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Several theoretical predictions have claimed that the neutral exciton of TMDCs splits into a transversal and longitudinal exciton branch, with the longitudinal one, which is the upper branch, exhibiting an extraordinary strong dispersion in…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

The dark exciton state in semiconductor quantum dots constitutes a long-lived solid-state qubit which has the potential to play an important role in implementations of solid-state based quantum information architectures. In this work, we…

Luminescent colloidal CdSe nanorings are a new type of semiconductor structure that have attracted interest due to the potential for unique physics arising from their non-trivial toroidal shape. However, the exciton properties and dynamics…

The photoluminescence spectra of spherical CdTe nanocrystals with zincblende structure are studied by size-selective spectroscopic techniques. We observe a resonant Stokes shift of 15 meV when the excitation laser energy is tuned to the red…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee , M. Chamarro , P. Lavallard , V. D. Petrikov , A. A. Lipovskii

Excitons, Coulomb-bound electron and hole pairs, are elementary photo-excitations in semiconductors, that can couple directly to light through radiative relaxation. In contrast to these bright excitons, dark excitons X$\rm{_D}$ with…

Materials Science · Physics 2018-02-14 Kyoung-Duck Park , Tao Jiang , Genevieve Clark , Xiaodong Xu , Markus B. Raschke

In an effort to elucidate the spin (rather than charge) degrees of freedom in colloidal semiconductor nanocrystal quantum dots, we report on a series of static and time-resolved photoluminescence measurements of colloidal CdSe quantum dots…

Materials Science · Physics 2007-05-23 Madalina Furis , Jennifer Hollingsworth , Victor I. Klimov , Scott A. Crooker

The fine structure of the exciton spectrum, containing optically allowed (bright) and forbidden (dark) exciton states, determines the radiation efficiency in nanostructures. We study time-resolved micro-photoluminescence in MoS$_2$…

Circularly polarized optical excitation is used to demonstrate the efficient injection of spin-polarized excitons to individual self-assembled CdSe quantum dots in ZnSe barrier. The exciton spin-transfer is studied by means of…

Mesoscale and Nanoscale Physics · Physics 2014-08-14 T. Smoleński , W. Pacuski , M. Goryca , M. Nawrocki , A. Golnik , P. Kossacki

We report on the exciton spin dynamics of nanowire embedded GaN/AlN Quantum Dots (QDs) investigated by time-resolved photoluminescence spectroscopy. Under a linearly polarized quasiresonant excitation we evidence the quenching of the…

Materials Science · Physics 2015-05-28 A. Balocchi , J. Renard , C. T. Nguyen , B. Gayral , T. Amand , H. Mariette , B. Daudin , G. Tourbot , X. Marie

We present a comparative study of two self-assembled quantum dot (QD) systems based on II-VI compounds: CdTe/ZnTe and CdSe/ZnSe. Using magneto-optical techniques we investigated a large population of individual QDs. The systematic…

We study an impact of the fine structure of the heavy--hole ground state exciton confined in semiconductor quantum dots on the photoluminescence polarization dynamics solving the relevant system of the rate equations. The presence of the…

Mesoscale and Nanoscale Physics · Physics 2014-02-21 E. Tsitsishvili , H. Kalt

Using a first-principle approach beyond density functional theory we calculate the electronic and optical properties of small diameter CdSe nanowires.Our results demonstrate how some approximations commonly used in bulk systems fail at this…

Mesoscale and Nanoscale Physics · Physics 2010-07-30 J. G. Vilhena , S. Botti , M. A. L. Marques

We measure the photoluminescence (PL) lifetime, $\tau$, of excitons in colloidal PbSe nanocrystals (NCs) at low temperatures to 270~mK and in high magnetic fields to 15~T. For all NCs (1.3-2.3~nm radii), $\tau$ increases sharply below 10~K…

Mesoscale and Nanoscale Physics · Physics 2010-08-24 R. D. Schaller , S. A. Crooker , D. A. Bussian , J. M. Pietryga , J. Joo , V. I. Klimov

We present both experimental and theoretical results on the influence of a magnetic field on excitons in semiconductor quantum dots. We find a pronounced difference between the strong and weak confinement regimes. For weak confinement, the…

We demonstrate a new method of measuring the exciton spin relaxation time in semiconductor nanostructures by continuous-wave photoluminescence. We find that for self-assembled CdTe quantum dots the degree of circular polarization of…

Materials Science · Physics 2009-11-10 S. Mackowski , T. A. Nguyen , H. E. Jackson , L. M. Smith , J. Kossut , G. Karczewski

Semiconductor nanoplatelets (NPLs), with their large exciton binding energy, narrow photoluminescence (PL), and absence of dielectric screening for photons emitted normal to the NPL surface, could be expected to become the fastest…

The optical properties of particularly the tungsten-based transition-metal dichalcogenides are strongly influenced by the presence of dark excitons. Recently, theoretical predictions as well as indirect experimental insights have shown that…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Formation of excitonic states in quantum dots of nitride based III-V semiconductors GaN and AlN including coulomb and exchange interactions are investigated. Dark exciton formation is found to occur for both GaN quantum dots(QDs) with…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Anjana Bagga , P. K. Chattopadhyay , Subhasis Ghosh

The recombination dynamics and spin polarization of excitons in CdSe nanocrystals synthesized in a glass matrix are investigated using polarized photoluminescence in high magnetic fields up to 30 Tesla. The dynamics are accelerated by…

The optical orientation and alignment of excitons in semiconductor indirect gap quantum dots have been studied theoretically. A special regime is analyzed in which the energy of the hyperfine interaction of an electron with lattice nuclei…

Mesoscale and Nanoscale Physics · Physics 2024-05-27 D. S. Smirnov , E. L. Ivchenko