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The two-dimensional transition-metal dichalcogenides (2D TMDCs) are an intriguing platform for studying light-matter interactions because they combine the electronic properties of conventional semiconductors with the optical resonances…

Mesoscale and Nanoscale Physics · Physics 2022-05-02 Aaron H. Rose , Taylor J. Aubry , Hanyu Zhang , Jao van de Lagemaat

The realization and control of polaritons is of paramount importance in the prospect of novel photonic devices. Here, we investigate the emergence of plasmon-exciton polaritons in hybrid structures consisting of a two-dimensional (2D)…

Mesoscale and Nanoscale Physics · Physics 2018-01-10 P. A. D. Gonçalves , L. P. Bertelsen , Sanshui Xiao , N. Asger Mortensen

Plasmonic structures are known to support the modes with subwavelength volumes in which the field matter interactions are greatly enhanced. Coupling between the molecular excitations and plasmons leading to formation of plexcitons has been…

Optics · Physics 2018-11-27 Jacob B Khurgin

The strong interaction of individual quantum emitters with resonant cavities is of fundamental interest for understanding light matter interactions. Plasmonic cavities hold the promise of attaining the strong coupling regime even under…

Optics · Physics 2016-06-28 Kotni Santhosh , Ora Bitton , Lev Chuntonov , Gilad Haran

We demonstrate strong exciton-plasmon coupling in silver nanodisk arrays integrated with monolayer MoS2 via angle-resolved reflectance microscopy spectra of the coupled system. Strong exciton-plasmon coupling is observed with the…

Materials Science · Physics 2016-04-20 Wenjing Liu , Bumsu Lee , Carl H. Naylor , Ho-Seok Ee , Joohee Park , A. T. Charlie Johnson , Ritesh Agarwal

We use the macroscopic quantum electrodynamics approach suitable for absorbing and dispersing media to study the properties and role of collective surface excitations --- excitons and plasmons --- in single-wall and double-wall carbon…

Mesoscale and Nanoscale Physics · Physics 2017-08-14 I. V. Bondarev , L. M. Woods , A. Popescu

Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial…

Recent years have seen a growing interest in strong coupling between plasmons and excitons, as a way to generate new quantum optical testbeds and influence chemical dynamics and reactivity. Strong coupling to bright plasmonic modes has been…

Mesoscale and Nanoscale Physics · Physics 2020-02-11 Ora Bitton , Satyendra Nath Gupta , Lothar Houben , Michal Kvapil , Vlastimil Křápek , Tomas Šikola , Gilad Haran

The demonstration of enhanced spontaneous emission of nanoscaled optical emitters near metallic nanoparticles and the recent realization of a nanolaser based on surface plasmon amplification by stimulated emission of radiation (spaser)…

Quantum Physics · Physics 2010-03-12 S. Savasta , R. Saja , A. Ridolfo , O. Di Stefano , P. Denti , F. Borghese

Achieving strong coupling between excitons of colloidal semiconductor quantum dots (QDs) and localized surface plasmon polaritons (LSPs) is critical for advanced room-temperature quantum emitter and sensing applications. A key challenge is…

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

We investigate the interactions between exciton-polaritons in N two-dimensional semiconductor layers embedded in a planar microcavity. In the limit of low-energy scattering, where we can ignore the composite nature of the excitons, we…

Mesoscale and Nanoscale Physics · Physics 2020-11-11 O. Bleu , G. Li , J. Levinsen , M. M. Parish

Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical…

Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale…

Room temperature strong coupling of WS_2 monolayer exciton transitions to metallic Fabry-Perot and plasmonic optical cavities is demonstrated. A Rabi splitting of 101 meV is observed for the Fabry-Perot cavity, more than double those…

Materials Science · Physics 2016-08-24 S. Wang , S. Li , T. Chervy , A. Shalabney , S. Azzini , E. Orgiu , J. A. Hutchison , C. Genet , P. Samori , T. W. Ebbesen

All-solid-state strong light-matter coupling systems with large vacuum Rabi splitting are great important for quantum information application, such as quantum manipulation, quantum information storage and processing. The monolayer…

Mesoscale and Nanoscale Physics · Physics 2017-04-27 Jinxiu Wen , Hao Wang , Huanjun Chen , Shaozhi Deng , Ningsheng Xu

Two-dimensional (2D) semiconducting microcavity, where exciton-polaritons can be formed, constitues a promising setup for exploring and manipulating various regimes of light-matter interaction. Here, the coupling between 2D excitons and…

Materials Science · Physics 2021-09-08 Dino Novko , Vito Despoja

We report on the resonant coupling between localized surface plasmon resonances (LSPRs) in nanostructured Ag films, and an adsorbed monolayer of Rhodamine 6G dye. Hybridization of the plasmons and molecular excitons creates new coupled…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 N. I. Cade , T. Ritman-Meer , D. Richards

Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D)…

We investigate the conditions yielding plasmon-exciton strong coupling at the single emitter level in the gap between two metal nanoparticles. A quasi-analytical transformation optics approach is developed that makes possible a thorough…

Mesoscale and Nanoscale Physics · Physics 2016-09-07 Rui-Qi Li , D. Hernangómez-Pérez , F. J. García-Vidal , A. I. Fernández-Domínguez