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Recent high resolution measurements of the momenta of two electrons emitted from Argon atoms in a strong laser field show a strong preference for the outgoing electrons to have similar momenta and to be ejected in the same direction along…

Atomic Physics · Physics 2007-05-23 Bruno Eckhardt , Krzysztof Sacha

Double ionization in intense laser fields can comprise electron correlations, which manifest in the non-independent emission of two electrons from an atom or molecule. However, experimental methods that directly access the electron emission…

We report a novel experimental technique for the comparison of ionization processes in ultrafast laser pulses irrespective of pulse ellipticity. Multiple ionization of xenon by 50 fs 790 nm, linearly and circularly polarized laser pulses is…

A three-dimensional semiclassical model is used to study double ionization of Ar when driven by a near-infrared and near-single-cycle laser pulse for intensities ranging from 0.85$\times$10$^{14}$ W/cm$^{2}$ to 5$\times$10$^{14}$…

Atomic Physics · Physics 2017-02-15 A. Chen , M. Kübel , B. Bergues , M. F. Kling , A. Emmanouilidou

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

Atomic Physics · Physics 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We present a detailed study of the ionisation probability of H and H$_{2}^{+}$ induced by a short intense laser pulse. Starting from a Coulomb-Volkov description of the process we derive a multipole-like expansion where each term is…

Atomic Physics · Physics 2013-07-11 Renata Della Picca , Juan Fiol , Pablo Daniel Fainstein

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

The formation of an electron-hole plasma during the interaction of intense femtosecond laser pulses with transparent solids lies at the heart of femtosecond laser processing. Advanced micro- and nanomachining applications require improved…

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry…

Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…

Atomic Physics · Physics 2009-11-13 D. A. Horner , T. N. Rescigno , C. W. McCurdy

The process of nonsequential two-photon double ionization of helium is studied by two complementary numerical approaches. First, the time-dependent Schr{\"o}dinger equation is solved and the final wave function is analyzed in terms of…

Quantum Physics · Physics 2010-09-13 Sølve Selstø , Tore Birkeland , Simen Kvaal , Raymond Nepstad , Morten Førre

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

We use classical electron ensembles and the aligned-electron approximation to examine the effect of laser pulse duration on the dynamics of strong-field double ionization. We cover the range of intensities $10^{14}-10^{16} W/cm^2$ for the…

Atomic Physics · Physics 2007-05-23 Phay J. Ho , J. H. Eberly

We discuss the final stages of the simultaneous ionization of two or more electrons due to a strong laser pulse. An analysis of the classical dynamics suggests that the dominant pathway for non-sequential escape has the electrons escaping…

Quantum Physics · Physics 2009-11-06 Bruno Eckhardt , Krzysztof Sacha

When a diatomic molecule is ionized by an intense laser field, the ionization rate depends very strongly on the inter-nuclear separation. That dependence exhibits a pronounced maximum at the inter-nuclear separation known as the critical…

Chemical Physics · Physics 2015-04-21 Han Xu , Feng He , D. Kielpinski , R. T. Sang , I. V. Litvinyuk

Single ionization of H$_2$ molecules exposed to strong and short laser pulses is investigated by a semi-classical method. Three laser characteristics are considered: i) The carrier-wave frequency corresponds to wavelengths covering and…

Atomic Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , O. Atabek , Thanh-Tung Nguyen-Dang , Eric Charron

We analyze the dynamical processes behind delayed double ionization of atoms subjected to strong laser pulses. Using reduced models, we show that these processes are a signature of Hamiltonian chaos which results from the competition…

Atomic Physics · Physics 2012-06-19 Francois Mauger , Adam Kamor , Cristel Chandre , Turgay Uzer