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A prominent band centered at around 1000-1300 cm-1 and associated with resonant enhancement of two-phonon Raman scattering is reported in multiferroic BiFeO3 thin films and single crystals. A strong anomaly in this band occurs at the…

We have elucidated the spin, lattice, charge and orbital coupling mechanism underlying the multiferroic character in tensile strained EuTiO3 films. Symmetry determined by oxygen octahedral tilting shapes the hybridization between the Eu 4f…

Multiferroic materials, characterized by the coexisting of ferroelectric polarization (breaking spatial inversion symmetry) and magnetism (breaking time-reversal symmetry), with strong magnetoelectric coupling, are highly sought after for…

Materials Science · Physics 2025-04-14 Wei Sun , Wenxuan Wang , Changhong Yang , Ying Liu , Xiaotian Wang , Shifeng Huang , Zhenxiang Cheng

The coupling between ferroelectric and magnetic orders in multiferroic materials and the nature of magnetoelectric (ME) effects are enduring experimental challenges. In this work, we have studied the response of magnetization to…

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric…

Strongly Correlated Electrons · Physics 2014-03-18 Tathamay Basu , P. L. Paulose , Kartik K Iyer , Kiran Singh , N. Mohapatra , S. Chowki , Babu Gonde , E. V. Sampathkumaran

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

Magnetic structure evolution of multiferroic hexagonal $YMn_{1-x}Fe_{x}O_{3}$ (${x} = 0, 0.05,$ and $0.1$) has been studied by carrying out detailed temperature-dependent neutron diffraction at zero- and 5T-fields. Thermodynamic data…

Materials Science · Physics 2017-07-26 Sonu Namdeo , S. S. S. Rao , S. D. Kaushik , V. Siruguri , A. M. Awasthi

We studied magneto-optical response of a canonical topological insulator Bi$_2$Se$_3$ with the goal of addressing a controversial issue of electron-phonon coupling. Magnetic-field induced modifications of reflectance are very pronounced in…

Strongly Correlated Electrons · Physics 2016-10-12 S. V. Dordevic , G. M. Foster , M. S. Wolf , N. Stojilovic , H. Lei , C. Petrovic , Z. Chen , Z. Q. Li , L. C. Tung

The coexistence and coupling of magnetic and ferroelectric orderings in single phase multiferroics has evinced enormous scientific interest as it involves breaking of time reversal and space inversion symmetries in the same material. The…

Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any other known material in which the electric polarization is induced by spontaneous…

The emergence of magnetism in quantum materials creates a platform to realize spin-based applications in spintronics, magnetic memory, and quantum information science. A key to unlocking new functionalities in these materials is the…

Recent developments in two-dimensional (2D) magnetism have motivated the search for novel van-der Waals (vdWs) magnetic materials to explore new magnetic phenomenon in the 2D limit. Metal thiophosphates, MPX3, is a class of magnetic vdWs…

Materials Science · Physics 2021-06-30 Rabindra Basnet , Aaron Wegner , Krishna Pandey , Stephen Storment , Jin Hu

Topological quantum magnets FeSn and Fe$_{3}$Sn$_{2}$ were studied using neutron scattering and first-principles calculations. Both materials are metallic but host dispersionless flat bands with Dirac nodes at the $K$ point in reciprocal…

Materials Science · Physics 2023-05-17 Yu Tao , Luke Daemen , Yongqiang Cheng , Joerg C. Neuefeind , Despina Louca

We have investigated the temperature-dependent Raman-active phonons and the magnetic properties of Gd(Co1/2Mn1/2)O3 perovskite ceramics in the temperature range from 40 K to 300 K. The samples crystallized in an orthorhombic distorted…

Materials Science · Physics 2015-06-17 R. X. Silva , H. Reichlova , X. Marti , D. A. B. Barbosa , M. W. Lufaso , A. P. Ayala , C. W. A. Paschoal

We have studied the magnetodielectric and magnetoelastic coupling in TbFe3(BO3)4 single crystals by means of capacitance, magnetostriction and Raman spectroscopy measurements. The data reveal strong magnetic field effects on the dielectric…

We present the muon spin relaxation/rotation spectra in the multiferroic compound (Cu,Zn)$_{3}$Mo$_{2}$O$_{9}$. The parent material Cu$_{3}$Mo$_{2}$O$_{9}$ has a multiferroic phase below $T_{\rm N}$ = 8.0 K, where the canted…

Strongly Correlated Electrons · Physics 2014-03-26 H. Kuroe , K. Aoki , T. Sato , R. Kino , H. Kuwahara , T. Sekine , M. Hase , I. Kawasaki , T. Kawamata , T. Suzuki , I. Watanabe , K. Oka , T. Ito , H. Eisaki

In this work, we report the growth and functional characterizations of multiferroic TbMnO3 thin films grown on Nb-doped SrTiO3 (001) substrates using pulsed laser deposition. By performing detailed magnetic and ferroelectric properties…

Materials Science · Physics 2015-12-16 Ni Hu , Chengliang Lu , Zhengcai Xia , Rui Xiong , Pengfei Fang , Jing Shi , Jun-Ming Liu

We use a combination of optical spectra, first principles calculations, and energy dependent magneto-optical measurements to elucidate the electronic structure and to study the phase diagram of Ni$_3$V$_2$O$_8$. We find a remarkable…

Strongly Correlated Electrons · Physics 2007-05-23 R. C. Rai , J. Cao , S. Brown , J. L. Musfeldt , D. Kasinathan , D. J. Singh , G. Lawes , N. Rogado , R. J. Cava , X. Wei

Using spectral ellipsometry, we have measured the dielectric function of a Na$_{0.82(2)}$CoO$_2$ crystal that exhibits bulk antiferromagnetism with T$_{N}$=19.8 K. We identify two prominent transitions as a function of temperature. The…

Strongly Correlated Electrons · Physics 2009-11-10 C. Bernhard , A. V. Boris , N. N. Kovaleva , G. Khaliullin , A. Pimenov , L. Yu , D. P. Chen , C. T. Lin , B. Keimer

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch
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