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Observational constraints on the primordial deuterium-to-hydrogen ratio (D/H) can test theories of the early universe and provide constraints on models of big bang nucleosynthesis (BBN). We measure deuterium absorption in high-redshift,…

Astrophysics · Physics 2007-05-23 Scott Burles , David Tytler

In this paper we demonstrate atomic-scale lithography on hydrogen terminated Ge(001. The lithographic patterns were obtained by selectively desorbing hydrogen atoms from a H resist layer adsorbed on a clean, atomically flat Ge(001) surface…

Mesoscale and Nanoscale Physics · Physics 2009-12-07 G. Scappucci , G. Capellini , W. C. T. Lee , M. Y. Simmons

The main challenge to exploiting plasmons for gas vibrational mode sensing is the extremely weak infrared absorption of gas species. In this work, we explore the possibility of trapping free gas molecules via surface adsorption, optical, or…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Kaveh Khaliji , Sudipta Romen Biswas , Hai Hu , Xiaoxia Yang , Qing Dai , Sang-Hyun Oh , Phaedon Avouris , Tony Low

Porous nanocarbon materials are seen as potential excellent materials for hydrogen storage due to their high surface area, excellent cycling stability and favorable kinetics. This study employs Density Functional Theory (DFT) simulations to…

Materials Science · Physics 2026-01-21 Hongyan Ma , Qing Wang , Huilin Sun , Qingyu Li , Yunhui Wang , Zhihong Yang , Huaihong Zhao , Huazhong Shu

NaBH4 is a very cheap and hydrogen rich material and a potential hydrogen store. However, high temperature of its thermal decomposition (above 530{\deg}C) renders it inapplicable in practical use. Here, we have studied the effect of…

Materials Science · Physics 2022-05-24 Piotr Orłowski1 , Wojciech Grochala

We report on the transverse laser cooling of a magnetically guided beam of ultra cold chromium atoms. Radial compression by a tapering of the guide is employed to adiabatically heat the beam. Inside the tapered section heat is extracted…

We propose a multi-layer graphene-based device in which storage and release of atomic hydrogen is obtained by exploiting and controlling the corrugation of the layers. The proposal is based on density-functional simulations of hydrogen…

Mesoscale and Nanoscale Physics · Physics 2011-01-07 Valentina Tozzini , Vittorio Pellegrini

We deposit intrinsic hydrogenated amorphous silicon (a-Si:H) thin films by reactive pulsed laser deposition, for various hydrogen pressures in the 0-20 Pa range, at a low deposition temperature of 120C, and investigate the hydrogen…

Materials Science · Physics 2017-04-17 A. Mellos , M. Kandyla , D. Palles , M. Kompitsas

Adsorption of hydrogen atoms to a carbon atom vacancy in graphene is investigated by means of periodic \emph{first principles} calculations, up to the fully hydrogenated state where six H atoms chemically bind to the vacancy. Addition of a…

Materials Science · Physics 2013-12-30 M. Casartelli , S. Casolo , G. F. Tantardini , R. Martinazzo

We study the interaction of atomic and molecular hydrogen with a surface of tholin, a man-made polymer considered to be an analogue of aerosol particles present in Titan's atmosphere, using thermal programmed desorption at low temperatures…

Earth and Planetary Astrophysics · Physics 2010-10-08 Ling Li , Hui Zhao , Gianfranco Vidali , Yechiel Frank , Ingo Lohmar , Hagai B. Perets , Ofer Biham

A new setup for doping helium nanodroplets by means of laser ablation at kilohertz repetition rate is presented. The doping process is characterized and two distinct regimes of laser ablation are identified. The setup is shown to be…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Mudrich , B. Forkl , S. Mueller , M. Dvorak , O. Buenermann , F. Stienkemeier

Pristine graphene is not suitable for hydrogen storage at ambient conditions since it binds the hydrogen molecules only by van der Waals interactions. However, the adsorption energy of the hydrogen molecules can be improved by doping or…

Materials Science · Physics 2022-10-24 Vikram Mahamiya , Alok Shukla , Nandini Garg , Brahmananda Chakraborty

Nanostrucured Europium oxide and hydroxide films were obtained by pulsed Nd:Yag (532 nm) laser ablation of an Europium metallic target, in the presence of a 1 mbar Helium buffer atmosphere. Both the produced film and the ambient plasma were…

We demonstrate the temperature-mediated and completely reversible process of desorption-readsorption of water on a few layers of epitaxial graphene on a 4H-SiC(0001) substrate. We show that under ambient conditions water forms solid…

Mesoscale and Nanoscale Physics · Physics 2012-04-17 Tim L. Burnett , Jack Patten , Olga Kazakova

Using the pseudopotential density functional method as well as equilibrium thermodynamic functions, we explore the process of releasing H2 molecules adsorbed on a transition metal atom caused by the hydrogen-ammonia partial pressure…

Materials Science · Physics 2015-05-19 Hoonkyung Lee , Bing Huang , Wenhui Duan , Jisoon Ihm

Density functional calculations of electronic structure, total energy, structural distortions, and magnetism for hydrogenated single-layer, bilayer, and multi-layer graphene are performed. It is found that hydrogen-induced magnetism can…

Materials Science · Physics 2008-01-24 D. W. Boukhvalov , M. I. Katsnelson , A. I. Lichtenstein

Terahertz (THz) radiation has uses from security to medicine; however, sensitive room-temperature detection of THz is notoriously difficult. The hot-electron photothermoelectric effect in graphene is a promising detection mechanism:…

The ability of atomic hydrogen to chemisorb on graphene makes the latter a promising material for hydrogen storage. Based on scanning tunneling microscopy techniques, we report on site-selective adsorption of atomic hydrogen on convexly…

Absorption spectra of liquid water at 300 K are calculated from both classical and density functional theory molecular dynamics simulation data, which together span from 1 MHz to hundreds of THz, agreeing well with experimental data…

Chemical Physics · Physics 2020-09-09 Shane Carlson , Florian N. Brünig , Philip Loche , Douwe Jan Bonthuis , Roland R. Netz