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Magnetoelectric properties were investigated for an S=1/2 chain antiferromagnet CuCl2, which turns out to be the first example of non-chalcogen based spiral-spin induced multiferroics. Upon the onset of helimagnetic order propagating along…

Strongly Correlated Electrons · Physics 2010-09-01 S. Seki , T. Kurumaji , S. Ishiwata , H. Matsui , H. Murakawa , Y. Tokunaga , Y. Kaneko , T. Hasegawa , Y. Tokura

The spin dynamics of the geometrically frustrated triangular antiferromagnet multiferroic CuCrO2 have been mapped out using inelastic neutron scattering. The relevant spin Hamiltonian parameters modelling the incommensurate modulated…

Strongly Correlated Electrons · Physics 2015-05-14 M. Poienar , F. Damay , C. Martin , J. Robert , S. Petit

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

We present the results of the first neutron powder and single crystal diffraction studies of the coupled spin tetrahedra systems ${\CuTeX}$ (X=Cl, Br). Incommensurate antiferromagnetic order with the propagation vectors…

Strongly Correlated Electrons · Physics 2009-11-10 O. Zaharko , A. Daoud-Aladine , S. Streule , J. Mesot , P. -J. Brown , H. Berger

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

Strongly Correlated Electrons · Physics 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel

The ordered tetragonal intermetallic Cr$_2$Al forms the same structure type as Mn$_2$Au, and the latter has been heavily investigated for its potential in antiferromagnetic spintronics due to its degenerate in-plane N\'{e}el vector. We…

Materials Science · Physics 2022-01-20 Chengxi Zhao , Kisung Kang , Joerg C. Neuefeind , Andre Schleife , Daniel P. Shoemaker

High pressure neutron diffraction is employed to investigate the magnetic behavior of CaMn$_2$Bi$_2$ in extreme conditions. In contrast to antiferromagnetic ordering on Mn atoms reported at ambient pressure, our results reveal that at high…

Materials Science · Physics 2023-12-04 Madalynn Marshall , Haozhe Wang , Antonio M. dos Santos , Bianca Haberl , Weiwei Xie

{\alpha}-CaCr2O4 is a distorted triangular antiferromagnet. The magnetic Cr3+ ions which have spin-3/2 and interact with their nearest neighbors via Heisenberg direct exchange interactions, develop long-range magnetic order below T_N=42.6…

Strongly Correlated Electrons · Physics 2011-11-22 S. Tóth , B. Lake , S. A. J. Kimber , O. Pieper , M. Reehuis , A. T. M. N. Islam , O. Zaharko , C. Ritter , A. H. Hill , H. Ryll , D. N. Argyriou , A. J. Williams

Motivated by the discovery of multiferroicity in the geometrically frustrated triangular antiferromagnet CuCrO$_2$ below its N\'eel temperature $T_N$, we investigate its magnetic and ferroelectric properties using ab initio calculations and…

Materials Science · Physics 2017-10-23 Ahmed Albaalbaky , Yaroslav Kvashnin , Denis Ledue , Renaud Patte , Raymond Frésard

Neutron powder diffraction experiment has been performed on the quasicrystal approximant Au$_{72}$Al$_{14}$Tb$_{14}$, a body-center-cubic crystal of icosahedral spin clusters. The long-range antiferromagnetic order was confirmed at the…

Materials Science · Physics 2019-08-21 Taku J Sato , Asuka Ishikawa , Akira Sakurai , Masashi Hattori , Maxim Avdeev , Ryuji Tamura

Polarized and unpolarized neutron diffraction studies have been carried out on single crystals of the coupled spin tetrahedra systems Cu2Te2O5X2 (X=Cl, Br). A model of the magnetic structure associated with the propagation vectors k'Cl ~…

We have carried out $^{63,65}$Cu NMR spectra measurements in magnetic field up to about 45~T on single crystal of a multiferroic triangular antiferromagnet CuCrO$_2$. The measurements were performed for magnetic fields aligned along the…

Strongly Correlated Electrons · Physics 2016-12-21 Yu. A. Sakhratov , L. E. Svistov , P. L. Kuhns , H. D. Zhou , A. P. Reyes

This paper presents results of a recent study of multiferroic \CCO\ by means of single crystal neutron diffraction. This system has two close magnetic phase transitions at $T\nsub{N1}=24.2$ K and $T\nsub{N2}=23.6$ K. The low temperature…

Materials Science · Physics 2015-05-30 M. Frontzek , G. Ehlers , A. Podlesnyak , H. Cao , M. Matsuda , O. Zaharko , N. Aliouane , S. Barilo , S. V. Shiryaev

A detailed study of poly- and single crystalline samples of the normal spinel HgCr2S4 is reported. The structural refinement reveals enhanced values of the atomic displacements suggesting closeness to a structural instability.…

Materials Science · Physics 2009-11-11 V. Tsurkan , J. Hemberger , A. Krimmel , H. -A. Krug von Nidda , P. Lunkenheimer , S. Weber , V. Zestrea , A. Loidl

A complex magnetic order of the multiferroic compound Co3TeO6 has been revealed by neutron powder diffraction studies on ceramics and crushed single crystals. The compound adopts a monoclinic structure (s.g. C2/c) in the studied temperature…

Materials Science · Physics 2011-11-28 S. A. Ivanov , R. Tellgren , C. Ritter , P. Nordblad , R. Mathieu , G. Andre , N. V. Golubko , E. D. Politova , M. Weil

We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

Periodic and cluster density-functional theory (DFT) calculations, including DFT+U and hybrid functionals, are applied to study magnetostructural correlations in spin-1/2 frustrated chain compounds CuX2: CuCl2, CuBr2, and a fictitious chain…

Strongly Correlated Electrons · Physics 2013-07-02 S. Lebernegg , M. Schmitt , A. A. Tsirlin , O. Janson , H. Rosner

Antiferromagnetic order at $T_{\mathrm{N}} = 23$ K has been identified in Mn(III)F(salen), salen = H$_{14}$C$_{16}$N$_2$O$_2$, an $S = 2$ linear-chain system. Using single crystals, specific heat studies performed in magnetic fields up to 9…

Using powder neutron diffraction we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature an antiferromagnetic phase with propagation vector k=(0.5,-0.5,1) emerges…

Strongly Correlated Electrons · Physics 2011-05-17 S. Agrestini , C. L. Fleck , L. C. Chapon , C. Mazzoli , A. Bombardi , M. R. Lees , O. A. Petrenko

The crystal and magnetic structures of the spinel compounds ZnCr$_2$S$_4$ and ZnCr$_2$Se$_4$ were investigated by high resolution powder synchrotron and neutron diffraction. ZnCr$_2$Se$_4$ exhibits a first order phase transition at $T_N=21$…

Strongly Correlated Electrons · Physics 2009-11-13 F. Yokaichiya , A. Krimmel , V. Tsurkan , I. Margiolaki , P. Thompson , H. N. Bordallo , A. Buchsteiner , N. Stüßer , D. N. Argyriou , A. Loidl
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