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The increasing demand for sustainable energy solutions necessitates advancements in hydrogen storage technologies. This study investigates the hydrogen adsorption characteristics of graphene and a (8,0) carbon nanotube (CNT) decorated with…

Materials Science · Physics 2025-09-16 Thomas Leiner , David Holec

Hydration properties of graphene oxide (GO) are essential for most of its potential applications. In this work, we employ atomistic molecular dynamics simulations to investigate seven GO compositions with different levels of oxygenation.…

Materials Science · Physics 2018-02-14 Antenor Neto , Vitaly V. Chaban , Eudes E. Fileti

Using the pseudopotential density functional method, we find that a Be atom on a nanostructure with H2 molecules forms a Be-dihydrogen complex through the hybridization of the Be s or p orbits with the H2 sigma orbits and the binding energy…

Materials Science · Physics 2015-05-18 Hoonkyung Lee , Bing Huang , Wenhui Duan , Jisoon Ihm

First-principles DFT calculations on the hydrides Ca2NiH6, Sr2NiH6, and Ba2NiH6 reveal key thermodynamic properties. These compounds exhibit increasing entropy and heat capacity with temperature, and are thermodynamically stable at elevated…

Materials Science · Physics 2026-02-11 K. Aafi , Z. El Fatouaki , A. Jabar , A. Tahiri , M. Idiri

We have studied solid hydrogen up to pressures of 300 GPa and temperatures of 350 K using density functional theory methods and have found "mixed structures" that are more stable than those predicted earlier. Mixed structures consist of…

Materials Science · Physics 2012-06-20 Chris J. Pickard , Miguel Martinez-Canales , Richard J. Needs

Hydrogen-based fuel cells are promising solutions for the efficient and clean delivery of electricity. Since hydrogen is an energy carrier, a key step for the development of a reliable hydrogen-based technology requires solving the issue of…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 Valentina Tozzini , Vittorio Pellegrini

The absorption energy of atomic hydrogen at rotated graphene bilayers is studied using ab initio methods based on the density functional theory including van der Waals interactions. We find that, due to the surface corrugation induced by…

Mesoscale and Nanoscale Physics · Physics 2017-10-06 Ivan Brihuega , Felix Yndurain

Graphynes are 2D porous structures deriving from graphene featuring triangular and regularly distributed subnanometer pores, which may be exploited to host small gaseous species. First principles adsorption energies of molecular hydrogen…

Chemical Physics · Physics 2015-10-06 Massimiliano Bartolomei , Estela Carmona-Novillo , Giacomo Giorgi

We study a versatile structurally favorable periodic $sp^2$-bonded carbon atomic planar sheet with $C_{4v}$ symmetry by means of the first-principles calculations. This carbon allotrope is composed of carbon octagons and squares with two…

Materials Science · Physics 2012-11-12 Xian-Lei Sheng , Hui-Juan Cui , Fei Ye , Qing-Bo Yan , Qing-Rong Zheng , Gang Su

We report on hydrogen adsorption and desorption on titanium-covered graphene in order to test theoretical proposals to use of graphene functionalized with metal atoms for hydrogen storage. At room temperature titanium islands grow with an…

Chemical Physics · Physics 2013-12-06 Torge Mashoff , Makoto Takamura , Shinichi Tanabe , Hiroki Hibino , Fabio Beltram , Stefan Heun

This paper focuses on the performance of the storage of Li and the stability of the hybrid structure of different lattice planes of the silicon clusters and graphene by the first-principle theory. In this paper, we calculate the binding…

Mesoscale and Nanoscale Physics · Physics 2012-03-01 Wu Jiangbin , Qian Yao , Guo Xiaojie , Cui Xianhui , Miao Ling , Jiang Jianjun

In this work, we studied the hydrogen adsorption-desorption properties and storage capacities of Ti functionalized [2,2,2]paracyclophane (PCP222) using density functional theory and molecular dynamic simulation. The Ti atom was bonded…

Chemical Physics · Physics 2023-01-11 Rakesh K. Sahoo , Sridhar Sahu

The thermodynamic, kinetic and magnetic properties of the hydrogen monomer on doped graphene layers were studied by ab initio simulations. Electron doping was found to heighten the diffusion potential barrier, while hole doping lowers it.…

Materials Science · Physics 2011-08-17 Liang Feng Huang , Mei Yan Ni , Guo Ren Zhang , Wang Huai Zhou , Yong Gang Li , Xiao Hong Zheng , Zhi Zeng

Gas hydrates are systems of prime importance. In particular, hydrogen hydrates are potential materials of icy satellites and comets, and may be used for hydrogen storage. We explore the H2O-H2 system at pressures in the range 0-100 GPa with…

Materials Science · Physics 2014-04-01 Guang-Rui Qian , Andriy O. Lyakhov , Qiang Zhu , Artem R. Oganov , Xiao Dong

Density-functional theory based global geometry optimization is used to scrutinize the possibility of using endohedrally-doped hydrogenated Si clusters as building blocks for constructing highly magnetic materials. In contrast to the known…

Materials Science · Physics 2013-07-26 Dennis Palagin , Karsten Reuter

An ideal material for on-board hydrogen storage must release hydrogen at practical temperature and pressure and also regenerate efficiently under similarly gentle conditions. Therefore, thermodynamically, the hydride material must lie…

Materials Science · Physics 2015-05-18 T. A. Abtew , Bi-ching Shih , Pratibha Dev , Vincent H. Crespi , Peihong Zhang

Hydrogen is deemed as an attractive energy carrier alternative to fossil fuels, and it is required to store for many applications. Physisorption is one of the promising ways to store H$_2$ for its practical applications. Covalent Organic…

Materials Science · Physics 2021-11-05 Nilima Sinha , Srimanta Pakhira

We demonstrate in this paper that high pressure can promote the reactions between the ionic compounds and H2 molecules and form thermodynamically stable hybrid compounds. Using crystal structure search method based on first principles…

Materials Science · Physics 2019-07-29 Feng Peng , Yanming Ma , Maosheng Miao

Finding a suitable material for hydrogen storage at ambient atmospheric conditions is challenging for material scientists and chemists. In this work, using a first principles based cluster expansion approach, the hydrogen storage capacity…

Materials Science · Physics 2023-02-22 Pritam Das , Krishnamohan Thekkepat , Young-Su Lee , Seung-Cheol Lee , Satadeep Bhattacharjee

Two-dimensional (2D) materials as electrodes is believed to be the trend for future Li-ion and Na-ion batteries technologies. Here, by using first-principles methods, we predict that the recently reported borophene (2D born sheet) can serve…

Mesoscale and Nanoscale Physics · Physics 2016-10-19 Xiaoming Zhang , Junping Hu , Yingchun Cheng , Hui Ying Yang , Yugui Yao , Shengyuan A. Yang
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