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Fully quantum treatment explicitly presents the high harmonic generation as a three-stage process: above threshold ionization (ATI) is followed by the continuum electron propagation in a laser field and subsequent stimulated recombination…

Atomic Physics · Physics 2009-10-31 M. Yu. Kuchiev , V. N. Ostrovsky

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We extend our recently developed semiclassical strong-field Herman-Kluk propagator (SFHK) method to calculate high-order harmonic generation (HHG) for atoms in intense lasers. We show that our method, based on a combination of the…

Atomic Physics · Physics 2026-01-27 Phi-Hung Tran , Hao Quan Truong , R. Esteban Goetz , Anh-Thu Le

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

Atomic and Molecular Clusters · Physics 2009-11-13 A. Abdurrouf , F. H. M. Faisal

We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…

Atomic Physics · Physics 2016-08-24 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

Atomic Physics · Physics 2016-04-27 M. A. Khokhlova , V. V. Strelkov

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

The tomographic imaging of arbitrary molecular orbitals via high-order harmonic generation requires that electrons recollide from one direction only. Within a semi-classical model, we show that extremely short phase-stabilized laser pulses…

Atomic Physics · Physics 2009-11-13 Elmar V. van der Zwan , Manfred Lein

We present a study of non-sequential double recombination (NSDR) high harmonic generation (HHG) in a molecular-like system. Using a Coulomb-corrected three-step model we are able to classically describe the observed NSDR HHG cutoffs…

Atomic Physics · Physics 2017-07-12 Kenneth K. Hansen , Lars Bojer Madsen

High-harmonic generation (HHG) is widely used for up-conversion of amplified (near) infrared ultrafast laser pulses to short wavelengths. We demonstrate that Ramsey-comb spectroscopy, based on two such pulses derived from a frequency-comb…

Atomic Physics · Physics 2019-11-21 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. Favier , K. S. E. Eikema

We report here on results of experimental-theoretical investigation of high-order harmonic generation (HHG) in layers of CdSe semiconductor quantum dots of different sizes and a reference bulk CdSe thin film. We observe a strong decrease in…

The spectra produced by high-harmonic generation (HHG) typically exhibit well-defined peaks at odd integers times the laser frequency. However, in recent investigations of HHG from correlated materials, spectra exhibit signals at noninteger…

Atomic Physics · Physics 2024-06-05 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

We introduce high-harmonic sideband spectroscopy (HHSS) and show that it can be a robust probe of attosecond charge migration (CM) in a halogenated carbon-chain molecule. We simulate both the CM and harmonic-generation (HHG) dynamics using…

Quantum information science and intense laser matter interaction are two apparently unrelated fields. Here, we introduce the notion of quantum information theory to intense laser driven processes by providing the quantum mechanical…

Quantum Physics · Physics 2022-12-12 Philipp Stammer

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

The phenomenon of quantum revivals resulting from the self-interference of wave packets has been observed in several quantum systems and utilized widely in spectroscopic applications. Here, we present a combined analytical and numerical…

Quantum Physics · Physics 2021-01-04 Chuan-Cun Shu , Qian-Qian Hong , Yu Guo , Niels E. Henriksen

Motivated by the emerging experiments [e.g. \textit{Z. Nie et al. Nat. Photon. \textbf{12}, 489 (2018)}] on producing infrared (IR) single cycle pulses in the spectral region 5 - 14 $\mu m$, we theoretically investigate their role for…

Atomic Physics · Physics 2020-12-01 Abdelmalek Taoutioui , Hicham Agueny

A quantum coherent capacitor subject to large amplitude pulse cycles can be made to emit or reabsorb an electron in each half cycle. Quantized currents with pulse cycles in the GHz range have been demonstrated experimentally. We develop a…

Mesoscale and Nanoscale Physics · Physics 2008-02-27 M. Moskalets , P. Samuelsson , M. Buttiker
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