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Ultrafast optical excitation of metals induces a non-equilibrium energy distribution in the electronic system, with a characteristic step-structure determined by Pauli blocking. On a femtosecond timescale, electron-electron scattering…

During the last decade, significant progress has been achieved in the rapidly growing field of the dynamics of {\it hot} carriers in metals. Here we present an overview of the recent achievements in the theoretical understanding of electron…

Materials Science · Physics 2007-05-23 J. M. Pitarke , V. P. Zhukov , R. Keyling , E. V. Chulkov , P. M. Echenique

We report a first-principles description of inelastic lifetimes of excited electrons in real Cu and Al, which we compute, within the GW approximation of many-body theory, from the knowledge of the self-energy of the excited quasiparticle.…

Materials Science · Physics 2009-10-31 I. Campillo , J. M. Pitarke , A. Rubio , E. Zarate , P. M. Echenique

Recent developments in electron hydrodynamics have demonstrated the importance of considering the full structure of the electron-electron scattering operator, which encodes a sequence of lifetimes, one for each component of the Fermi…

Strongly Correlated Electrons · Physics 2025-10-08 Davis Thuillier , Sayak Ghosh , B. J. Ramshaw , Thomas Scaffidi

A semiempirical theory for the excitation and subsequent relaxation of nonthermal electrons is described. The theory, which is applicable to ultrafast-laser excited metals, is based on the Boltzmann transport equation for the carrier…

Materials Science · Physics 2023-07-12 D. M. Riffe , Richard B. Wilson

We present an analysis of positron lifetimes in solids with unprecedented depth. Instead of modeling correlation effects with density functionals, we study positron-electron wave functions with long-range correlations included. This gives…

Other Condensed Matter · Physics 2022-10-18 K. A. Simula , J. E. Muff , I. Makkonen , N. D. Drummond

We derive and evaluate expressions for the dc tunneling conductance between interacting two-dimensional electron systems at non-zero temperature. The possibility of using the dependence of the tunneling conductance on voltage and…

Condensed Matter · Physics 2009-10-28 T. Jungwirth , A. H. MacDonald

An effective Hamiltonian which could model the interaction between a tunneling proton and the conduction electrons of a metal is investigated. A remarkably simple correlation between the motion of the $TLS$-atom and an angular-momentum…

Strongly Correlated Electrons · Physics 2007-11-19 I. Nagy , A. Zawadowski

Linear-scaling electronic structure methods based on the calculation of moments of the underlying electronic Hamiltonian offer a computationally efficient and numerically robust scheme to drive large-scale atomistic simulations, in which…

Materials Science · Physics 2017-01-09 Eunan J. McEniry , Ralf Drautz

First-principles calculations of the inelastic lifetime of low-energy electrons in Al, Mg, Be, and Cu are reported. Quasiparticle damping rates are evaluated from the knowledge of the electron self-energy, which we compute within the GW…

Materials Science · Physics 2009-10-31 I. Campillo , V. M. Silkin , J. M. Pitarke , E. V. Chulkov , A. Rubio , P. M. Echenique

In this paper, we study the one-level Friedrichs model with using the quantum time super-operator that predicts the excited state decay inside the continuum. Its survival probability in long time limit is an algebraically decreasing…

Quantum Physics · Physics 2007-11-26 Maurice Courbage , Seyed Majid Saberi Fathi

The non-equilibrium dynamics of electrons is of a great experimental and theoretical value providing important microscopic parameters of the Coulomb and electron-phonon interactions in metals and other cold plasmas. Because of the…

Superconductivity · Physics 2008-11-19 V. V. Kabanov , A. S. Alexandrov

Electron-photon temporal correlations in electron energy loss (EELS) and cathodoluminescence (CL) spectroscopies have recently been used to measure the relative quantum efficiency of materials. This combined spectroscopy, named…

We introduce a general Monte Carlo scheme for achieving atomistic simulations with monoelectronic Hamiltonians including the thermalization of both nuclear and electronic degrees of freedom. The kinetic Monte Carlo algorithm is used to…

Materials Science · Physics 2009-11-07 F. Calvo , F. Spiegelman

The structural evolution of laser-excited systems of gold has previously been measured through ultrafast MeV electron diffraction. However, there has been a long-standing inability of atomistic simulations to provide a consistent picture of…

Materials Science · Physics 2024-06-19 J. M. Molina , T. G. White

We propose a multipole representation of the Fermi-Dirac function and the Fermi operator, and use this representation to develop algorithms for electronic structure analysis of metallic systems. The new algorithm is quite simple and…

Materials Science · Physics 2010-10-26 Lin Lin , Jianfeng Lu , Roberto Car , Weinan E

A simple Monte Carlo procedure is described for simulating the multiple scattering and absorption of electrons with the incident energy in the range 1-50 keV moving through a slab of uniformly distributed material of given atomic number,…

Materials Science · Physics 2007-05-23 Nima Ghal-eh , Mohammad Farhad Rahimi , Mehrnoush Manouchehri

We consider a simple model for the geminate electron-hole separation process in organic photovoltaic cells, in order to illustrate the influence of dimensionality of conducting channels on the efficiency of the process. The Miller-Abrahams…

Computational Physics · Physics 2014-03-27 Paraskevas Giazitzidis , Panos Argyrakis , Juan Bisquert , Vyacheslav S. Vikhrenko

We calculate potential curves for transition metal dimers using Monte Carlo configuration interaction (MCCI). These results, and their associated spectroscopic values, are compared with experimental and computational studies. The…

Chemical Physics · Physics 2014-05-23 J. P. Coe , P. Murphy , M. J. Paterson

Focusing on the $2\mathrm{p}-1\mathrm{s}$ transition in atomic Hydrogen, we investigate through first order perturbation theory the time evolution of the survival probability of an electron initially taken to be in the excited…

Quantum Physics · Physics 2015-09-07 V. Debierre , T. Durt , A. Nicolet , F. Zolla
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