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Using generalizations of natural orbitals, spin-averaged natural orbitals, and two-particle charge correlators for solids, we investigate electronic structure of antiferromagnetic transition-metal oxides with a fully self-consistent,…

Strongly Correlated Electrons · Physics 2024-02-07 Pavel Pokhilko , Dominika Zgid

The ab-initio many-body method suggested in the preceding paper is applied to the 3d transition metals Fe, Co, Ni, and Cu. We use a linearized muffin-tin orbital calculation to determine Bloch functions for the Hartree one-particle…

Condensed Matter · Physics 2007-05-23 I. Schnell , G. Czycholl , R. C. Albers

High entropy alloys (HEA) represent a class of materials with promising properties, such as high strength and ductility, radiation damage tolerance, etc. At the same time, a combinatorially large variety of compositions and a complex…

Materials Science · Physics 2025-10-03 Franco Moitzi , Lorenz Romaner , Andrei V. Ruban , Oleg E. Peil

Theoretical prediction of the 2nd-order magnetic transition temperature (TM) used to be arduous. Here, we develop a first principle-based, fully automatic structure-to-TM method for two-dimensional (2D) magnets whose effective Hamiltonians…

Materials Science · Physics 2023-12-08 Haichang Lu , Tai Yang , Zhimei Sun , John Robertson , Weisheng Zhao

Fe$_2$P alloys have been identified as promising candidates for magnetic refrigeration at room-temperature and for custom magnetostatic applications. The intent of this study is to accurately characterize the magnetic ground state of the…

We provide exact analytical expressions for the magnetic susceptibility function in the high temperature expansion for finite Heisenberg spin systems with an arbitrary coupling matrix, arbitrary single-spin quantum number, and arbitrary…

Statistical Mechanics · Physics 2009-11-07 H. -J. Schmidt , J. Schnack , Marshall Luban

We present an ab initio study of electronic correlation effects in a molecular cluster derived from the hexanuclear ferric wheel [LiFe6(OCH3)12-(dbm)6]PF6. The electronic and magnetic properties of this cluster have been studied with…

Materials Science · Physics 2007-05-23 H. Nieber , K. Doll , G. Zwicknagl

The concept of exchange in strongly-correlated fermions is reviewed with emphasis on the generalization of the Heisenberg pair exchange to higher order n-particle permutations. The "frustration" resulting from competing ferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-11 Michel Roger

We propose a new Monte Carlo method called the pinhole trace algorithm for {\it ab initio} calculations of the thermodynamics of nuclear systems. For typical simulations of interest, the computational speedup relative to conventional…

Based on a multi-scale calculations, combining ab-initio methods with spin dynamics simulations, we perform a detailed study of the magnetic behavior of Ni2MnAl/Fe bilayers. Our simulations show that such a bilayer exhibits a small exchange…

Mesoscale and Nanoscale Physics · Physics 2017-09-06 Rocio Yanes , Eszter Simon , Sebastian Keller , Balazs Nagyfalusi , Sergii Khmelevsky , Laszlo Szunyogh , Ulrich Nowak

We compute the binding energy of neutron-rich oxygen isotopes and employ the coupled-cluster method and chiral nucleon-nucleon interactions at next-to-next-to-next-to-leading order with two different cutoffs. We obtain rather well-converged…

Nuclear Theory · Physics 2009-09-11 G. Hagen , T. Papenbrock , D. J. Dean , M. Hjorth-Jensen , B. Velamur Asokan

Ab initio approaches to the nuclear many-body problem have seen their reach considerably extended over the past decade. However, collective excitations have been scarcely addressed so far due to the prohibitive cost of solving the…

Nuclear Theory · Physics 2023-02-22 Y. Beaujeault-Taudière , M. Frosini , J. -P. Ebran , T. Duguet , R. Roth , V. Somà

The engineered spin structures recently built and measured in scanning tunneling microscope experiments are calculated using density functional theory. By determining the precise local structure around the surface impurities, we find the Mn…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Chiung-Yuan Lin , B. A. Jones

Estimates of the exchange interaction parameter (J) between electronic magnetic momenta residing in the d-shells of several divalent first row transition metal ions, and those residing on the [TCNE]$^-$. anion-radicals (TCNE =…

Chemical Physics · Physics 2011-12-07 A. L. Tchougréeff

The present paper is comprised of two parts. First, we give a brief survey of the theoretical framework for microscopic nuclear structure calculations starting from a free nucleon-nucleon potential. Then, we present some selected results of…

Nuclear Theory · Physics 2007-05-23 A. Covello , L. Coraggio , A. Gargano , N. Itaco

Magnetoelasticity plays a crucial role in numerous magnetic phenomena, including magnetocalorics, magnon excitation via acoustic waves, and ultrafast demagnetization/Einstein-de Haas effect. Despite a long-standing discussion on…

In low-temperature anti-ferromagnetic LaMnO$_{3}$, strong and localized electronic interactions among Mn 3d electrons prevent a satisfactory description from standard local density and generalized gradient approximations in density…

Materials Science · Physics 2015-09-02 Thomas A. Mellan , Furio Cora , Ricardo Grau-Crespo , Sohrab Ismail-Beigi

We present an ab initio theory of the spin-wave stiffness tensor for ordered and disordered itinerant ferromagnets with pair exchange interactions derived from a method of infinitesimal spin rotations. The resulting formula bears an…

Materials Science · Physics 2020-04-15 Ilja Turek , Josef Kudrnovsky , Vaclav Drchal

The emergence of ferro- and ferrimagnetic behavior in insulating materials is uncommon, largely due to Hund's rules. Utilizing symmetry analysis, first-principles methods, and classical Monte Carlo simulations, \textcolor{black}{we report…

The interaction between electrons and lattice vibrations determines key physical properties of materials, including their electrical and heat transport, excited electron dynamics, phase transitions, and superconductivity. We present a new…

Materials Science · Physics 2018-07-04 Luis A. Agapito , Marco Bernardi
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