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We present a tight-binding based GW approach for the calculation of quasiparticle energy levels in confined systems such as molecules. Key quantities in the GW formalism like the microscopic dielectric function or the screened Coulomb…

Materials Science · Physics 2009-11-10 T. A. Niehaus , M. Rohlfing , F. Della Sala , A. Di Carlo , Th. Frauenheim

Absorption spectra of closed-shell Na_2, Na_3+, Na_4, Na_5+, Na_6, Na_7+, and Na_8 clusters are calculated using a recently implemented conserving linear response method. In the framework of a quasiparticle approach, we determine…

Materials Science · Physics 2015-05-14 George Pal , Georgios Lefkidis , Hans Christian Schneider , Wolfgang Huebner

We present results for the electronic structure of plutonium by using a recently developed quasiparticle self-consistent $GW$ method (\qsgw). We consider a paramagnetic solution without spin-orbit interaction as a function of volume for the…

Strongly Correlated Electrons · Physics 2009-07-23 A. N. Chantis , R. C. Albers , A. Svane , N. E. Christensen

We present theoretical calculations of quasiparticle energies in closed-shell molecules using the GW method. We compare three different approaches: a full-frequency $G_0W_0$ (FF-$G_0W_0$) method with density functional theory (DFT-PBE) used…

Materials Science · Physics 2015-06-22 Johannes Lischner , Sahar Sharifzadeh , Jack Deslippe , Jeffrey B. Neaton , Steven G. Louie

We apply the renormalized singles with correlation (RSc) Green's function in the $GW$ approximation to calculate accurate quasiparticle (QP) energies and orbitals. The RSc Green's function includes all orders of singles contributions from…

Chemical Physics · Physics 2022-10-19 Jiachen Li , Weitao Yang

A stochastic cumulant GW method is presented, allowing us to map the evolution of photoemission spectra, quasiparticle energies, lifetimes and emergence of collective excitations from molecules to bulk-like systems with up to thousands of…

Mesoscale and Nanoscale Physics · Physics 2018-03-21 Vojtech Vlcek , Eran Rabani , Daniel Neuhauser

Quasi-elastic responses in nuclear matter and in $^{12}$C and $^{40}$Ca nuclei are calculated in ring approximation to investigate the finite size effects on the electromagnetic quasi-elastic responses. A method to simulate these effects in…

Nuclear Theory · Physics 2008-11-26 E. Bauer , G. Co'

Using quasiparticle self-consistent $GW$ calculations, we re-examined the electronic structure of Sr$_2$RuO$_4$ and SrRuO$_3$. Our calculations show that the correlation effects beyond the conventional LDA (local density approximation) and…

Strongly Correlated Electrons · Physics 2016-02-16 Hyeonsang Ryee , Seung Woo Jang , Hiori Kino , Takao Kotani , Myung Joon Han

The GW approach produces highly accurate quasiparticle energies, but its application to large systems is computationally challenging, which can be largely attributed to the difficulty in computing the inverse dielectric matrix. To address…

Materials Science · Physics 2023-07-26 Mario G. Zauchner , Andrew Horsfield , Johannes Lischner

We present quasiparticle (QP) energies from fully self-consistent $GW$ (sc$GW$) calculations for a set of prototypical semiconductors and insulators within the framework of the projector-augmented wave methodology. To obtain converged…

Materials Science · Physics 2018-10-31 Manuel Grumet , Peitao Liu , Merzuk Kaltak , Jiří Klimeš , Georg Kresse

We explore the ability of the recently established quasilocal density functional theory for describing the isoscalar giant monopole resonance. Within this theory we use the scaling approach and perform constrained calculations for obtaining…

Nuclear Theory · Physics 2009-11-10 V. B. Soubbotin , V. I. Tselyaev , X. Vinas

We have developed a new type of self-consistent scheme within the $GW$ approximation, which we call quasiparticle self-consistent $GW$ (QS$GW$). We have shown that QS$GW$ rather well describes energy bands for a wide-range of materials,…

Materials Science · Physics 2007-10-05 Takao Kotani , Mark van Schilfgaarde , Sergey V. Faleev

We introduce an alternative route to quasiparticle self-consistent $GW$ calculations ($\mathrm{qs}GW$) on the basis of a Joint Approximate Diagonalization of the one-body $GW$ Green's functions $G(\varepsilon_n^{QP})$ taken at the input…

Materials Science · Physics 2024-12-05 Ivan Duchemin , Xavier Blase

We investigate two examples of node-based cluster summation rules that have been proposed for the quasicontinuum method: a force-based approach (Knap & Ortiz, J. Mech. Phys. Solids 49, 2001), and an energy-based approach which is a…

Numerical Analysis · Mathematics 2010-07-19 Mitchell Luskin , Christoph Ortner

Although the GW approximation is recognized as one of the most accurate theories for predicting materials excited states properties, scaling up conventional GW calculations for large systems remains a major challenge. We present a powerful…

Computational Physics · Physics 2018-03-28 Weiwei Gao , Weiyi Xia , Xiang Gao , Peihong Zhang

In past decades the scientific community has been looking for a reliable first-principles method to predict the electronic structure of solids with high accuracy. Here we present an approach which we call the quasiparticle self-consistent…

Materials Science · Physics 2009-11-11 M. van Schilfgaarde , T. Kotani , S. Faleev

Light clusters (mass number $A \leq 4$) in nuclear matter at subsaturation densities are described using a quantum statistical approach. In addition to self-energy and Pauli-blocking, effects of continuum correlations are taken into account…

Nuclear Theory · Physics 2015-11-18 G. Röpke

We investigate the convergence of quasi-particle energies for periodic systems to the thermodynamic limit using increasingly large simulation cells corresponding to increasingly dense integration meshes in reciprocal space. The…

We present an approach to calculate the electronic structure for a range of materials using the quasiparticle self-consistent GW method with vertex corrections included in the screened Coulomb interaction W. This is achieved by solving the…

Materials Science · Physics 2023-10-10 Brian Cunningham , Myrta Gruening , Dimitar Pashov , Mark van Schilfgaarde

Quasiparticle calculations are performed to investigate the electronic band structures of various polymorphs of Hf and Zr oxides. The corrections with respect to density-functional-theory results are found to depend only weakly on the…

Materials Science · Physics 2015-05-14 Myrta Grüning , Riad Shaltaf , Gian-Marco Rignanese
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