Related papers: Extraordinary nonlinear optics in ordinary semicon…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably…
We investigate the nonlinear optical process of third-harmonic generation in the thus far unexplored regime of focusing the pump light from a full solid angle, where the nonlinear process is dominantly driven by a standing dipole-wave. We…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
Optical control over elementary molecular vibration establishes fundamental capabilities for exploiting the broad range of optical linear and nonlinear phenomena. However, experimental demonstration of the coherently driven molecular…
We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…
The propagation of light-pulse with negative group-velocity in a nonlinear medium is studied theoretically. We show that the necessary conditions for these effects to be observable are realized in a three-level $\Lambda$-system interacting…
Enabling perfect light absorption in ultrathin materials promises the development of exotic photonic devices. Here we demonstrate new strategies that can provide capabilities to rationally design ultrathin (thickness <…
We report on the new non--linear optical signatures of quantum phase transitions in the high-temperature superconductor YBCO, observed through high harmonic generation. While the linear optical response of the material is largely unchanged…
Breaking the symmetry between forward and backward propagating optical modes is of fundamental scientific interest and enables crucial functionalities, such as isolators, circulators, and duplex communication systems. Whereas there has been…
We demonstrate time-resolved nonlinear extreme-ultraviolet absorption spectroscopy on multiply charged ions, here applied to the doubly charged neon ion, driven by a phase-locked sequence of two intense free-electron laser pulses.…
A possibility to greatly enhance frequency-conversion efficiency of stimulated Raman scattering is shown by making use of extraordinary properties of three-wave mixing of ordinary and backward waves. Such processes are commonly attributed…
Nonlinear optics underpins quantum photonics by enabling the generation and control of quantum states of light. We present new applications of optical resonators as mode selectors in nonlinear processes. First, we show that cavity-enhanced…
The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse…
Nonlinear optical phenomena play important roles in the vast emerging fields of micro- and nano-technology. This paper describes the general characteristics of nonlinear optical materials and systems, with a focus on parametric…
We present a plasmonic waveguide where light pulses are stopped at well-accessed complex-frequency zero-group-velocity points. Introducing gain at such points results in cavity-free, "thresholdless" nanolasers beating the diffraction limit…
Determined polarization state of light is required in nonlinear optics applications related to ultrashort and single-cycle light pulse generation. Such short time scales require up to full octave of spectral width of light. Fiber-based,…
We analyze the stability of a non-Hermitian coupler with respect to modulational inhomogeneous perturbations in the presence of unbalanced gain and loss. At the parity-time (PT) symmetry point the coupler is unstable. Suitable symmetry…
Nonreciprocal transport is generally observed in superconductors in which time reversal and inversion symmetries are simultaneously broken. This effect, which may become one of the backbones for future superconducting electronics, arises…
Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…