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The magnetic structure of multiferroic Ni$_3$V$_2$O$_8$ has been investigated using non-resonant X-ray magnetic scattering. Incident circularly polarized X-rays combined with full polarization analysis of the scattered beam is shown to…

Strongly Correlated Electrons · Physics 2015-05-18 F. Fabrizi , H. C. Walker , L. Paolasini , F. de Bergevin , T. Fennell , N. Rogado , R. J. Cava , Th. Wolf , M. Kenzelmann , D. F. McMorrow

We have studied the high temperature multiferroic cupric oxide using polarized neutron diffraction as a function of temperature and applied electric field. We find that the chiral domain population can be varied using an external electric…

Strongly Correlated Electrons · Physics 2012-08-08 P. Babkevich , A. Poole , R. D. Johnson , B. Roessli , D. Prabhakaran , A. T. Boothroyd

The magnetic field induced rearrangement of the cycloidal spin structure in ferroelectric mono-domain single crystals of the room-temperature multiferroic BiFeO$_3$ is studied using small-angle neutron scattering (SANS). The cycloid…

Strongly Correlated Electrons · Physics 2018-04-11 S. Bordács , D. G. Farkas , J. S. White , R. Cubitt , L. DeBeer-Schmitt , T. Ito , I. Kézsmárki

Magnetic ferroelectrics or multiferroics, which are currently extensively explored, may provide a good arena to realize a novel magnetoelectric function. Here we demonstrate the genuine electric control of the spiral magnetic structure in…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Yamasaki , H. Sagayama , T. Goto , M. Matsuura , K. Hirota , T. Arima , Y. Tokura

The control of multiferroic domains through external electric fields has been studied by dielectric measurements and by polarized neutron diffraction on single-crystalline TbMnO$_3$. Full hysteresis cycles were recorded by varying an…

Strongly Correlated Electrons · Physics 2016-02-10 Jonas Stein , Max Baum , Simon Holbein , Vladimir Hutanu , Alexander C. Komarek , Markus Braden

We present the microscopic theory of improper multiferroicity in BiMnO3, which can be summarized as follows: (1) the ferroelectric polarization is driven by the hidden antiferromagnetic order in the otherwise centrosymmetric C2/c structure;…

Materials Science · Physics 2010-11-01 I. V. Solovyev , Z. V. Pchelkina

By combining bulk properties, neutron diffraction and non-resonant X-ray diffraction measurements, we demonstrate that the new multiferroic Cu$_3$Nb$_2$O$_8$ becomes polar simultaneously with the appearance of generalised helicoidal…

Strongly Correlated Electrons · Physics 2015-05-28 R. D. Johnson , Sunil Nair , L. C. Chapon , A. Bombardi , C. Vecchini , D. Prabhakaran , A. T. Boothroyd , P. G. Radaelli

The spin-driven component of electric polarization in a single crystal of multiferroic BiFeO$_{3}$ was experimentally investigated in pulsed high magnetic fields up to 41 T. Sequential measurements of electric polarization for various…

Strongly Correlated Electrons · Physics 2020-01-08 Shiro Kawachi , Shin Miyahara , Toshimitsu Ito , Atsushi Miyake , Nobuo Furukawa , Jun-ichi Yamaura , Masashi Tokunaga

Neutron spherical polarimetry, which is directly sensitive to the absolute magnetic configuration and domain population, has been used in this work to unambiguously prove the multiferroicity of (ND4)2[FeCl5(D2O)]. We demonstrate that the…

Transition metal molybdenum oxides A2Mo3O8 (A= Mn, Fe, Co) are known to be polar magnets where A ions are located in either octahedrally or tetrahedrally coordinated sites. In this paper we predict that their polarizations can be reversed…

Materials Science · Physics 2025-03-18 Yaxin Gao , Sha Li , Menghao Wu

Layered van der Waals two-dimensional (2D) magnets are a cornerstone of ultrathin spintronic and magnonic devices. The recent discovery of a 2D multiferroic with strong magnetoelectric coupling in NiI$_2$ offers a promising platform for the…

Materials Science · Physics 2024-08-01 Andrey Rybakov , Adolfo O. Fumega , Dorye L. Esteras , Jose L. Lado , José J. Baldoví

The electric field effect on magnetism was examined in the multiferroic conical magnet Mn$_2$GeO$_4$, which shows a strong coupling between ferromagnetic and ferroelectric order parameters. The systematic evaluation of the electric…

Strongly Correlated Electrons · Physics 2020-08-12 Jonas K. H. Fischer , Hiroki Ueda , Tsuyoshi Kimura

We have demonstrated that ferroelectric polarization in a spin-driven multiferroic CuFe1-xGaxO2 with x = 0.035 can be controlled by the application of uniaxial pressure. Our neutron diffraction and in-situ ferroelectric polarization…

Strongly Correlated Electrons · Physics 2015-05-28 T. Nakajima , S. Mitsuda , T. Nakamura , H. Ishii , T. Haku , Y. Honma , M. Kosaka , N. Aso , Y. Uwatoko

We report a comprehensive inelastic neutron scattering study of the hybrid molecule-based multiferroic compound (ND4)2FeCl5D2O in the zero-field incommensurate cycloidal phase and the high-field quasi-collinear phase. The spontaneous…

We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be…

Strongly Correlated Electrons · Physics 2015-05-19 H. Murakawa , Y. Onose , S. Miyahara , N. Furukawa , Y. Tokura

We employ neutron spherical polarimetry to determine the nature and population of the coexisting antiferromagnetic domains in multiferroic YMn2O5. By applying an electric field, we prove that reversing the electrical polarization results in…

Materials Science · Physics 2009-11-13 P. G. Radaelli , L. C. Chapon , A. Daoud-Aladine , C. Vecchini , P. J. Brown , T. Chatterji , S. Park , S-W. Cheong

BiFeO3 is a model multiferroic in which the ferroelectric polarization is coupled to ferroelastic lattice distortions, yet deterministic control of its domain structure remains limited by high switching fields and competing polarization…

Despite remarkable progress in developing multifunctional materials, spin-driven ferroelectrics featuring both spontaneous magnetization and electric polarization are still rare. Among such ferromagnetic ferroelectrics are conical spin…

Strongly Correlated Electrons · Physics 2017-06-09 T. Honda , J. S. White , A. B. Harris , L. C. Chapon , A. Fennell , B. Roessli , O. Zaharko , Y. Murakami , M. Kenzelmann , T. Kimura

Cu3Nb2O8 is an unusual multiferroic compound that undergoes a series of magnetic ordering at low temperatures. Concurrent development of electric polarization has been reported at TN1 ~25 K corresponding to a non-collinear helicoidal…

Strongly Correlated Electrons · Physics 2015-06-22 G. Sharma , J. Saha , S. D. Kaushik , V. Siruguri , S. Patnaik

The coupling of magnetic chiralities to the ferroelectric polarisation in multiferroic RbFe(MoO$_4$)$_2$ is investigated by neutron spherical polarimetry. Because of the axiality of the crystal structure below $T_\textrm{c}$ = 190 K,…

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