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The notion of strong electronic correlations arose in the context of $d$-metal oxides such as NiO but can be exemplified on systems as simple as the H$_2$ molecule. Here we shed light on correlation effects on B$_6^{2-}$ clusters as found…

Strongly Correlated Electrons · Physics 2022-11-11 Thorben Petersen , Ulrich K. Rößler , Liviu Hozoi

Very recently, two-dimensional(2D) boron sheets (borophene) with rectangular structure has been grown successfully on single crystal Ag(111) substrates.The fabricated boroprene is predicted to have unusual mechanical properties. We…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 Haifeng Wang , Qingfang Li , Yan Gao , F. Miao , Xiang-Feng Zhou , X. G. Wan

Boron is a unique element, being the only element, all known polymorphs of which are superhard, and all of its crystal structures are distinct from any other element. The electron-deficient bonding in boron explains its remarkable…

Materials Science · Physics 2011-01-11 A. R. Oganov , V. L. Solozhenko

Using density functional theory (DFT) and quantum Monte Carlo (QMC) calculations we show that the B12Hn and B12Fn (n = 0-4) quasi-planar structures are energetically more favorable than the corresponding icosahedral clusters. Moreover, we…

Mesoscale and Nanoscale Physics · Physics 2021-09-21 N. Gonzalez Szwacki , C. J. Tymczak

A family of unusually stable boron cages was identified and examined using first-principles local density functional method. The structure of the fullerenes is similar to that of the B12 icosahedron and consists of six crossing…

Materials Science · Physics 2021-09-21 Nevill Gonzalez Szwacki

The present work carries out molecular dynamics simulations to compute the thermal conductivity of the borophene nanoribbon and the borophene nanotube using the Muller-Plathe approach. We investigate the thermal conductivity of the armchair…

Computational Physics · Physics 2020-06-30 Yue Jia , Chun Li , Jin-Wu Jiang , Ning Wei , Yang Chen , Yongjie Jessica Zhang

In the present study, the structural and hitherto uninvestigated mechanical (elastic stiffness constants, machinability index, Cauchy pressure, anisotropy indices, brittleness/ductility, Poissons ratio), electronic, optical, and…

Materials Science · Physics 2021-05-19 M. M. Hossain , M. A. Ali , M. M. Uddin , A. K. M. A. Islam , S. H. Naqib

We show that newly found BF3-doped polyaniline, though highly conducting, remains amorphous. Magnetic studies reveal many unusual properties, while suggesting that the intrinsic conductivity of this system is significantly larger than all…

Materials Science · Physics 2009-11-10 Debangshu Chaudhuri , Ashwani Kumar , D. D. Sarma , M. Garcia-Hernandez , J. Joshi , S. V. Bhat

The electronic structure of benzene in the presence of a high-intensity high-frequency circularly polarized laser supports a middle-of-the-ring electron localization. Here, the laser polarization coincides with the ring plane of benzene.…

Chemical Physics · Physics 2019-11-19 Prashant Raj , Mishu Paul , Mythreyi R. , Balanarayan Pananghat

Interstellar aromatic molecules such as polycyclic aromatic hydrocarbons and polycyclic nitrogen and oxygen bearing molecules are thought to be abundant in the interstellar medium. In this class of molecules, benzonitrile ($c$-C$_6$H$_5$CN)…

Astrophysics of Galaxies · Physics 2024-01-19 M. Ben Khalifa , J. Loreau

Theoretical predictions of pressure-induced phase transformations often become long-standing enigmas because of limitations of contemporary available experimental possibilities. Hitherto the existence of a non-icosahedral boron allotrope…

Boron arsenide (BAs) with a zinc blende structure has recently been discovered to exhibit unusual and ultrahigh thermal conductivity (k), providing a new outlook for research on BAs and other high thermal conductivity materials. Technology…

In recent years, two-dimensional boron sheets (borophene) have been experimentally synthesized and theoretically observed as promising conductor or transistor with novel thermal and electronic properties. We first give a general survey of…

Materials Science · Physics 2018-03-16 Dengfeng Li , Ying Chen , Jia He , Qiqi Tang , Chengyong Zhong , Guangqian Ding

The most recent experimental advances could provide ways for the fabrication of several atomic thick and planar forms of boron atoms. For the first time, we explore the mechanical properties of five types of boron films with various vacancy…

Materials Science · Physics 2017-04-17 Minh-Quy Le , Bohayra Mortazavi , Timon Rabczuk

Boron suboxide B6O, the hardest known oxide, has an R-3m crystal structure ({\alpha}-B6O) that can be described as an oxygen-intercalated structure of {\alpha}-boron, or, equivalently, as a cubic close packing of B12 icosahedra with two…

We study the mechanical properties of two-dimensional (2D) boron, borophenes, by first-principles calculations. The recently synthesized borophene with 1/6 concentration of hollow hexagons (HH) is shown to have in-plane modulus C up to 210…

Materials Science · Physics 2017-01-12 Zhuhua Zhang , Yang Yang , Evgeni S. Penev , Boris I. Yakobson

By bridging graphene and benzene through a well-defined sequence of polycyclic aromatic hydrocarbons and their inherent shell structure, J. Phys. Chem. C, 2018, 122, 17526, it is shown that graphene is actually a coherent arrangement of…

Chemical Physics · Physics 2020-07-01 Aristides D. Zdetsis

This letter investigates the applications and extensions of the resource theory of quantum superposition within the realm of quantum chemistry. Specifically, we explore aromaticity, a fundamental concept originally developed to elucidate…

Quantum Physics · Physics 2024-04-16 Mahir H. Yeşiller , Onur Pusuluk

Charge transfer from a metal substrate stabilizes honeycomb borophene, whose electron deficit would otherwise spoil the hexagonal order of a $\pi$-bonded 2D atomic network. However, the coupling between the substrate and the boron overlayer…

Materials Science · Physics 2022-11-30 Mandana Safari , Erik Vesselli , Stefano de Gironcoli , Stefano Baroni

Borophene, a monoatomic layer of boron atoms, stands out among two-dimensional (2D) materials, with its versatile properties of polymorphism, metallicity, plasmonics, superconductivity, tantalizing for physics exploration and…

Materials Science · Physics 2021-11-25 Qiyuan Ruan , Luqing Wang , Ksenia V. Bets , Boris I. Yakobson