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Correlation between dielectric and magnetic properties was investigated on the triangular lattice antiferromagnets ACrO2 (A= Cu, Ag, Li, or Na) showing 120-degree spiral spin structure with easy-axis anisotropy. For the A= Cu and Ag…

Strongly Correlated Electrons · Physics 2009-11-13 S. Seki , Y. Onose , Y. Tokura

Using first principle calculations under the framework of density functional theory we have investigated the electronic structure, magnetism and ferroelectric polarization in the triangular lattice antiferromagnet AgFeO2, and its comparison…

Materials Science · Physics 2018-01-03 Jayita Chakraborty , Indra Dasgupta

The ferroelectric polarization of triangular-lattice antiferromagnets induced by helical spin-spiral order is not explained by any existing model of magnetic-order-driven ferroelectricity. We resolve this problem by developing a general…

Strongly Correlated Electrons · Physics 2011-10-11 H. J. Xiang , E. J. Kan , Y. Zhang , M. -H. Whangbo , X. G. Gong

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

Strongly Correlated Electrons · Physics 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

Multiferroic materials, in which electric polarization and magnetic order coexist and couple, offer rich opportunities for both fundamental discovery and technology. However, multiferroicity remains rare due to conflicting electronic…

Materials Science · Physics 2025-10-14 Y. Sun , Y. Ahn , D. Sapkota , H. S. Arachchige , R. Xue , S. Mozaffari , D. G. Mandrus , L. Zhao , J. Orenstein , V. Sunko

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

Dielectric study on Ca3Mn2O7 features relaxor-like segmented dynamics below the antiferromagnetic ordering. Dipolar relaxations of different origin are spectrally resolved exhibiting distinct H-field alterations. This identifies their…

Materials Science · Physics 2019-09-10 Pooja Sahlot , Gaurav Sharma , Vasant Sathe , Anand Mohan Awasthi

Ag2CrO2 is an S=3/2 frustrated triangular lattice antiferromagnet without orbital degree of freedom. With decreasing temperature, a 4-sublatice spin state develops. However, a long-range partially disordered state with 5 sublattices…

Strongly Correlated Electrons · Physics 2012-04-13 M. Matsuda , H. Yoshida , M. Isobe , C. de la Cruz , R. S. Fishman

Magnetic and dielectric properties of the hexagonal triangular lattice antiferromagnet 2H-AgFeO2 have been studied by neutron diffraction, magnetic susceptibility, specific heat, pyroelectric current, and dielectric constant measurements.…

Strongly Correlated Electrons · Physics 2019-03-05 Noriki Terada , Dmitry D. Khalyavin , Pascal Manuel , Yoshihiro Tsujimoto , Alexei A. Belik

We have performed high resolution neutron diffraction and inelastic neutron scattering experiments in the frustrated multiferroic hexagonal compounds RMnO3 (R=Ho, Yb, Sc, Y), which provide evidence of a strong magneto-elastic coupling in…

Strongly Correlated Electrons · Physics 2009-06-01 X. Fabreges , S. Petit , I. Mirebeau , S. Pailhes , L. Pinsard , A. Forget , M. T. Fernandez-Diaz , F. Porcher

We performed neutron single crystal and synchrotron X-ray powder diffraction experiments in order to investigate the magnetic and crystal structures of the conductive layered triangular-lattice antiferromagnet PdCrO2 with a putative spin…

The coupling of magnetic chiralities to the ferroelectric polarisation in multiferroic RbFe(MoO$_4$)$_2$ is investigated by neutron spherical polarimetry. Because of the axiality of the crystal structure below $T_\textrm{c}$ = 190 K,…

A phase transition is often accompanied by the appearance of an order parameter and symmetry breaking. Certain magnetic materials exhibit exotic hidden-order phases, in which the order parameters are not directly accessible to conventional…

Strongly Correlated Electrons · Physics 2019-10-10 Yao Shen , Changle Liu , Yayuan Qin , Shoudong Shen , Yao-Dong Li , Robert Bewley , Astrid Schneidewind , Gang Chen , Jun Zhao

The contribution of the polarization associated with the noncollinear parts of spins in the dielectric permeability tensor of multiferroic materials is considered. As the equilibrium state, we consider the systems of parallel spins, so we…

Materials Science · Physics 2025-05-13 Pavel A. Andreev

We study the multiferroic properties in the distorted tetrahedral quasi-one dimensional spin system Cu$_3$Mo$_2$O$_9$, in which the effects of the low dimensionality and the magnetic frustration are expected to appear simultaneously. We…

Strongly Correlated Electrons · Physics 2015-06-03 T. Hosaka , S. Hachiuma , H. Kuroe , T. Sekine , M. Hase , K. Oka , T. Ito , H. Eisaki , M. Fujisawa , S. Okubo , H. Ohta

The ferroelectricity of the spiral magnets LiCu2O2 and LiCuVO4 was examined by calculating the electric polarizations of their spin spiral states on the basis of density functional theory with spin-orbit coupling. Our work unambiguously…

Materials Science · Physics 2011-11-10 H. J. Xiang , M. -H. Whangbo

We present the microscopic theory of improper multiferroicity in BiMnO3, which can be summarized as follows: (1) the ferroelectric polarization is driven by the hidden antiferromagnetic order in the otherwise centrosymmetric C2/c structure;…

Materials Science · Physics 2010-11-01 I. V. Solovyev , Z. V. Pchelkina

We have demonstrated that ferroelectric polarization in a spin-driven multiferroic CuFe1-xGaxO2 with x = 0.035 can be controlled by the application of uniaxial pressure. Our neutron diffraction and in-situ ferroelectric polarization…

Strongly Correlated Electrons · Physics 2015-05-28 T. Nakajima , S. Mitsuda , T. Nakamura , H. Ishii , T. Haku , Y. Honma , M. Kosaka , N. Aso , Y. Uwatoko

Magnetoelectric and magnetoelastic phenomena correlated with a phase transition into noncollinear magnetic phase have been investigated for single crystals of CuFeO2 with a frustrated triangular lattice. CuFeO2 exhibits several…

Strongly Correlated Electrons · Physics 2009-11-11 T. Kimura , J. C. Lashley , A. P. Ramirez

We figure out that the ground state of a multiple-spin exchange model applicable to thin films of solid 3He possesses an octahedral spin nematic order. In the presence of magnetic field, it is deformed into an antiferro-quadrupolar order in…

Strongly Correlated Electrons · Physics 2012-02-06 Tsutomu Momoi , Philippe Sindzingre , Kenn Kubo
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