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Silica nanoparticles trapped at air-water interface form a 2D solid state with amorphous order. We propose a theoretical model to describe how this solid-like state deforms under a shear strain ramp up to and beyond a yielding point which…

Soft Condensed Matter · Physics 2017-10-30 Armando Maestro , Alessio Zaccone

Cells offer numerous inspiring examples where proteins and membranes combine to form complex structures that are key to intracellular compartmentalization, cargo transport, and specialization of cell morphology. Despite this wealth of…

The interaction of mass-selected atomic clusters and nanoparticles with surfaces attracts strong interest in view of fundamental research and technological applications. Understanding dynamics of the deposition process is important for…

Atomic and Molecular Clusters · Physics 2021-07-12 Yannick Fortouna , Pablo de Vera , Alexey Verkhovtsev , Andrey V. Solov'yov

The effect of silica nanoparticles on transient microemulsion networks made of microemulsion droplets and telechelic copolymer molecules in water is studied, as a function of droplet size and concentration, amount of copolymer, and…

Soft Condensed Matter · Physics 2010-12-07 Nicolas Puech , Serge Mora , Ty Phou , Gregoire Porte , Jacques Jestin , Julian Oberdisse

The motion of three-phase contact lines is one of the most relevant research topics of micro- and nano-fluidics. According to many hydrodynamic and molecular models, the dynamics of contact lines is assumed overdamped and dominated by…

Fluid Dynamics · Physics 2022-09-29 Michele Pellegrino , Berk Hess

We used single-molecule tracking to probe the local rheology of interfacial water. Fluorescent rhodamine molecules were tracked on silica surfaces as a function of ambient relative humidity, which controlled the thickness of condensed water…

Soft Condensed Matter · Physics 2020-01-20 Raphael Sarfati , Daniel K. Schwartz

Large scale molecular dynamics simulations are used to study the dispersion of nanoparticles (NPs) in a polymer film during solvent evaporation. As the solvent evaporates, a dense polymer-rich skin layer forms at the liquid/vapor interface,…

Soft Condensed Matter · Physics 2016-05-23 Shengfeng Cheng , Gary S. Grest

We present a detailed analysis of the effective force between two smooth spherical colloids floating at a fluid interface due to deformations of the interface. The results hold in general and are applicable independently of the source of…

Soft Condensed Matter · Physics 2007-05-23 M. Oettel , A. Dominguez , S. Dietrich

Using classical density functional theory (DFT) we calculate the density profile $\rho({\mathbf r})$ and local compressibility $\chi({\mathbf r})$ of a simple liquid solvent in which a pair of blocks with (microscopic) rectangular…

Soft Condensed Matter · Physics 2017-04-05 Blesson Chacko , Robert Evans , Andrew J. Archer

The dispersive spreading of microscopic particles in shear flows is influenced both by advection and thermal motion. At the nanoscale, interactions between such particles and their confining boundaries become unavoidable. We address the…

Soft Condensed Matter · Physics 2023-02-01 Alexandre Vilquin , Vincent Bertin , Elie Raphaël , David S Dean , Thomas Salez , Joshua D. McGraw

We perform a systematic application of the hybrid particle-field molecular dynamics technique [Milano et al, J. Chem. Phys. 2009, 130, 214106] to study interfacial properties and potential of mean force (PMF) for separating nanoparticles…

Non-equilibrium molecular dynamics (NEMD) simulations of fluid flow have highlighted the peculiarities of nanoscale flows compared to classical fluid mechanics; in particular, boundary conditions can deviate from the no-slip behavior at…

Soft Condensed Matter · Physics 2025-03-11 Giorgia Marcelli , Tecla Bottinelli Montandon , Roya Ebrahimi Viand , Felix Höfling

We present a detailed description of biopolymer translocation through a nanopore in the presence of a solvent, using an innovative multi-scale methodology which treats the biopolymer at the microscopic scale as combined with a…

Computational Physics · Physics 2008-02-27 Massimo Bernaschi , Simone Melchionna , Sauro Succi , Maria Fyta , Efthimios Kaxiras

The dynamics of particles attached to an interface separating two immiscible fluids are encountered in a wide variety of applications. Here we present a combined asymptotic and numerical investigation of the fluid motion past spherical…

Fluid Dynamics · Physics 2022-07-11 Zhi Zhou , Petia M. Vlahovska , Michael J. Miksis

Pulmonary surfactant forms a sub-micrometer thick fluid layer that covers the surface of alveolar lumen and inhaled nanoparticles therefore come in to contact with surfactant prior to any interaction with epithelial cells. We investigate…

Soft Condensed Matter · Physics 2021-09-21 M. Radiom , M. Sarkis , O. Brookes , E. K. Oikonomou , A. Baeza-Squiban , J. -F. Berret

Hypothesis: We test whether the wettability of nanoparticles (NPs) straddling at an air/water surface or oil/water interface can be extrapolated from sessile drop-derived macroscopic contact angles (mCAs) on planar substrates, assuming that…

The van der Waals forces across a very thin liquid layer (nanofilm) in contact with a plane solid wall make the liquid nonhomogeneous. The dynamics of such flat liquid nanofilms is studied in isothermal case. The Navier-Stokes equations are…

Classical Physics · Physics 2008-09-23 Henri Gouin , Sergey Gavrilyuk

The movement of small particles and molecules through membranes is widespread and has far-reaching implications. Consequently, the development of mathematical models is essential for understanding these processes on a micro level, leading…

We investigate the solvent mediated interactions between nanoparticles adsorbed at a liquid-vapor interface in comparison to the solvent mediated interactions in the bulk liquid and vapor phases of a Lennard-Jones solvent. Molecular…

Soft Condensed Matter · Physics 2010-09-06 F. Bresme , H. Lehle , M. Oettel

This work provides a recipe for creating drag, lift and torque closures for static assemblies of axisymmetric, non-spherical particles. Apart from Reynolds number $Re$ and solids volume fraction $\epsilon_s$, we propose four additional…

Fluid Dynamics · Physics 2020-11-10 Sathish K. P. Sanjeevi , Johan T. Padding