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We show that one may view the self and the distinct part of the van Hove dynamic correlation function of a simple fluid as the one-body density distributions of a binary mixture that evolve in time according to dynamical density functional…

Soft Condensed Matter · Physics 2011-11-09 Andrew J. Archer , Paul Hopkins , Matthias Schmidt

We study the relaxation dynamics of a binary Lennard-Jones liquid in the presence of an amorphous wall generated from equilibrium particle configurations. In qualitative agreement with the results presented in Nature Phys. {\bf 8}, 164…

Statistical Mechanics · Physics 2014-06-16 Glen M Hocky , Ludovic Berthier , Walter Kob , David R. Reichman

Starting with a formally exact diagrammatic kinetic theory for the equilibrium correlation functions of particle density and current fluctuations for a monatomic liquid, we develop a theory for high density liquids whose interatomic…

Statistical Mechanics · Physics 2015-06-17 Kevin R. Pilkiewicz , Hans C. Andersen

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

Statistical Mechanics · Physics 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

By means of the isoconfigurational method we calculate the change in the propensity for motion that the structure of a glass-forming system experiences during its relaxation dynamics. The relaxation of such a system has been demonstrated to…

Soft Condensed Matter · Physics 2008-10-09 J. A. Rodriguez Fris , L. M. Alarcón , G. A. Appignanesi

Elucidating the nature of the glass transition has been the holy grail of condensed matter physics and statistical mechanics for several decades. A phenomenological aspect that makes glass formation a conceptually formidable problem is that…

Soft Condensed Matter · Physics 2016-08-11 Shreyas Gokhale , K. Hima Nagamanasa , A. K. Sood , Rajesh Ganapathy

Despite the use of glasses for thousands of years, the nature of the glass transition is still mysterious. On approaching the glass transition, the growth of dynamic heterogeneity has long been thought to play a key role in explaining the…

Soft Condensed Matter · Physics 2018-03-23 Lijin Wang , Ning Xu , W. H. Wang , Pengfei Guan

We analyze one thousand independent equilibrium trajectories of a system of 155 Lennard Jones particles to separate in a model-free approach the role of temperature and the role of the explored potential energy landscape basin depth in the…

Disordered Systems and Neural Networks · Physics 2009-11-11 Emilia La Nave , Srikanth Sastry , Francesco Sciortino

The dynamic structure factor, vorticity and entropy density dynamic correlation functions are measured for Stochastic Rotation Dynamics (SRD), a particle based algorithm for fluctuating fluids. This allows us to obtain unbiased values for…

Soft Condensed Matter · Physics 2009-11-11 Erkan Tuzel , Thomas Ihle , Daniel M. Kroll

In a recent paper [S. Mandal et al., Phys. Rev. E 88, 022129 (2013)] the nature of spatial correlations of plasticity in hard sphere glasses was addressed both via computer simulations and in experiments. It was found that the…

We use a recently proposed method [Berthier L.; Biroli G.; Bouchaud J.P.; Cipelletti L.; El Masri D.; L'Hote D.; Ladieu F.; Pierno M. Science 2005, 310, 1797.] to obtain an approximation to the 4-point dynamic correlation function from…

Soft Condensed Matter · Physics 2009-08-27 D. Fragiadakis , R. Casalini , C. M. Roland

Crystallization kinetics has features that are universal and independent of the type of crystallized system. The possibility of using scaling relations to describe the temperature dependences of the surface self-diffusion coefficient $D_s$,…

Materials Science · Physics 2020-01-07 Anatolii V. Mokshin , Bulat N. Galimzyanov , Dinar T. Yarullin

We simulate binary soft disk systems in two dimensions, and investigate how the dynamics slow as the area fraction is increased toward the glass transition. The "fragility" quantifies how sensitively the relaxation time scale depends on the…

Soft Condensed Matter · Physics 2010-10-12 Rei Kurita , Eric R. Weeks

Correlation of interacting particles is studied in their dynamics and localization in ideal and disordered lattice systems with the help of numerical tools. Both 1D and 2D systems are considered. In 1D lattices with long-range hopping,…

Quantum Gases · Physics 2018-09-27 Tirthaprasad Chattaraj

The study of the low temperature phase of spin glass models by means of Monte Carlo simulations is a challenging task, because of the very slow dynamics and the severe finite size effects they show. By exploiting at the best the…

Disordered Systems and Neural Networks · Physics 2014-04-02 Lucas Nicolao , Giorgio Parisi , Federico Ricci-Tersenghi

We present experimental confirmation of dynamic facilitation in monodisperse and bidisperse colloidal suspensions near the glass transition volume fraction. Correlations in particle dynamics are seen to exist not only in space (clusters and…

Soft Condensed Matter · Physics 2014-06-24 Scott V. Franklin , Eric R. Weeks

The super-Arrhenius dynamic slowdown in fragile supercooled liquids remains one of the central unresolved questions in condensed matter physics. In this study, we analyze particle jump dynamics in a prototypical fragile glass-forming…

Soft Condensed Matter · Physics 2026-05-27 Zhiye Tang , Shubham Kumar , Shinji Saito

Previous studies have suggested a conundrum in the relaxation dynamics of polydisperse supercooled liquids. It has been shown that in two dimensions, the relative relaxation times of particles of different sizes become more similar as the…

Soft Condensed Matter · Physics 2025-03-06 Ilian Pihlajamaa , Lotte van Gessel , Corentin Laudicina , Luc van Burik , Liesbeth Janssen

We present molecular dynamics results for a two component, two-dimensional Lennard-Jones supercooled liquid near the glass transition. We find that the supercooled liquid is spatially heterogeneous and that there are long-lived clusters…

Disordered Systems and Neural Networks · Physics 2009-10-31 Gregory Johnson , Andrew I. Melcuk , Harvey Gould , W. Klein , Raymond D. Mountain

We perform molecular dynamics simulations of a model glass-forming liquid to measure the size of kinetic heterogeneities, using a dynamic susceptibility $\chi_{\rm ss}(a, t)$ that quantifies the number of particles whose dynamics are…

Soft Condensed Matter · Physics 2014-04-04 T. K. Haxton , A. J. Liu