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Photoionization of two buckyonions, C$_{60}$@C$_{240}$ and C$_{20}$@C$_{60}$, is investigated by means of time-dependent density-functional theory (TDDFT). The TDDFT-based photoabsorption spectrum of C$_{60}$@C$_{240}$, calculated in a…

Atomic and Molecular Clusters · Physics 2016-10-26 Alexey Verkhovtsev , Andrei V. Korol , Andrey V. Solov'yov

It is demonstrated for the first time that in spite of well known big similarities between atomic ionization by photons and fast electrons, a qualitative difference exists in angular anisotropy parameters of electrons knocked out in these…

Atomic Physics · Physics 2015-05-30 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

In this Letter, we investigate the non-dipole effects in time delay of photoelectrons emitted by multi-electron atoms, negative ions, and respective endohedrals. We present the necessary general formulas in the frame of the random phase…

Atomic Physics · Physics 2020-12-02 M. Ya. Amusia , L. V. Chernysheva

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

Atomic Physics · Physics 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

Angular distribution of photoelectrons released by the ionization of randomly-oriented molecules with two laser fields of carrier frequencies $\omega$ and $2\omega$, which are linearly polarized in two mutually-orthogonal directions, is…

Quantum Physics · Physics 2019-06-11 Philipp V. Demekhin

Photoionization of a Xe atom confined inside C$_{60}$ has been studied using the random phase approximation with exchange (RPAE) method. The C$_{60}$ fullerene has been descr ibed by an attractive short range spherical well with potential…

Atomic Physics · Physics 2009-11-13 Zhifan Chen , Alfred Z. Msezane

The spatial distributions of electric charges forming the C60 shell have been analyzed with the Poisson equation. It has been shown that the modification of formulas for the rectangular-potential-well as a model potential of the C60 shell…

Atomic Physics · Physics 2019-05-03 M. Ya. Amusia , A. S. Baltenkov

Possible reasons that confinement resonances are not observed in a recent photoionization experiment on the endohedral fullerene Ce@C82+ are explored. The effect of the polarization of the fullerene shell in response to the ionization of…

Atomic Physics · Physics 2010-03-23 V. K. Dolmatov , S. T. Manosn

We present a combined theoretical and experimental work investigating the angle-resolved phases of the photoionization process driven by a two-color field consisting of an attosecond pulse train and an infrared pulse in an ensemble of…

The present paper explores possible features of electron elastic scattering off endohedral fullerenes $A$@C$_{60}$. It focuses on how dynamical polarization of the encapsulated atom $A$ by an incident electron might alter scattering off…

Atomic Physics · Physics 2015-11-03 V. K. Dolmatov , M. Ya. Amusia , L. V. Chernysheva

Until recently, theoretical and experimental studies of photoelectron angular distributions (PADs) including non-dipole effects in atomic photo\-ionization have been performed mainly for the conventional plane-wave radiation. One can…

Atomic Physics · Physics 2023-08-21 Maksim D. Kiselev , Elena V. Gryzlova , Alexei N. Grum-Grzhimailo

Novel equations for the electric dipole polarizability $\alpha_{_{E1}}$ of low-lying excited states in atomic nuclei -- and the related $(-2)$ moment of the total photo-absorption cross section, $\sigma_{_{-2}}$ -- are inferred in terms of…

Nuclear Theory · Physics 2024-03-12 José Nicolás Orce , Cebo Ngwetsheni

The electron and ion properties observed in a photoionization inherit a symmetry properties of both a target and a radiation. Introducing a symmetry breaking in a photoionization process one can expect to observe a noticeable variation of…

Atomic Physics · Physics 2024-02-09 Maksim D. Kiselev , Elena V. Gryzlova , Alexei N. Grum-Grzhimailo

It is discovered theoretically that significant confinement resonances in an $nl$ photoionization of a \textit{multielectron} atom $A$ encaged in carbon fullerenes, A@C$_{60}$, may re-appear and be strong at photon energies far exceeding…

Atomic Physics · Physics 2015-05-13 V. K. Dolmatov , G. T. Craven , E. Guler , D. Keating

We provide the initial insight into the angle-differential photodetachment spectra of fullerene anions beyond the dipole approximation by utilizing a broadly used modelling of C$_{n}$. In the model, the C$_{n}$ cage is approximated by a…

Atomic Physics · Physics 2018-10-02 V K Dolmatov , A Edwards , C G Lane

It is demonstrated that the fullerene shell affects dramatically the radiative and Auger vacancy decay of an endohedral atom A@C60. The collectivized electrons of the C60 shell add new possibilities for radiative and non-radiative decays…

Atomic Physics · Physics 2022-06-13 M. Ya. Amusia , A. S. Baltenkov

Photoionization from atom-C60 hybrid levels in halogen endufullerene molecules, Cl@C60, Br@C60 and I@C60, are calculated using a linear response density functional method. Both the ordinary electron-configuration where the open shell…

Atomic and Molecular Clusters · Physics 2021-06-08 Dakota Shields , Ruma De , Esam Ali , Mohamed E Madjet , Steven T Manson , Himadri S. Chakraborty

Photoelectron angular distributions (PADs) obtained from ionization of potassium atoms using moderately intense femtosecond IR fields ($\sim$10$^{12}$Wcm$^{-2}$) of various polarization states are shown to provide a route to "complete"…

Atomic Physics · Physics 2015-01-15 Paul Hockett , Matthias Wollenhaupt , Christian Lux , Thomas Baumert

Photoelectron circular dichroism refers to the forward/backward asymmetry in the photoelectron angular distribution with respect to the propagation axis of circularly polarized light. It has recently been demonstrated in femtosecond…

Quantum Physics · Physics 2017-01-16 R. E. Goetz , T. A. Isaev , B. Nikoobakht , R. Berger , C. P. Koch

A theoretical investigation of photoabsorption and photoionization of Fe^{14+} extending beyond an earlier frame transformation R-matrix implementation is performed using a fully-correlated, Breit-Pauli R-matrix formulation including both…

Atomic Physics · Physics 2015-06-04 M. F. Hasoglu , T. W. Gorczyca , M. A. Bautista , Z. Felfli , S. T. Manson