. Ratcliff , S-W. Cheong

A major impediment towards realizing technologies based on the emerging principles of antiferromagnetic spintronics is the shortage of suitable materials. In this paper, we propose a design of polar|nonpolar heterostructures of perovskite…

Materials Science · Physics 2020-12-23 Jayita Chakraborty , Nirmal Ganguli

Measuring the ESR of Gd spin probes we have studied the magnetic properties of the copper oxide planes in the low temperature tetragonal (LTT) phase of Eu doped La_{2-x}Sr_xCuO_4. The data give evidence that at particular levels of Sr and…

Superconductivity · Physics 2009-10-28 V. Kataev , B. Rameev , B. Buechner , M. Huecker , R. Borowski

We demonstrated experimentally a direct way to probe a hidden propensity to the formation of spin density wave (SDW) in a non-magnetic metal with strong Fermi surface nesting. Substituting Fe for a tiny amount of Cu (1%) induced an…

Superconductivity · Physics 2011-09-16 Rui-Hua He , M. Fujita , M. Enoki , M. Hashimoto , S. Iikubo , S. -K. Mo , Hong Yao , T. Adachi , Y. Koike , Z. Hussain , Z. -X. Shen , K. Yamada

We have investigated the electronic structure of rare-earth tetraborides, $\textrm{RB}_{4}$, using first-principle electronic structure methods (DFT) implemented in Quantum Espresso (QE). In this article we have studied heather-to neglected…

Strongly Correlated Electrons · Physics 2023-03-22 Ismail Sk , Nandan Pakhira

The orthorhombic perovskite NaOsO3 undergoes a continuous metal-insulator transition (MIT), accompanied by antiferromagnetic (AFM) order at T_N=410 K, suggested to be an example of the rare Slater (itinerant) MIT. We study this system using…

Strongly Correlated Electrons · Physics 2013-03-15 Myung-Chul Jung , Young-Joon Song , K. -W. Lee , W. E. Pickett

Perovskites like LaAlO3, (or SrTiO3) undergo displacive structural phase transitions from a cubic crystal to a trigonal (or tertagonal) structure. For many years, the critical exponents in both these types of transitions have been fitted to…

Statistical Mechanics · Physics 2022-02-21 Amnon Aharony , Ora Entin-Wohlman

In the series of 3d1 t2g perovskites, SrVO3--CaVO3--LaTiO3--YTiO3 the transition-metal d electron becomes increasingly localized and undergoes a Mott transition between CaVO3 and LaTiO3. By defining a low-energy Hubbard Hamiltonian in the…

Strongly Correlated Electrons · Physics 2009-09-29 E. Pavarini , A. Yamasaki , J. Nuss , O. K. Andersen