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The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…

Atomic Physics · Physics 2008-02-27 J. Mauritsson , P. Johnsson , E. Gustafsson , M. Swoboda , T. Ruchon , A. LHuillier , K. J. Schafer

Attosecond observations of coherent electron dynamics in molecules and nanostructures can be achieved by combining conventional scanning tunneling microscopy (STM) with ultrashort femtosecond laser pulses. While experimental studies in the…

Quantum Physics · Physics 2024-10-01 Boyang Ma , Michael Krüger

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

We study theoretically the photoabsorption spectra of an attosecond XUV pulse by a laserdressed atomic system. A weak XUV excites an autoionizing state which is strongly coupled to another autoionizing state by a laser. The theory was…

Atomic Physics · Physics 2012-05-23 Wei-Chun Chu , C. D. Lin

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

Atomic Physics · Physics 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

Attosecond dynamics of electron reflection from a thin film is studied based on a one-dimensional jellium model. Following the Eisenbud-Wigner-Smith concept, the reflection time delay $\Delta\tau_{\rm R}$ is calculated as the energy…

Materials Science · Physics 2025-06-10 R. O. Kuzian , E. E. Krasovskii

Measuring the delay for an electron to emerge from different states is one of the major achievements of attosecond science. This delay can have two origins - the electron wave packet is reshaped during departure by the electrostatic field…

Atomic Physics · Physics 2020-10-14 Graham G. Brown , Dong Hyuk Ko , Chunmei Zhang , P. B. Corkum

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

Atomic Physics · Physics 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity,…

Atomic Physics · Physics 2016-03-09 Chen-Ting Liao , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde , Arvinder Sandhu

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Quasi-free field-driven electron trajectories are a key element of strong-field dynamics. Upon recollision with the parent ion, the energy transferred from the field to the electron may be released as attosecond duration XUV emission in the…

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

Atomic Physics · Physics 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost

We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…

Optics · Physics 2017-11-22 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…

Chemical Physics · Physics 2013-04-26 P. A. Carpeggiani , P. Tzallas , A. Palacios , D. Gray , F. Martín , D. Charalambidis

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…