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The effect of exchange interactions within spin pairs on spin-dependent transport and recombination rates through localized states in semiconductors during coherent electron spin resonant excitation is studied theoretically. It is shown…

Materials Science · Physics 2008-01-09 A. Gliesche , C. Michel , V. Rajevac , K. Lips , S. D. Baranovskii , F. Gebhard , C. Boehme

We theoretically investigate quantum spin transfer from spin-correlated conduction-electron pairs to localized spins in a ferromagnet, given that electrons are correlated intrinsically. We show that even spin-singlet pairs and triplet pairs…

Mesoscale and Nanoscale Physics · Physics 2026-01-09 Seongmun Hwang , Jung Hyun Oh , Paul M. Haney , Mark D. Stiles , Kyung-Jin Lee

We present a practical semiclassical method for computing the electron spin dynamics of a radical in which the electron spin is hyperfine coupled to a large number of nuclear spins. This can be used to calculate the singlet and triplet…

Chemical Physics · Physics 2014-07-09 David E. Manolopoulos , P. J. Hore

We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…

Mesoscale and Nanoscale Physics · Physics 2024-02-16 Yan Sun , L. R. Weiss , V. Derkach , J. E. Anthony , M. Monteverde , A. D. Chepelianskii

Spin-orbit coupling is relatively weak for electrons in bulk silicon, but enhanced interactions are reported in nanostructures such as the quantum dots used for spin qubits. These interactions have been attributed to various dissimilar…

From organic electronics to biological systems, understanding the role of intermolecular interactions between spin pairs is a key challenge. Here we show how such pairs can be selectively addressed with combined spin and optical…

We have evaluated hyperfine-induced electron spin dynamics for two electrons confined to a double quantum dot. Our quantum solution accounts for decay of a singlet-triplet correlator even in the presence of a fully static nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 W. A. Coish , Daniel Loss

We have used an efficient new quantum mechanical method for radical pair recombination reactions to study the spin-dependent charge recombination along PTZ$^{\bullet+}$--Ph$_n$--PDI$^{\bullet-}$ molecular wires. By comparing our results to…

Chemical Physics · Physics 2017-10-31 Thomas P. Fay , Alan M. Lewis , David E. Manolopoulos

S=1/2 quantum spin chains and ladders with random exchange coupling are studied by using an effective low-energy field theory and transfer matrix methods. Effects of the nonlocal correlations of exchange couplings are investigated…

Disordered Systems and Neural Networks · Physics 2007-05-23 K. Takeda , I. Ichinose

Radical pair recombination reactions are normally described using a quantum mechanical master equation for the electronic and nuclear spin density operator. The electron spin state selective (singlet and triplet) recombination processes are…

Chemical Physics · Physics 2018-08-10 Thomas P. Fay , Lachlan P. Lindoy , David E. Manolopoulos

Dynamical buildup of spin-singlet correlations between the two quantum dots is investigated by means of the time-dependent numerical renormalization group method. By calculating the timeevolution of the spin-spin expectation value upon a…

Mesoscale and Nanoscale Physics · Physics 2024-03-19 Kacper Wrześniewski , Tomasz Ślusarski , Ireneusz Weymann

The transfer of information between quantum systems is essential for quantum communication and computation. In quantum computers, high connectivity between qubits can improve the efficiency of algorithms, assist in error correction, and…

Orbital entropies, pair entropies, and mutual information have become popular tools for analysis of strongly correlated wave functions. They can quantitatively measure how strongly an orbital (e.g. from the DMRG active space) participates…

Chemical Physics · Physics 2025-05-19 Jiri Pittner

Electron wave function entanglement and spin reconfiguration as source of electron correlation are investigated. Properties of correlation function are shown to have the best concordance with experimental data under supposition that…

Quantum Physics · Physics 2007-05-23 V O Hnatovsky , C V Usenko

In this paper we outline a physically motivated framework for describing spin-selective recombination processes in chiral systems, from which we derive spin-selective reaction operators for recombination reactions of donor-bridge-acceptor…

Chemical Physics · Physics 2023-03-09 Thomas P. Fay , David T. Limmer

We determine the spin exchange coupling J between two electrons located in two vertically tunnel-coupled quantum dots, and its variation when magnetic (B) and electric (E) fields (both in-plane and perpendicular) are applied. We predict a…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Guido Burkard , Georg Seelig , Daniel Loss

We theoretically study the interplay of spin-orbit and hyperfine interactions in dynamical nuclear polarization in two-electron semiconductor double quantum dots near the singlet $(S)$ - triplet $(T_+)$ anticrossing. The goal of the scheme…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Marko J. Rančić , Guido Burkard

We perform a systematic exact diagonalization study of spin-orbit coupling effects for stationary few-electron states confined in quasi two-dimensional double quantum dots. We describe the spin-orbit-interaction induced coupling between…

Mesoscale and Nanoscale Physics · Physics 2010-06-17 M. P. Nowak , B. Szafran

We estimate the triplet-singlet relaxation rate due to spin-orbit coupling assisted by phonon emission in weakly-confined quantum dots. Our results for two and four electrons show that the different triplet-singlet relaxation trends…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Juan I. Climente , Andrea Bertoni , Guido Goldoni , Massimo Rontani , Elisa Molinari

Based on a scheme that produces an entanglement between the spin and the path variables of a single spin-1/2 particle (qubit) using a beam-splitter and a spin-flipper, we formulate a procedure for transferring this intraparticle hybrid…

Quantum Physics · Physics 2015-05-14 S. Adhikari , A. S. Majumdar , Dipankar Home , Alok Kumar pan
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