English
Related papers

Related papers: Self diffusion and binary Maxwell-Stefan diffusion…

200 papers

Self- and binary Maxwell-Stefan diffusion coefficients were determined by equilibrium molecular dynamics simulations with the Green-Kubo method. This study covers self-diffusion coefficients at liquid states for eight pure fluids, i.e.…

Chemical Physics · Physics 2009-04-30 Gimmy Alex Fernandez Ramirez , Jadran Vrabec , Hans Hasse

Shear and bulk viscosity and thermal conductivity for argon, krypton, xenon, and methane and the binary mixtures argon+krypton and argon+methane were determined by equilibrium molecular dynamics with the Green-Kubo method. The fluids were…

Chemical Physics · Physics 2009-06-10 G. A. Fernandez , J. Vrabec , H. Hasse

The linear response description for impurity diffusion in a granular fluid undergoing homogeneous cooling is developed in the preceeding paper. The formally exact Einstein and Green-Kubo expressions for the self-diffusion coefficient are…

Soft Condensed Matter · Physics 2009-11-07 James Lutsko , J. Javier Brey , James W. Dufty

We study a kinetic model for non-reactive mixtures of monatomic gases with hard-sphere cross-sections under isothermal condition. By considering a diffusive scaling of the kinetic model and using the method of moments, we formally obtain…

Computational Physics · Physics 2020-04-24 Benjamin Anwasia

Transport properties of liquid methanol and ethanol are predicted by molecular dynamics simulation. The molecular models for the alcohols are rigid, non-polarizable and of united-atom type. They were developed in preceding work using…

Chemical Physics · Physics 2009-06-10 Gabriela Guevara-Carrion , Carlos Nieto-Draghi , Jadran Vrabec , Hans Hasse

We present a method to measure the binary diffusion coefficient of mercury atoms in a gas at room temperature and low pressure. It is based on the measurement of the longitudinal spin relaxation of optically pumped mercury-199 atoms in a…

Atomic Physics · Physics 2022-12-20 B. Clément , M. Guigue , A. Leredde , G. Pignol , D. Rebreyend , S. Roccia , S. Touati

We study the diffusion of tracers (self-diffusion) in a homogeneously cooling gas of dissipative particles, using the Green-Kubo relation and the Chapman-Enskog approach. The dissipative particle collisions are described by the coefficient…

Statistical Mechanics · Physics 2009-11-11 Nikolai V. Brilliantov , Thorsten Poeschel

Equilibrium molecular dynamics simulation and the Green-Kubo formalism were used to calculate self-diffusion coefficient, shear viscosity, and thermal conductivity for 38 different dipolar two-center Lennard-Jones fluids along the bubble…

Chemical Physics · Physics 2009-06-18 G. A. Fernandez , J. Vrabec , H. Hasse

We present a systematic study of the self-diffusion coefficient for a fluid of particles interacting via the square-well pair potential by means of molecular dynamics simulations in the canonical (N,V,T) ensemble. The discrete nature of the…

Soft Condensed Matter · Physics 2018-11-14 Alexis Torres-Carbajal , Victor M. Trejos , Luz Adriana Nicasio-Collazo

In this article we deduce a mathematical model of Maxwell-Stefan type for a reactive mixture of polyatomic gases with a continuous structure of internal energy. The equations of the model are derived in the diffusive limit of a kinetic…

Analysis of PDEs · Mathematics 2019-11-18 Benjamin Anwasia , Marzia Bisi , Francesco Salvarani , Ana Jacinta Soares

In this work, we have estimated self diffusion coefficients along with the binary diffusion coefficients of mixtures of alkane (methane, ethane, propane and n-butane) in SPC/E water(H$_2$O). Molecular dynamics study of a binary mixture of…

The paper studies a higher-order diffusion model of Maxwell-Stefan kind. The model is based upon higher-order moment equations of kinetic theory of mixtures, which include viscous dissipation in the model. Governing equations are analyzed…

Analysis of PDEs · Mathematics 2023-05-16 Bérénice Grec , Srboljub Simic

In this paper we perform a formal asymptotic analysis on a kinetic model for reactive mixtures in order to derive a reaction-diffusion system of Maxwell-Stefan type. More specifically, we start from the kinetic model of simple reacting…

Fluid Dynamics · Physics 2019-11-20 Benjamin Anwasia , Patrícia Gonçalves , Ana Jacinta Soares

Equilibrium molecular dynamics simulation and the Green-Kubo formalism were used to calculate self-diffusion coefficient, shear viscosity,and thermal conductivity for 30 different quadrupolar two-center Lennard-Jones fluids along the bubble…

Chemical Physics · Physics 2009-06-18 G. A. Fernandez , J. Vrabec , H. Hasse

This paper explores the mathematical formulations of Fick and Maxwell-Stefan diffusion in the context of polymer electrolyte membrane fuel cell cathode gas diffusion layers. Formulations of diffusion combined with mass-averaged Darcy flow…

Fluid Dynamics · Physics 2013-12-06 Michael Lindstrom , Brian Wetton

A symmetrical binary, A+B Lennard-Jones mixture is studied by a combination of semi-grandcanonical Monte Carlo (SGMC) and Molecular Dynamics (MD) methods near a liquid-liquid critical temperature $T_c$. Choosing equal chemical potentials…

Statistical Mechanics · Physics 2009-11-11 Subir K. Das , Juergen Horbach , Kurt Binder , Michael E. Fisher , Jan V. Sengers

The applicability of theories describing the kinetic evolution of fluid mixtures depends on the underlying physical assumptions. The Maxwell-Stefan equations, widely used for miscible fluids, express forces depending on coupled fluxes. They…

Chemical Physics · Physics 2019-08-21 Olivier J. J. Ronsin , Jens Harting

Much effort has been put into developing theories for dense fluids, as a result of these efforts many theories work for a certain type of particle or in a certain concentration regime. Rosenfeld proposed a dependence of the self-diffusion…

Statistical Mechanics · Physics 2023-12-22 Melina Sampayo Puelles , Miguel Hoyuelos

We present tables for self-diffusion coefficients of the Lennard-Jones liquids and gases for various model formulas in the modified free volume theory of diffusion in the case of reduced temperatures $T^{\ast}=6.0$, 4.0, 1.3, 1.0, 0.8, 0.7…

Fluid Dynamics · Physics 2011-05-16 Jagtar Singh Hunjan , Byung Chan Eu

We consider the system of Maxwell-Stefan equations which describe multicomponent diffusive fluxes in non-dilute solutions or gas mixtures. We apply the Perron-Frobenius theorem to the irreducible and quasi-positive matrix which governs the…

Analysis of PDEs · Mathematics 2010-07-13 Dieter Bothe
‹ Prev 1 2 3 10 Next ›