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An octupole ordering model is studied by the mean field theory, and its relevance to the phase IV of CexLa1-xB6 is discussed. The observed lattice distortion along the [111] direction is interpreted in terms of the \Gamma_{5g}-type…

Strongly Correlated Electrons · Physics 2009-08-11 Katsunori Kubo , Yoshio Kuramoto

Experimental evidence of the magnetic resonance in the antiferro-quadrupole phase of CeB6 is reported. We have shown that below orbital ordering temperature a new magnetic contribution from localized magnetic moments (LMM) emerge and gives…

Strongly Correlated Electrons · Physics 2015-06-25 S. V. Demishev , A. V. Semeno , A. V. Bogach , Yu. B. Paderno , N. Yu. Shitsevalova , N. E. Sluchanko

We report experimental observation of a new type of magnetic resonance caused by orbital ordering in a strongly correlated electronic system. Cavity measurements performed on CeB6 single crystals in a frequency range 60-100 GHz show that a…

Strongly Correlated Electrons · Physics 2009-11-11 S. V. Demishev , A. V. Semeno , A. V. Bogach , Yu. B. Paderno , N. Yu. Shitsevalova , N. E. Sluchanko

Possible order parameters of the phase IV in CexLa1-xB6 are discussed with special attention to the lattice distortion recently observed. A \Gamma_{5u}-type octupole order with finite wave number is proposed as the origin of the distortion…

Strongly Correlated Electrons · Physics 2009-08-11 Katsunori Kubo , Yoshio Kuramoto

The origin of non-collinear magnetism under quadrupolar ordering is investigated with CeB6 taken as a target system. The mode-mixing effect among 15 multipoles is analyzed based on the Ginzburg-Landau free energy. Then the lower magnetic…

Strongly Correlated Electrons · Physics 2009-11-07 Hiroaki Kusunose , Yoshio Kuramoto

In contrast to magnetic order formed by electrons' dipolar moments, ordering phenomena associated with higher-order multipoles (quadrupoles, octupoles, etc.) are more difficult to characterize because of the limited choice of experimental…

The azimuthal angle dependence observed in the resonant X-ray scattering in phase IV of Ce$_{0.7}$La$_{0.3}$B$_6$ is analyzed theoretically. It is shown that the peculiar angle dependence observed in the E2 channel is consistent with the…

Strongly Correlated Electrons · Physics 2009-11-11 Hiroaki Kusunose , Yoshio Kuramoto

Under zero magnetic field, a quadrupolar order parameter at q_Q=(1/2,1/2,1/2) in a typical antiferro-quadrupole (AFQ) ordering compound CeB6 has been observed for the first time by means of a resonant X-ray scattering (RXS) te\ chnique. The…

We study f-electron lattice models which are capable of supporting octupolar, as well dipolar and quadrupolar, order. Analyzing the properties of the Gamma8 ground state quartet, we find that (111)-type combinations of the Gamma5 octupoles…

Strongly Correlated Electrons · Physics 2009-11-10 Annamaria Kiss , P. Fazekas

Possible ways of identification are discussed of an electronic order of higher multipoles such as octupoles and hexadecapoles. A particularly powerful method is resonant X-ray scattering (RXS) using quadrupolar resonance processes called…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kuramoto , H. Kusunose , A. Kiss

We study the resonant x-ray scattering (RXS) spectra of CeB_{6} in an antiferroquadrupole (AFQ) ordering phase, near the Ce L_3 edge under the applied magnetic field H // (-1,1,0). On the basis of a localized electron model equipped with a…

Strongly Correlated Electrons · Physics 2010-07-13 Tatsuya Nagao , Jun-ichi Igarashi

In heavy fermion systems, multipole degrees of freedom make possible the emergence of rich phenomena, such as hidden orders and superconductivities. However, many of them remain unsolved since the origin of higher-rank multipole interaction…

Strongly Correlated Electrons · Physics 2019-12-11 Rina Tazai , Hiroshi Kontani

Cerium-hexaboride (CeB$_6$) f-electron compound displays a rich array of low-temperature magnetic phenomena, including `magnetically hidden' order, identified as multipolar in origin via advanced x-ray scattering. From first-principles…

Materials Science · Physics 2019-02-27 Chanchal Barman , Prashant Singh , Duane D. Johnson , Aftab Alam

We investigate a possibility of odd-parity multipole orderings in a locally noncentrosymmetric tetragonal compound CeCoSi. By performing symmetrical and microscopic mean-field analyses on a two-orbital tight-binding model, we propose…

Strongly Correlated Electrons · Physics 2019-12-19 Megumi Yatsushiro , Satoru Hayami

The heavy-fermion superconductor CeRh2As2 exhibits a non-superconducting phase transition that precedes the emergence of superconductivity. The nature of the corresponding order parameter remains under debate, with competing proposals…

Strongly Correlated Electrons · Physics 2026-04-06 Koki Numa , Eri Matsuda , Akimitsu Kirikoshi , Junya Otsuki

The recent experimental finding of large-amplitude antiferromagnetism induced by uniaxial strain shows that the "hidden" low-field order of URu2Si2 breaks time reversal invariance. We propose a new crystal field model which supports…

Strongly Correlated Electrons · Physics 2016-08-31 Annamaria Kiss , Patrik Fazekas

An antiferro ordering of an electric hexadecapole moment is discussed as a promising candidate for the long standing mystery of the hidden order phase in URu$_{2}$Si$_{2}$. Based on localized $f$-electron picture, we discuss the rationale…

Strongly Correlated Electrons · Physics 2015-05-27 Hiroaki Kusunose , Hisatomo Harima

A nonmagnetic phase transition at $T_0 \sim 12$ K in the tetragonal system CeCoSi with a Kramers doublet ground state is reminiscent of an electric quadrupole ordering, even though its well-separated crystal-electric-field (CEF) levels are…

Strongly Correlated Electrons · Physics 2023-08-21 Masahiro Manago , Ayano Ishigaki , Hideki Tou , Hisatomo Harima , Hiroshi Tanida , Hisashi Kotegawa

Possibility of a novel pseudo-scalar (octupole) order is studied theoretically for orbitally degenerate systems with strong spin-orbit coupling such as Ce$_x$La$_{1-x}$B$_6$. It is discussed that coexistence of an octupole order parameter…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshio Kuramoto , Hiroaki Kusunose

We show that time-reversal symmetry broken, centrosymmetric antiferromagnets with nonrelativistic spin-splitting are conveniently described in terms of the ferroic ordering of magnetic octupoles. The magnetic octupoles are the lowest-order…

Strongly Correlated Electrons · Physics 2025-06-10 Sayantika Bhowal , Nicola A. Spaldin
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