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The capacity of carbon atomic chains with different terminations for hydrogen storage is studied using first-principles density functional theory calculations. Unlike the physisorption of H2 on the H-terminated chain, we show that two Li…

Mesoscale and Nanoscale Physics · Physics 2010-07-23 Chun-Sheng Liu , Hui An , Zhi Zeng

Density functional calculations of electronic structure, total energy, structural distortions, and magnetism for hydrogenated single-layer, bilayer, and multi-layer graphene are performed. It is found that hydrogen-induced magnetism can…

Materials Science · Physics 2008-01-24 D. W. Boukhvalov , M. I. Katsnelson , A. I. Lichtenstein

Structure, stability and reactivity of clathrate hydrates with or without hydrogen encapsulation are studied using standard density functional calculations. Conceptual density functional theory based reactivity descriptors and the…

Atomic and Molecular Clusters · Physics 2016-09-28 Pratim Kumar Chattaraj , Sateesh Bandaru , Sukanta Mondal

Efficient hydrogen storage in solid-state materials is essential for next-generation energy systems, yet achieving a high gravimetric capacity with optimal adsorption characteristics remains a critical challenge. Although Li-decorated…

Materials Science · Physics 2025-06-04 Jose A. S. Laranjeira , Warda Elaggoune , Nicolas F. Martins , Xihao Chen , Julio R. Sambrano

Strain effects on the stability, electronic structure, and hydrogen storage capacity of lithium-doped graphane (CHLi) have been investigated by stateof-the art first principle density functional theory (DFT). Molecular dynamics MD)…

Materials Science · Physics 2015-06-05 Tanveer Hussain , Abir De Sarkar , Rajeev Ahuja

Li and Na attachment to free tetracyanoethylene (TCNE) molecules and TCNE adsorbed on doped graphene is studied using density functional theory. While TCNE is adsorbed only weakly on ideal graphene, we identified a configuration in which…

Materials Science · Physics 2016-02-05 Yingqian Chen , Sergei Manzhos

The increase in threats from global warming due to the consumption of fossil fuels requires our planet to adopt new strategies to harness the inexhaustible sources of energy. Hydrogen is an energy carrier which holds tremendous promise as a…

Materials Science · Physics 2011-06-23 N. S. Venkataramanan , A. Suvitha , H. Mizuseki , Y. Kawazoe

In this work, we have studied the hydrogen adsorption-desorption properties and storage capacities of Li functionalized [2,2,2]paracyclophane (PCP222) using dispersion-corrected density functional theory and molecular dynamic simulation.…

Chemical Physics · Physics 2023-01-11 Rakesh K. Sahoo , Sridhar Sahu

We have investigated the hydrogen storage capabilities of scandium decorated holey graphyne, a recently synthesized carbon allotrope, by applying density functional theory and molecular dynamics simulations. We have observed that one unit…

Materials Science · Physics 2022-02-11 Vikram Mahamiya , Alok Shukla , Nandini Garg , Brahmananda Chakraborty

Pristine graphene is not suitable for hydrogen storage at ambient conditions since it binds the hydrogen molecules only by van der Waals interactions. However, the adsorption energy of the hydrogen molecules can be improved by doping or…

Materials Science · Physics 2022-10-24 Vikram Mahamiya , Alok Shukla , Nandini Garg , Brahmananda Chakraborty

By employing the state-of-the-art density functional theory, we report the hydrogen storage capability of yttrium decorated C$_{24}$ fullerene. Single Y atom attached on C$_{24}$ fullerene can reversibly adsorb a maximum number of 6 H$_2$…

Materials Science · Physics 2022-02-11 Vikram Mahamiya , Alok Shukla , Brahmananda Chakraborty

The capacity of Ti-capped sp carbon atomic chains for use as hydrogen storage media is studied using first-principles density functional theory. The Ti atom is strongly attached at one end of the carbon chains via d-p hybridization, forming…

Materials Science · Physics 2017-03-15 Chun-Sheng Liu , Hui An , Zhi Zeng

This article presents the reversible hydrogen storage capacities of Li-decorated Si6C14 and Si8C12 using Density Functional Theory (DFT). The chemical stabilities of the designed Si6C14Li6 and Si8C12Li4 nanocages are investigated using…

Materials Science · Physics 2024-07-24 Ankita Jaiswal , Rakesh K. Sahoo , Sridhar Sahu

Borophosphene is investigated for hydrogen storage by density functional theory calculations through Li, Na and Ca decoration. Decoration enhances the binding energy from -0.047 eV/H2 to -0.20 -- -0.42 eV/H2. PDOS and Bader charge analysis…

Materials Science · Physics 2023-10-25 Sandip Haldar

Adsorption of hydrogen atoms on a single graphite sheet (graphene) has been investigated by first-principles electronic structure means, employing plane-wave based, periodic density functional theory. A reasonably large 5x5 surface unit…

Materials Science · Physics 2009-11-13 Simone Casolo , Ole Martin Lovvik , Rocco Martinazzo , Gian Franco Tantardini

The energy demands for the growing development of society need to be catered with alternative and green fuels like hydrogen energy for a lasting and sustainable culture. One essential component of the hydrogen economy is the efficiency of…

Materials Science · Physics 2023-03-07 Mukesh Singh , Alok Shukla , Brahmananda Chakraborty

Exceptionally high energy density by mass, natural abundance, widespread applications, and environmental friendliness make hydrogen (H2) a front-runner among clean energy options. However, the transition toward clean and renewable energy…

Materials Science · Physics 2024-07-25 Wael Othman , Wadha Al Falasi , Tanveer Hussain , Nacir Tit

We propose a multi-layer graphene-based device in which storage and release of atomic hydrogen is obtained by exploiting and controlling the corrugation of the layers. The proposal is based on density-functional simulations of hydrogen…

Mesoscale and Nanoscale Physics · Physics 2011-01-07 Valentina Tozzini , Vittorio Pellegrini

We have found that a beryllium (Be) atom on nanostructured materials with H2 molecules generates a Kubas-like dihydrogen complex [H. Lee et al. arXiv:1002.2247v1 (2010)]. Here, we investigate the feasibility of Be-decorated fullerenes for…

Materials Science · Physics 2015-05-18 Hoonkyung Lee , Bing Huang , Wenhui Duan , Jisoon Ihm

Using density functional theory we show that an applied electric field substantially improves the hydrogen storage properties of a BN sheet by polarizing the hydrogen molecules as well as the substrate. The adsorption energy of a single H2…

Materials Science · Physics 2016-12-28 J. Zhou , Q. Wang , Q. Sun , P. Jena , X. S. Chen