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We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…

Optics · Physics 2022-01-25 Yigeng Peng , Tong Wu , Guanglu Yuan , Lihan Chi , Chao Yu , Ruifeng Lu

Recent advancements in the generation of mid-infrared and terahertz laser pulses have enabled us to observe strong-field driven non-perturbative high-harmonic generation (HHG) from semiconductors, dielectrics, and semimetals. HHG has added…

Optics · Physics 2022-03-22 M. S. Mrudul

We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

The mechanism of the terahertz (THz) wave generation (TWG) in dual-color fields is elucidated within the theoretical framework of single-atom based strong field approximation (SFA). Evaluating the transition dipole moment, the…

Quantum Physics · Physics 2019-04-30 Kaixuan Zhang , Yizhu Zhang , Shuai Li , Xincheng Wang , Tian-Min Yan , Y. H. Jiang

High-order harmonic generation (HHG) in gases has been studied for almost 40 years in many different conditions, varying the laser wavelength, intensity, focusing geometry, target design, gas species, etc. However, no systematic…

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

We study nonlinear optical response of Landau quantized graphene to an intense electromagnetic wave. In particular, we consider high harmonic generation process. It is shown that one can achieve efficient generation of high harmonics with…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 H. K. Avetissian , A. G. Ghazaryan , G. F. Mkrtchian , Kh. V. Sedrakian

Squeezing of optical fields, used as a powerful resource for many applications, and the radiation properties in the process of high harmonic generation have thus far been considered separately. In this Letter, we want to clarify that the…

High harmonic generation is a convenient way to obtain extreme ultraviolet light from table-top laser systems and the experimental tools to exploit this simple and powerful light source for time-resolved spectroscopy are being developed by…

Atomic and Molecular Clusters · Physics 2013-12-20 Jakob Grilj , Emily Sistrunk , Markus Koch , Markus Gühr

The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

We investigate the role of excited states in High-order Harmonic Generation by studying the spectral, spatial and temporal characteristics of the radiation produced near the ionization threshold of argon by few-cycle laser pulses. We show…

High-harmonic generation (HHG) has recently emerged as a promising method for generating non-classical states of light with frequencies spanning from the infrared up to the extreme ultraviolet regime. In this work, we theoretically…

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

The bi-circular scheme for high harmonic generation, which combines two counter-rotating circular fields with frequency ratio 2:1, has recently permitted to generate high harmonics with essentially circular polarization, opening the way for…

Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…

Atomic Physics · Physics 2008-08-14 Anh-Thu Le , Toru Morishita , C. D. Lin

We report on the development of a high-order harmonic generation (HHG)-based ultrafast high-repetition-rate (250 kHz) monochromatic extreme ultraviolet (21.6 eV) source with polarization tunability, specifically designed for multi-modal…

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

Atomic and Molecular Clusters · Physics 2009-11-13 A. Abdurrouf , F. H. M. Faisal

In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations…

Strongly Correlated Electrons · Physics 2024-08-20 Negin Moharrami Allafi , Michael H. Kolodrubetz , Marin Bukov , Vadim Oganesyan , Mohsen Yarmohammadi

Contributions of the pre-ionized H$_2$ (PI-H$_2$) and ionized H$_2^+$ subsystems of the two-electron H$_2$ system to its high-order harmonic generation in 8-cycle $\sin^{2}$-like ultrafast intense laser pulses are calculated and analyzed…

Atomic Physics · Physics 2018-04-18 Hossein Iravani , Hassan Sabzyan , Mohsen Vafaee , Behnaz Buzari
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