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The dielectric properties of CaCu3Ti4O12, a material showing colossal values of the dielectric constant, were investigated in a broad temperature and frequency range extending up to 1.3 GHz. A detailed equivalent circuit analysis of the…

Materials Science · Physics 2009-11-10 P. Lunkenheimer , R. Fichtl , S. G. Ebbinghaus , A. Loidl

Many transition-metal oxides show very large ("colossal") magnitudes of the dielectric constant and thus have immense potential for applications in modern microelectronics and for the development of new capacitance-based energy-storage…

Strongly Correlated Electrons · Physics 2015-03-13 P. Lunkenheimer , S. Krohns , S. Riegg , S. G. Ebbinghaus , A. Reller , A. Loidl

Recently, materials exhibiting colossal dielectric constant ($CDC$) have attracted significant attention because of their high dielectric constant and potential applications in electronic devices, such as high dielectric capacitors,…

Materials Science · Physics 2013-09-19 K. Liu , X. Y. Zhang

We present dielectric measurements of the colossal dielectric constant material CaCu3Ti4O12 extending up to 1.3 GHz also covering so far only rarely investigated single crystalline samples. Special emphasis is put on the second relaxation…

Materials Science · Physics 2007-07-19 S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

The dielectric constant of CaCu3Ti4O12 is measured with a different electrode geometry than previous measurements. Similar colossal values are obtained showing that they are "intrinsic" to the material. We show that in braced structures…

Condensed Matter · Physics 2007-05-23 A. P. Ramirez , G. Lawes , V. Butko , M. A. Subramanian , C. M. Varma

A thorough investigation of the dielectric properties of Cu2Ta4O12, a material crystallizing in a pseudo-cubic, perovskite-derived structure is presented. We measured the dielectric constant and conductivity of single crystals in an…

Materials Science · Physics 2009-11-10 B. Renner , P. Lunkenheimer , M. Schetter , A. Loidl , A. Reller , S. G. Ebbinghaus

In the present work the authors report results of broadband dielectric spectroscopy on various samples of CaCu3Ti4O12, including so far only rarely investigated single crystalline material. The measurements extend up to 1.3 GHz, covering…

Materials Science · Physics 2008-09-03 S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

The search for new materials with extremely high ("colossal") dielectric constants, required for future electronics, is one of the most active fields of modern materials science. However, the applicability of the colossal-epsilon'…

Materials Science · Physics 2009-03-24 S. Krohns , P. Lunkenheimer , Ch. Kant , A. V. Pronin , H. B. Brom , A. A. Nugroho , M. Diantoro , A. Loidl

The origins of an ultrahigh dielectric constant in polycrystalline CaCu3Ti4O12 (CCTO) was studied using the combination of impedance spectroscopy, electron microscopy, and scanning probe microscopy (SPM). Impedance spectra indicate that the…

Materials Science · Physics 2009-11-10 S. V. Kalinin , J. Shin , G. M. Veith , A. P. Baddorf , M. V. Lobanov , H. Runge , M. Greenblatt

Low-temperature specific-heat study has been performed on the insulating giant dielectric constant material CaCu3Ti4O12 and two related compounds, Bi2/3Cu3Ti4O12 and La0.5Na0.5Cu3Ti4O12, from 0.6 to 10 K. From analyzing the specific heat…

Materials Science · Physics 2009-11-13 C. P. Sun , Jianjun Liu , J. -Y. Lin , Chun-gang Duan , W. N. Mei , H. D. Yang

Experimental evidence is provided that colossal dielectric constants, epsilon >= 1000, sometimes reported to exist in a broad temperature range, can often be explained by Maxwell-Wagner type contributions of depletion layers at the…

Condensed Matter · Physics 2009-11-07 P. Lunkenheimer , V. Bobnar , A. V. Pronin , A. I. Ritus , A. A. Volkov , A. Loidl

The cubic perovskite-related ceramic CaCu3Ti4O12 has a very high static dielectric constant ~10000 at room temperature (RT), which drops to about 100 below about 100 K. Substituting Cd for Ca reduces the RT value of the dielectric constant…

Strongly Correlated Electrons · Physics 2007-05-23 C. C. Homes , T. Vogt , S. M. Shapiro , W. Si , S. Wakimoto , M. A. Subramanian

We have measured dielectric properties of Ca$_{1+x}$Cu$_{3-x}$Ti$_4$O$_{12}$ ($x$ = 0, 0.1, 0.5, 1, 1.5, 2, 2.9 and 3), and have found that Ca$_2$Cu$_2$Ti$_4$O$_{12}$ (a composite of CaCu$_3$Ti$_4$O$_{12}$ and CaTiO$_3$) exhibits a high…

Materials Science · Physics 2009-11-11 W. Kobayashi , I. Terasaki

We present a thorough dielectric investigation of the hexagonal perovskites La1.2Sr2.7IrO7.33 and La1.2Sr2.7RuO7.33 in a broad frequency and temperature range, supplemented by additional infrared measurements. The occurrence of giant…

Strongly Correlated Electrons · Physics 2016-08-16 P. Lunkenheimer , T. Götzfried , R. Fichtl , S. Weber , T. Rudolf , A. Loidl , A. Reller , S. G. Ebbinghaus

The large, temperature-independent, low-frequency dielectric constant recently observed in single-crystal CaCu{3}Ti{4}O{12} is most plausibly interpreted as arising from spatial inhomogenities of its local dielectric response. Probable…

Materials Science · Physics 2009-11-10 Morrel H. Cohen , J. B. Neaton , Lixin He , David Vanderbilt

We observe the large enhancement in the dielectric response near the percolation threshold in a composite nanoparticle system consisting of metallic RuO$_2$ grains embedded into dielectric CaCu$_3$Ti$_4$O$_1$$_2$ (CCTO) matrix and annealed…

Materials Science · Physics 2015-06-19 Rupam Mukherjee , Gavin Lawes , Boris Nadgorny

We report on phonon properties and electronic transitions in CaCu3Ti4O12, a material which reveals a colossal dielectric constant at room temperature without any ferroelectric transition. The results of far- and mid-infrared measurements…

Strongly Correlated Electrons · Physics 2008-01-28 Ch. Kant , T. Rudolf , F. Mayr , S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

Materials with high dielectric constant are in great demand for the miniaturization of electronic devices. More specifically, high dielectric constant polymer-ceramic composites are useful for embedded capacitor applications. A composite…

Materials Science · Physics 2013-01-18 P. Thomas , R. S. Ernest Ravindran , K. B. R. Varma

Using transmission electron microscopy (TEM) we studied CaCu3Ti4O12, an intriguing material that exhibits a huge dielectric response, up to kilohertz frequencies, over a wide range of temperature. Neither in single crystals, nor in…

Materials Science · Physics 2009-11-10 L. Wu , Y. Zhu , S. Park , S. Shapiro , G. Shirane , J. Tafto

The possibility of obtaining relatively high dielectric constant polymer-ceramic composite by incorporating the giant dielectric constant material, CaCu3Ti4O12 (CCTO) in a Poly(vinylidene fluoride) (PVDF) polymer matrix by melt mixing and…

Materials Science · Physics 2013-01-18 P. Thomasa , K. T. Varughese , K. Dwarakanath , K. B. R. Varma
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