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In equilibrium and supercooled liquids, polymorphism is manifested by thermodynamic regions defined in the phase diagram, which are predominantly of different short- and medium-range order (local structure). It is found that on the phase…

Soft Condensed Matter · Physics 2024-03-19 Anatolii V. Mokshin , Roman V. Vlasov

We report an experimental investigation of the caging motion in a uniformly heated granular fluid, for a wide range of filling fractions, $\phi$. At low $\phi$ the classic diffusive behavior of a fluid is observed. However, as $\phi$ is…

Soft Condensed Matter · Physics 2009-11-11 Pedro M. Reis , Rohit A. Ingale , Mark D. Shattuck

We investigate bridging and aggregation of two colloidal particles in a near-critical binary mixture when the fluid far from the particles is outside the coexistence (CX) curve and is rich in the component disfavored by the colloid…

Soft Condensed Matter · Physics 2015-05-26 Shunsuke Yabunaka , Ryuichi Okamoto , Akira Onuki

We study the behaviour of catalytically active droplets in multi-component conserved mixtures affected by noise. Working in the thin interface limit, we analytically determine the state diagram of the system, characterized by multiple…

Soft Condensed Matter · Physics 2025-12-01 Jacopo Romano , Martin Kjøllesdal Johnsrud , Benoît Mahault , Ramin Golestanian

Glasses and gels are the two dynamically arrested, disordered states of matter. Despite their importance, their similarities and differences remain elusive, especially at high density. We identify dynamical and structural signatures which…

Soft Condensed Matter · Physics 2014-09-22 C. Patrick Royall , Stephen R. Williams , Hajime Tanaka

We study numerically the crystallization of a hard-sphere mixture with 8\% polydispersity. Although often used as a model glass former, for small system sizes we observe crystallization in molecular dynamics simulations. This opens the…

Soft Condensed Matter · Physics 2016-09-05 Matteo Campo , Thomas Speck

We measure hydrodynamic interactions between colloidal particles confined in a thin sheet of fluid. The reduced dimensionality, compared to a bulk fluid, increases dramatically the range of couplings. Using optical tweezers we force a two…

Soft Condensed Matter · Physics 2009-11-13 R. Di Leonardo , S. Keen , F. Ianni , J. Leach , M. Padgett , G. Ruocco

We use molecular dynamics simulations of a simple model to show that dispersions of slightly elongated colloidal particles with long-range dipolar interactions, like ferrofluids, can form a physical (reversible) gel at low volume fractions.…

Soft Condensed Matter · Physics 2007-05-23 Ronald Blaak , Mark A. Miller , Jean-Pierre Hansen

The liquid-liquid phase separation of a binary solvent can be arrested by colloidal particles trapped at the interface [K. Stratford et al., Science 309, 5744 (2005)]. We show experimentally that the colloidal network so formed can remain…

Soft Condensed Matter · Physics 2015-05-14 Eduardo Sanz , Kathryn A. White , Paul S. Clegg , Michael E. Cates

Attractive colloids diffuse and aggregate to form gels, solid-like particle networks suspended in a fluid. Gravity is known to strongly impact the stability of gels once they are formed. However, its effect on the process of gel formation…

Soft Condensed Matter · Physics 2023-04-12 Joost de Graaf , Kim William Torre , Wilson C. K. Poon , Michiel Hermes

Three structural populations with distinct average mobility are identified within an equilibrium two-dimensional Lennard-Jones fluid simulated via molecular dynamics at a constant temperature and varying density. Quantifying the structure…

Soft Condensed Matter · Physics 2018-02-05 Tamoghna Das , Jack F. Douglas

Colloidal gels have strong industrial relevance as they can behave liquid- and solid-like. The latter allows them to support the buoyant weight against gravity. However, the system is intrinsically out-of-equilibrium, which means that the…

Soft Condensed Matter · Physics 2024-05-28 Kim William Torre , Joost de Graaf

Using extensive molecular dynamics simulations of an equilibrium, glass-forming Lennard-Jones mixture, we characterize in detail the local atomic motions. We show that spatial correlations exist among particles undergoing extremely large…

Soft Condensed Matter · Physics 2009-10-31 C. Donati , S. C. Glotzer , P. H. Poole , W. Kob , S. J. Plimpton

The collective dynamics of externally driven $N_{\rm p}$-colloidal systems ($1\le N_{\rm p}\le 4$) in a confined viscous fluid have been investigated using three-dimensional direct numerical simulations with fully resolved hydrodynamics.…

Soft Condensed Matter · Physics 2018-04-04 Norihiro Oyama , Kosuke Teshigawara , John Jairo Molina , Ryoichi Yamamoto , Takashi Taniguchi

Colloids dispersed in nematic liquid crystals form topological composites in which colloid-associated defects mediate interactions while adhering to fundamental topological constraints. Better realising the promise of such materials…

Soft Condensed Matter · Physics 2024-04-16 Louise C. Head , Yair A. G. Fosado , Davide Marenduzzo , Tyler N. Shendruk

We propose a method to determine the locally preferred structure of model liquids. This latter is obtained numerically as the global minimum of the effective energy surface of clusters formed by small numbers of particles embedded in a…

Soft Condensed Matter · Physics 2009-11-10 S. Mossa , G. Tarjus

We study the hydrodynamic behavior of three dimensional (3D) incompressible collections of self-propelled entities in contact with a momentum sink in a state with non-zero average velocity, hereafter called 3D easy-plane incompressible…

Soft Condensed Matter · Physics 2018-10-31 Leiming Chen , Chiu Fan Lee , John Toner

Understanding the physics of supercooled liquids near glassy transition remains one of the major challenges in condensed matter science. There has been long recognized that supercooled liquids have spatially dynamical heterogeneity whose…

Statistical Mechanics · Physics 2023-07-10 Viet Nguyen , Xueyu Song

Collisionless suspensions of inertial particles (finite-size impurities) are studied in 2D and 3D spatially smooth flows. Tools borrowed from the study of random dynamical systems are used to identify and to characterise in full generality…

Chaotic Dynamics · Physics 2007-05-23 Jeremie Bec

We develop and present a unified multi-scale model (involving three scales of spatial organisation) to study the dynamics of rigid aggregating particles suspended in a viscous fluid medium and subject to a steady poiseuille flow. At…

Soft Condensed Matter · Physics 2016-10-10 Sarthok Sircar , Anthony J. Roberts
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