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Ab initio quantum chemistry calculations are performed for the mixed alkali triatomic system. Global minima of the ground and first excited doublet states of the trimer are found and Born-Oppenheimer potential energy surfaces of the Li atom…

Chemical Physics · Physics 2018-03-14 Patryk Jasik , Tymon Kilich , Jan Kozicki , Józef E. Sienkiewicz

An accurate long-range {\em ab initio} potential energy surface has been calculated for the ground state ${}^2A'$ lithium trimer in the frozen diatom approximation using all electron RCCSD(T). The {\em ab initio} energies are corrected for…

Chemical Physics · Physics 2015-05-28 Jason N. Byrd , John A. Montgomery, , H. Harvey Michels , Robin Côté

A potential energy surface for the lowest quartet electronic state of lithium trimer is developed and used to study spin-polarized Li + Li_2 collisions at ultralow kinetic energies. The potential energy surface allows barrierless atom…

Chemical Physics · Physics 2009-11-13 Marko T. Cvitas , Pavel Soldan , Jeremy M. Hutson , Pascal Honvault , Jean-Michel Launay

We investigate the intermolecular interactions between laser-cooled CaF and Ca, in their ground and excited electronic states, aiming to understand atom-exchange reaction pathways. Using state-of-the-art \textit{ab initio} quantum chemistry…

Atomic Physics · Physics 2025-10-28 Dibyendu Sardar , John L. Bohn

State-of-the-art ab initio techniques have been applied to compute the potential energy surface for the lithium atom interacting with the lithium hydride molecule in the Born-Oppenheimer approximation. The interaction potential was obtained…

Accurate \textit{ab initio} potential energy surfaces are essential to understand and predict collisional outcomes in ultracold molecular systems. In this study, we explore the intermolecular interactions between two laser-cooled CaF…

Atomic Physics · Physics 2025-11-12 Dibyendu Sardar , Marcin Gronowski , Michał Tomza , John L. Bohn

We report state-of-the-art ab initio calculations of the potential energy curve for the $a^3\Sigma_u^+$ state of the lithium dimer conducted to achieve spectroscopic accuracy ($<$1cm$^{-1}$) without any prior adjustment to fit the…

Chemical Physics · Physics 2021-01-27 Michał Lesiuk , Monika Musiał , Robert Moszynski

New ab initio potential energy surfaces for the doublet pi ground electronic state of the Ar-SH complex are presented, calculated at the RCCSD(T)/aug-cc-pV5Z level. Weakly bound rotation-vibration levels are calculated using coupled-channel…

Chemical Physics · Physics 2007-05-23 Richard J. Doyle , David M. Hirst , Jeremy M. Hutson

The global potential energy surfaces of the first six singlet electronic states of CO$_2$, 1---3$^1/!A'$ and 1---3$^1/!A"$ are constructed using high level ab initio calculations. In linear molecule, they correspond to…

Chemical Physics · Physics 2015-06-15 Sergy Yu. Grebenshchikov

The LiFr diatomic represents a promising candidate for indirect laser cooling that has not yet been investigated not theoretically or experimentally. The potential energy curves of the ground and low_lying excited states of the LiFr…

Atomic Physics · Physics 2023-12-29 Maksim Shundalau , Patrizia Lamberti

We perform a systematic investigation of the electronic properties of the $^2\Sigma^+$ ground state of Li-alkaline-earth dimers. These molecules are proposed as possible candidates for quantum simulation of lattice-spin models. We apply…

Quantum Physics · Physics 2015-05-30 Svetlana Kotochigova , Jacek Kłos , Alexander Petrov , Maria Linnik , Paul S. Julienne

A full six-dimensional Born-Oppenheimer singlet potential energy surface is constructed for the reaction CaF + CaF $\rightarrow$ CaF$_2$ + Ca using a multireference configuration interaction (MRCI) electronic structure calculation. The {\it…

Atomic Physics · Physics 2023-04-05 Dibyendu Sardar , Arthur Christianen , Hui Li , John L. Bohn

In this study, we investigate the structure of the polar alkali-Strontium diatomic molecules as possible candidates for the realization of samples of new species of ultracold polar molecules. Using a quantum chemistry approach based on…

Atomic and Molecular Clusters · Physics 2015-05-19 Romain Guérout , Mireille Aymar , Olivier Dulieu

The electronic structure of Ce2 is studied in a valence bond model with two 4f electrons localized at two cerium sites. It is shown that the low-lying energy spectrum of the simplest cerium chemical bond is determined by peculiarities of…

Materials Science · Physics 2015-05-28 A. V. Nikolaev

Potential energy surfaces of the hydrogen molecular ion H$_2^+$ in the Born-Oppenheimer approximation are computed by means of the Riccati-Pad\'e method (RPM). The convergence properties of the method are analyzed for different states. The…

Chemical Physics · Physics 2022-10-25 Francisco Marcelo Fernández , Javier Garcia

The helium trimer is studied using two- and three-body soft-core potentials. Realistic helium-helium potentials present an extremely strong short-range repulsion and support a single, very shallow, bound state. The description of systems…

Atomic and Molecular Clusters · Physics 2015-03-17 A. Kievsky , E. Garrido , C. Romero-Redondo , P. Barletta

A new implementation of stochastic many-body perturbation theory for periodic 2D systems is presented. The method is used to compute quasiparticle excitations in twisted bilayer phosphorene. Excitation energies are studied using stochastic…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 Jacob Brooks , Guorong Weng , Stephanie Taylor , Vojtech Vlcek

No lines have been observed for transitions between the doublet and quartet levels of B I. Consequently, energy levels based on observation for the latter are obtained through extrapolation of wavelengths along the iso-electronic sequence…

We employ two-photon spectroscopy to study the vibrational states of the triplet ground state potential ($a^3\Sigma^+$) of the $^{23}$Na$^{6}$Li molecule. Pairs of Na and Li atoms in an ultracold mixture are photoassociated into an excited…

We present the most accurate up-to-date theoretical values of the {2p_{1/2}}-{2s} and {2p_{3/2}}-{2s} transition energies and the ground-state hyperfine splitting in ${\rm Sc}^{18+}$. All two- and three-electron contributions to the energy…

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