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The fundamental measure approach to classical density functional theory has been shown to be a powerful tool to predict various thermodynamic properties of hard-sphere systems. We employ this approach to determine not only one-particle…

Soft Condensed Matter · Physics 2015-11-02 Andreas Härtel , Matthias Kohl , Michael Schmiedeberg

This letter derives closed-form expressions for the probability density function of the distance between two nodes located in heterogeneous concentric geometries, namely a disk or sphere and a surrounding annulus or spherical shell. Two…

Information Theory · Computer Science 2026-05-07 Nicholas Vaiopoulos , Alexander Vavoulas , Harilaos G. Sandalidis , Konstantinos K. Delibasis

We report a detailed study, using state-of-the-art simulation and theoretical methods, of the depletion potential between a pair of big hard spheres immersed in a reservoir of much smaller hard spheres, the size disparity being measured by…

Statistical Mechanics · Physics 2013-05-29 Douglas J. Ashton , Nigel B. Wilding , Roland Roth , Robert Evans

A recently proposed rational-function approximation [Phys. Rev. E \textbf{84}, 041201 (2011)] for the structural properties of nonadditive hard spheres is applied to evaluate analytically (in Laplace space) the local density profiles of…

Soft Condensed Matter · Physics 2013-04-08 Riccardo Fantoni , Andrés Santos

An impurity particle coupling to its host fluid via inelastic hard sphere collisions is considered. It is shown that the exact equation for its distribution function can be mapped onto that for an impurity with elastic collisions and an…

Statistical Mechanics · Physics 2007-05-23 A. Santos , J. W. Dufty

We investigate excluded-volume effects in a bidisperse colloidal suspension near a flexible interface. Inspired by a recent experiment by Dinsmore et al. (Phys. Rev, Lett. 80, 409 (1998)), we study the adsorption of a mesoscopic bead on the…

Soft Condensed Matter · Physics 2009-11-10 Thomas Bickel

The influence of poor solvent quality on fluid demixing of a model mixture of colloids and nonadsorbing polymers is investigated using density functional theory. The colloidal particles are modelled as hard spheres and the polymer coils as…

Soft Condensed Matter · Physics 2009-11-07 Matthias Schmidt , Alan R. Denton

The structure of polydisperse hard sphere fluids, in the presence of a wall, is studied by the Rosenfeld density functional theory. Within this approach, the local excess free energy depends on only four combinations of the full set of…

Soft Condensed Matter · Physics 2009-10-31 I. Pagonabarraga , M. E. Cates , G. J. Ackland

We simulate a hard-sphere liquid in confined geometry where the separation of the two parallel, hard walls is smaller than two particle diameters. By systematically reducing the wall separation we analyze the behavior of structural and…

Soft Condensed Matter · Physics 2022-08-18 Gerhard Jung , Thomas Franosch

We extend the insertion approach for calculating depletion potentials to the case of non-spherical solutes. Instead of a brute-force calculation we suggest to employ the recently developed curvature expansion of density profiles close to…

Soft Condensed Matter · Physics 2009-11-11 P. -M. König , R. Roth , S. Dietrich

We simulate model systems of charged spherical particles in their counterion solution and measure the thermodynamic pressure and the pair distribution function from which we derive effective potentials of mean force. For a system with only…

Soft Condensed Matter · Physics 2007-05-23 Niels Gronbech-Jensen , Keith M Beardmore , Philip Pincus

A method is presented for finding anisotropic distribution functions for stellar systems with known, spherically symmetric, densities, which depends only on the two classical integrals of the energy and the magnitude of the angular…

Astrophysics · Physics 2008-12-31 Zhenglu Jiang , Leonid Ossipkov

Using a fundamental measure density functional theory we investigate both bulk and inhomogeneous systems of the binary non-additive hard sphere model. For sufficiently large (positive) non-additivity the mixture phase separates into two…

Soft Condensed Matter · Physics 2010-07-30 Paul Hopkins , Matthias Schmidt

A geometry-based density functional theory is presented for mixtures of hard spheres, hard needles and hard platelets; both the needles and the platelets are taken to be of vanishing thickness. Geometrical weight functions that are…

Soft Condensed Matter · Physics 2009-11-11 Ansgar Esztermann , Hendrik Reich , Matthias Schmidt

The structural properties of single component fluids of hard hyperspheres in odd space dimensionalities $d$ are studied with an analytical approximation method that generalizes the Rational Function Approximation earlier introduced in the…

Statistical Mechanics · Physics 2011-11-10 Rene D. Rohrmann , Andres Santos

We proposed a new extended version of Enskog theory for the description of the self-diffusion coefficient of a colloidal hard-sphere fluid adsorbed in a matrix of disordered hard-sphere obstacles. In a considered approach instead of contact…

Soft Condensed Matter · Physics 2025-06-26 M. F. Holovko , M. Ya. Korvatska

The response of amorphous solids to an applied shear deformation is an important problem, both in fundamental and applied research. To tackle this problem, we focus on a system of hard spheres in infinite dimensions as a solvable model for…

Statistical Mechanics · Physics 2019-10-11 Ada Altieri , Francesco Zamponi

The fundamental measure density functional theory for hard spheres is generalized to binary mixtures of arbitrary positive and moderate negative non-additivity between unlike components. In bulk the theory predicts fluid-fluid phase…

Soft Condensed Matter · Physics 2009-11-10 Matthias Schmidt

The discrepancy in nucleation rate densities between simulated and experimental hard spheres remains staggering and unexplained. Suggestively, more strongly sedimenting colloidal suspensions of hard spheres nucleate much faster than weakly…

Soft Condensed Matter · Physics 2021-12-08 Nicholas Wood , John Russo , Francesco Turci , C. Patrick Royall

We calculated the spatial distribution of reduced density and pair distribution function (PDF) of solvent hard spheres near a solute using three-dimensional Ornstein-Zernike (OZ) equations coupled with closures in which Percus-Yevick (PY)…

Soft Condensed Matter · Physics 2023-11-27 Mika Matsuo , Yuka Nakamura , Masahiro Kinoshita , Ryo Akiyama