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Related papers: The properties of fully flexible Lennard-Jones cha…

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We use Monte Carlo simulations to study polymer melts consisting of fully flexible and moderately stiff chains in the bond fluctuation model at a volume fraction $0.5$. In order to reduce the local density fluctuations, we test a…

Soft Condensed Matter · Physics 2015-06-24 Hsiao-Ping Hsu

Self-avoiding polymers in strictly two-dimensional ($d=2$) melts are investigated by means of molecular dynamics simulation of a standard bead-spring model with chain lengths ranging up to N=2048. % The chains adopt compact configurations…

Soft Condensed Matter · Physics 2015-05-18 H. Meyer , J. P. Wittmer , T. Kreer , A. Johner , J. Baschnagel

We have studied the thermodynamics of isolated homopolymer chains of varying stiffness using a lattice model. A complex phase behaviour is found; phases include chain-folded `crystalline' structures, the disordered globule and the coil. It…

Soft Condensed Matter · Physics 2008-02-03 Jonathan Doye , Richard Sear , Daan Frenkel

We investigate the crystallization of a single, flexible homopolymer chain using transition path sampling (TPS). The chain consists of N identical spherical monomers evolved according to Langevin dynamics. While neighboring monomers are…

Soft Condensed Matter · Physics 2016-08-17 Christian Leitold , Christoph Dellago

We introduce the concept of tetris chains, which are linear arrays of 4-site molecules that differ by their intermolecular hopping geometry. We investigate the fermionic symmetry-protected topological Haldane phase in these systems using…

Strongly Correlated Electrons · Physics 2025-02-17 Anas Abdelwahab , Christoph Karrasch , Roman Rausch

X-shaped liquid crystalline molecules (XLCMs) are obtained by tethering two flexible end A-blocks and two flexible side B-blocks to a rigid backbone (R). A rich array of ordered structures can be formed from XLCMs, driven by the competition…

Soft Condensed Matter · Physics 2024-10-25 Dan Wei , Zhijuan He , Yunqing Huang , An-Chang Shi , Kai Jiang

We study a generic model of self-assembling chains which can branch and form networks with branching points (junctions) of arbitrary functionality. The physical realizations include physical gels, wormlike micells, dipolar fluids and…

Soft Condensed Matter · Physics 2009-11-07 A. G. Zilman , S. A. Safran

In this paper, we present a theory to efficiently deal with mechanical properties of heterogeneous polymer chain in free space and the central problem is to evaluate the diffusion equation and orientation-orientation correlation function,…

Biological Physics · Physics 2019-11-05 Ming Li , Jizeng Wang

Recently the supercooled Wahnstrom binary Lennard-Jones mixture was partially crystallized into ${\rm MgZn_2}$ phase crystals in lengthy Molecular Dynamics simulations. We present Molecular Dynamics simulations of a modified Kob-Andersen…

Soft Condensed Matter · Physics 2012-10-01 Søren Toxvaerd , Ulf R. Pedersen , Thomas B. Schrøder , Jeppe C. Dyre

Synthetic copolymers and biopolymers, such as polypeptides and double-stranded DNA, often exhibit strong variations in bending stiffness along their contour, which can significantly impact conformational behavior at larger scales. To…

Soft Condensed Matter · Physics 2025-11-04 Yannick Witzky , Friederike Schmid , Arash Nikoubashman

Herein, we study the extended Jaynes-Cummings-Hubbard model mainly by the large-scale worm quantum Monte-Carlo method to check whether or not a light supersolid phase exists in various geometries, such as the one-dimensional chain, square…

Statistical Mechanics · Physics 2021-05-12 Huanhuan Wei , Jie Zhang , Sebastian Greschner , Tony C Scott , Wanzhou Zhang

Analytical relations for the mechanical response of single polymer chains are valuable for modeling purposes, on both the molecular and the continuum scale. These relations can be obtained using statistical thermodynamics and an idealized…

Statistical Mechanics · Physics 2023-10-02 Michael R. Buche , Meredith N. Silberstein , Scott J. Grutzik

Polymer chains immersed in different solvent molecules exhibit diverse properties due to multiple spatiotemporal scales and complex interactions. Using molecular dynamics simulations, we study the conformational and static properties of…

Soft Condensed Matter · Physics 2024-07-08 Hong-Yao Li , Bokai Zhang , Zhi-Yong Wang

In this work we extend Wertheim's thermodynamic perturbation theory (TPT) to binary mixtures (species A and species B) of patchy colloids where each species has a single patch which can bond a maximum of twice (divalent). Colloids are…

Soft Condensed Matter · Physics 2014-08-16 B. D. Marshall , W. G. Chapman

The zig-zag Nitrogen (N) chain similar to the Ch-N structure has long been considered a potential high energy density structure. However, all previously predicted zig-zag N chain structures similar to Ch-N exhibit imaginary frequencies in…

Materials Science · Physics 2025-02-28 Chengfeng zhang , Guo Chen , Yanfeng Zhang , Jie Zhang , Xianlong Wang

A simple Lennard-Jones fluid confined in a slit nanopore with hard walls is studied on the basis of a multilayer structured model. Each layer is homogeneous and parallel to the walls of the pore. The Helmholtz energy of this system is…

Mesoscale and Nanoscale Physics · Physics 2010-03-17 G. J. Zarragoicoechea , A. G. Meyra , V. A. Kuz

In a recent article, Wang et al (Phys. Chem. Chem. Phys., 22, 10624 (2020)) introduced a new class of interparticle potential for molecular simulations. The potential is defined by a single range parameter, eliminating the need to decide…

Statistical Mechanics · Physics 2023-11-08 Olivia S. Moro , Vincent Ballenegger , Tom L. Underwood , Nigel B. Wilding

Investigating thermodynamic properties of liquid-solid transitions of flexible homopolymers with elastic bonds by means of multicanonical Monte Carlo simulations, we find crystalline conformations that resemble ground-state structures of…

Soft Condensed Matter · Physics 2010-02-11 Stefan Schnabel , Thomas Vogel , Michael Bachmann , Wolfhard Janke

The dynamical stability of three-dimensional (3D) Lennard-Jones (LJ) crystals has been studied for many years. The face-centered-cubic and hexagonal close packed structures are dynamically stable, while the body-centered cubic structure is…

Mesoscale and Nanoscale Physics · Physics 2021-02-10 Shota Ono , Tasuku Ito

We investigate the phase ordering (pattern formation) of systems of two-dimensional core-shell particles using Monte-Carlo (MC) computer simulations and classical density functional theory (DFT). The particles interact via a pair potential…

Soft Condensed Matter · Physics 2024-10-01 Michael Wassermair , Gerhard Kahl , Roland Roth , Andrew J. Archer