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We study the effect of confinement on the phonon properties of ultra-narrow silicon nanowires of side sizes of 1-10nm . We use the modified valence force field method to compute the phononic dispersion, and extract the density of states,…

Mesoscale and Nanoscale Physics · Physics 2013-04-05 Hossein Karamitaheri , Neophytos Neophytou , Mohsen Karami Taheri , Rahim Faez , Hans Kosina

In order to clarify the relationship between the phonon spectra of nanoparticles and their melting temperature, we studied in detail the size-dependent low energy vibration modes. A minimum model with atoms on a lattice and harmonic…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Kai Kang , Shaojing Qin , Chuilin Wang

We study the size dependence of thermal conductivity in nanoscale semiconducting systems. An analytical formula including the surface scattering and the size confinement effects of phonon transport is derived. The theoretical formula gives…

Materials Science · Physics 2009-11-11 L. -H Liang , Baowen Li

We calculate low-frequency Raman scattering from the confined acoustic phonon modes of CdS1-xSex nanoparticles embedded in borosilicate glass. The calculation of the Raman scattering by acoustic phonons in nanoparticles has been performed…

Mesoscale and Nanoscale Physics · Physics 2009-04-16 Sanjeev K. Gupta , Prafulla K. Jha , Satyaprakash Sahoo , A. K. Arora , Y. M. Azhniuk

Raman microspectroscopy was used to characterize amorphous silica plastic behavior. Using a correlation between Raman spectrum and density, a map of the local residual indentation-induced densification is obtained. The existence of a…

The potential of silicon nanowires (SiNWs), (diameter < 10 nm) to transform into rigid bundle-like structures with distinct phonon confinement under high pressure (<= 15 GPa), instead of amorphising as per previous reports, is demonstrated…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Somnath Bhattacharyya , Dmitry Churochkin , Rudolph M Erasmus

Titanium dioxide (TiO2) nanocrystals were prepared by wet chemical method and characterized by x-ray diffraction (XRD), transmission electron microscopy (TEM), Raman scattering (RS) and photoluminescence (PL). The X-ray diffraction shows…

Mesoscale and Nanoscale Physics · Physics 2009-04-16 S. K. Gupta , Rucha Desai , P. K. Jha , S. P. Sahoo , D. Kirin

The structural, electronic and optical properties of Si nanocrystals of different size and shape, passivated with hydrogens, OH groups, or embedded in a SiO2 matrix are studied. The comparison between the embedded and free, suspended…

Materials Science · Physics 2010-09-01 Roberto Guerra , Elena Degoli , Stefano Ossicini

Micro-Raman scattering and electron field emission characteristics of silicon nanowires (SiNWs) synthesized by metal assisted chemical etching (MACE) are investigated. Scanning electron microscopy images reveal the growth of well aligned…

Mesoscale and Nanoscale Physics · Physics 2014-11-14 Vivek Kumar , Shailendra K. Saxena , Vishakha Kaushik , Kapil Saxena , Rajesh Kumar , A. K. Shukla

In crystalline nanoparticles the Raman peak is downshifted with respect to the bulk material and has asymmetric broadening. These effects are straightly related to the finite size of nanoparticles, giving the perspective to use the Raman…

Mesoscale and Nanoscale Physics · Physics 2018-09-05 S. V. Koniakhin , O. I. Utesov , I. N. Terterov , A. V. Siklitskaya , D. Solnyshkov , A. G. Yashenkin

We have performed first-principles calculations to study the lattice vibrational modes and their Raman activities in silicon nanowires (SiNWs). Two types of characteristic vibrational modes are examined: high-frequency optical modes and…

Mesoscale and Nanoscale Physics · Physics 2011-08-30 Li Yang , M. Y. Chou

Confined microexplosions induced in silicon by powerful ultrashort laser pulses can lead to new Si phases. Some of these have not previously been observed via near-equilibrium compression of silicon. In this study, confocal Raman…

Materials Science · Physics 2020-10-07 L. A. Smillie , M. Niihori , L. Rapp , B. Haberl , J. S. Williams , J. E. Bradby , C. J. Pickard , A. V. Rode

A new analytical expression for the size-dependent bandgap of colloidal semiconductor nanocrystals is proposed within the framework of the finite-depth square-well effective mass approximation in order to provide a quantitative description…

We present a theoretical model to describe the double-resonant scattering process in arbitrary carbon nanotubes. We use this approach to investigate the defect-induced $D$ mode in CNTs and unravel the dependence of the $D$-mode frequency on…

Materials Science · Physics 2016-01-20 Felix Herziger , Asmus Vierck , Jan Laudenbach , Janina Maultzsch

Optical properties of the lead halide perovskites nanocrystals are controlled by confined excitons and rich spectrum of confined acoustic and optical phonons. We study experimentally and theoretically the exciton-phonon interaction in…

New approach on interpretation and processing of Raman spectra of complex perovskites is suggested. Raman spectra of $PbMg_{1/3}Nb_{2/3}O_{3}$ and $% PbSc_{1/2}Ta_{1/2}O_{3}$ are successfully described on the basis of the phonon-confinement…

Materials Science · Physics 2007-05-23 E. A. Rogacheva

The temperature dependence of the first-order phonon mode of single crystal of Silicon (Si) is determined by Raman scattering in a broad temperature range of 4-623 K. Our studies reveal the anomalous red-shift of the Raman active phonon…

Materials Science · Physics 2020-01-24 Himanshi , Birender Singh , Pradeep Kumar

In the present paper, we utilize the coupled-oscillator model describing the hybridization of optical phonons in touching and/or overlapping particles in order to study the Raman spectra of nanoparticles organized into various types of…

Mesoscale and Nanoscale Physics · Physics 2023-12-01 S. V. Koniakhin , O. I. Utesov , A. G. Yashenkin

Si-SiO2 multilayer nanocomposite (NCp) films, grown using pulsed laser deposition with varying Si deposition time are investigated using Raman spectroscopy/mapping for studying the variation of Si phonon frequency observed in these NCps.…

Mesoscale and Nanoscale Physics · Physics 2015-03-12 Ekta Rani , Alka A. Ingale , A. Chaturvedi , C. Kamal , D. M. Phase , M. P. Joshi , Aparna Chakrabarti , Arup Banerjee , L. M. Kukreja

We used Raman scattering for study the phonon modes of self-organized Ge/Si quantum dots, grown by a molecular-beam epitaxy method. It is revealed, that Ge-Ge and Si-Ge vibrational modes considerably intensify at excitation of exciton…

Mesoscale and Nanoscale Physics · Physics 2011-05-17 I. V. Kucherenko , V. S. Vinogradov , N. N. Melnik , L. V. Arapkina , V. A. Chapnin , K. V. Chizh , V. A. Yuryev