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The crystal-fields causing $|J>$ electron states splittings of the same second moment $\sigma^{2}$ can produce different total splittings $\Delta E$ magnitudes. Based on the numerical data on crystal-field splittings for the representative…

Materials Science · Physics 2015-05-13 Jacek Mulak , Maciej Mulak

The second moment of the sublevels within the initial state | \alpha SLJ > which constitutes a natural and adequate measure of the crystal-field (CF) effect can be redefined as sigma^{2}=1/(2J+1)\sum_{k} S_{k}^{2} A_{k}^{2}, where…

Chemical Physics · Physics 2015-05-13 Jacek Mulak , Maciej Mulak

It has been shown that to calculate the parameters of the electrostatic field of the ion crystal lattice it sufficient to take into account ions located at a distance of 1-2 lattice spacings. More distant ions make insignificant…

General Physics · Physics 2010-01-26 Alexander Ivanchin

Any electron eigenstate |\Psi>of the paramagnetic ion open-shell is characterized by the three independent multipole asphericities A_{k}=<\Psi || C^(k)}||\Psi> for k=2,4 and 6 related to the second moments of the relevant crystal-field…

Chemical Physics · Physics 2015-05-28 Jacek Mulak , Maciej Mulak

The physically correct parametrization of the energy levels of transition ions in crystals in terms of crystal-field (CF) Hamiltonians ${\cal H}_{\rm CF}=\sum_{k}\sum_{q}B_{kq}C_{q}^{(k)}$ has to be based on the CF parameters $B_{kq}$ that…

Materials Science · Physics 2023-07-19 Jacek Mulak , Maciej Mulak

We report the computation of the Standard Hamiltonian of a coupled electron-phonon system by accurately computing the electron-phonon interaction (EPI) contribution to the total energy. This gives the most accurate ab initio total energy…

Materials Science · Physics 2025-08-25 Shilpa Paul , M. P. Gururajan , Amrita Bhattacharya , T. R. S. Prasanna

In the framework of the LDA+U approximation we propose the direct way of calculation of crystal-field excitation energy and apply it to La and Y titanates. The method developed can be useful for comparison with the results of spectroscopic…

Strongly Correlated Electrons · Physics 2007-05-23 S. V. Streltsov , A. S. Mylnikova , A. O. Shorikov , Z. V. Pchelkina , D. I. Khomskii , V. I. Anisimov

We study the exchange coupling in small Wigner crystals confined to one-dimensional space. In particular we concentrate on the simplest nontrivial case of two electrons in a box potential and calculate analytically the energy splitting…

Strongly Correlated Electrons · Physics 2025-12-30 Daniele Lagasco , Zoran Ristivojevic

We consider the asymmetric six--vertex model, {\it i.e.} the symmetric six--vertex model in an external field with both horizontal and vertical components, and the relevant asymmetric $XXZ$ chain. The model is widely used to describe the…

Condensed Matter · Physics 2011-07-19 Giuseppe Albertini , Silvio Renato Dahmen , Birgit Wehefritz

The energy splitings for $J = 1$, $F=3/2$, $|M_F|=3/2$ hyperfine levels of the $^3\Delta_1$ electronic state of $^{180}$Hf$^{19}$F$^+$ ion are calculated as functions of the external variable electric and magnetic fields within two…

Atomic Physics · Physics 2018-05-16 A. N. Petrov

In a quantum system, different energy eigenstates have different properties or features, allowing us define a classifier to divide them into different groups. We find that the ratio of each type of energy eigenstates in an energy shell…

Quantum Physics · Physics 2023-03-29 Zhelun Zhang , Zhenduo Wang , Biao Wu

Strong electric fields can be used to align molecules. However, a non-polar molecule such as H$_2$ has no preference for its orientation. There are thus two equivalent configurations with equal energy separated by a potential-energy…

Chemical Physics · Physics 2025-12-02 J. Amira Geuther , Marit R. Fiechter , Jeremy O. Richardson

The self-energy corrections to the hyperfine splitting is evaluated for higher excited states in hydrogenlike ions, using an expansion in the binding parameter Zalpha, where Z is the nuclear charge number, and alpha is the fine-structure…

Atomic Physics · Physics 2012-06-29 B. J. Wundt , U. D. Jentschura

The impacts of both exchange interaction and electron correlation, as well as their combined impact, on electron elastic scattering off a semifilled shell Mn(...$3d^{5}$$4s^{2}$, $^{6}S$) atom are theoretically studied in the electron…

Atomic Physics · Physics 2013-08-15 V. K. Dolmatov , M. Ya. Amusia , L. V. Chernysheva

We analyse the finite-size corrections to the free energy of crystals with a fixed center of mass. When we explicitly correct for the leading ($\ln N/N$) corrections, the remaining free energy is found to depend linearly on 1/N.…

Statistical Mechanics · Physics 2009-10-31 J. M. Polson , E. Trizac , S. Pronk , D. Frenkel

We investigate the hyperfine energy levels and Zeeman splittings for homonuclear alkali-metal dimers in low-lying rotational and vibrational states, which are important for experiments designed to produce quantum gases of deeply bound…

Atomic Physics · Physics 2010-03-09 J. Aldegunde , Jeremy M. Hutson

An anomalous energy splitting of spin triplet states at zero magnetic field has recently been measured in germanium quantum dots. This zero-field splitting could crucially alter the coupling between tunnel-coupled quantum dots, the basic…

Mesoscale and Nanoscale Physics · Physics 2022-09-21 Bence Hetényi , Stefano Bosco , Daniel Loss

We consider a system made up of N electrons interacting with a neutralizing positive background within a cubic box of volume V. After dividing the box into N (or N/2) cubic cells for the polarized (unpolarized) case, we average the creation…

Strongly Correlated Electrons · Physics 2007-12-11 Salvino Ciccariello

We report the results of a numerical investigation, performed in the frame of dynamical systems' theory, for a realistic model of a ionic crystal for which, due to the presence of long--range Coulomb interactions, the Gibbs distribution is…

Statistical Mechanics · Physics 2020-08-04 Andrea Carati , Luigi Galgani , Fabrizio Gangemi , Roberto Gangemi

The authors investigate the magnetic field dependence of the energy splitting between low-lying valley states for electrons in a Si/SiGe quantum well tilted with respect to the crystallographic axis. The presence of atomic steps at the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Mark Friesen , M. A. Eriksson , S. N. Coppersmith
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