Related papers: Tuning Magnetic Avalanches in Mn12-ac
In magnetic fields applied parallel to the anisotropy axis, the magnetization of Mn$_{12}$ has been measured in response to a field that is swept back and forth across the resonances corresponding to steps $N=4,5,...9$. The fraction of…
The magnetic instability at the front of the spin avalanche in a crystal of molecular magnets is considered. This phenomenon reveals similar features with the Darrieus-Landau instability, inherent to classical combustion flame fronts. The…
The spatial profile of the magnetization of Mn12 crystals in a swept magnetic field applied along the easy axis is determined from measurements of the local magnetic induction along the sample surface using an array of Hall sensors. We find…
The reversal of spins in a magnetic material as they relax toward equilibrium is accompanied by the release of Zeeman energy which can lead to accelerated spin relaxation and the formation of a well-defined self-sustained propagating…
The effect of thermal coupling on spin avalanches in Mn12-acetate has been probed using a single crystal assembly. Time-resolved, synchronized measurements of magnetization and temperature are reported. Unusually low avalanche trigger…
A comprehensive set of experiments on the effect of high-frequency surface acoustic waves, SAWs, in the spin relaxation in Mn12-acetate is presented. We have studied the quantum magnetic deflagration induced by SAWs under various…
The magnetization reversal in a single molecular magnet (SMM) weakly coupled to an electrode with spin-dependent splitting of chemical potentials (spin bias) is theoretically investigated by means of the rate equation. A microscopic…
In this work, we study the spin dynamics of Mn12-acetate molecules in the regime of thermally assisted tunneling. In particular, we describe the system in the presence of a strong transverse magnetic field. Similar to recent experiments,…
We report point by point measurements below the blocking temperature of the magnetic relaxation of Mn$_{12}$-acetate as a function of magnetic field applied along the easy axis of magnetization. Unexpectedly complex structure is observed…
The stability of a magnetic deflagration front in a collection of molecular magnets, such as Mn_12-acetate, is considered. It is demonstrated that stationary deflagration is unstable with respect to one-dimensional perturbations if the…
Decay of metastable states in molecular magnets (MM) leads to energy release that results in temperature increase that, in turn, positively affects the decay rate. This is the mechanism of recently discovered magnetic deflagration that is…
Theory of magnetic deflagration (avalanches) in crystals of molecular magnets has been developed. The phenomenon resembles the burning of a chemical substance, with the Zeeman energy playing the role of the chemical energy. Non-destructive…
We present a comprehensive theory of the magnetization relaxation in a Mn12-acetate crystal in the high-temperature regime (T>1 K), which is based on phonon-assisted spin tunneling induced by quartic magnetic anisotropy and weak transverse…
We present experimental results on resonant spin tunnelling in a single crystal of Mn$_{12}$-2Cl benzoate with different concentration of dislocations. The time evolution of the magnetisation follows the stretched exponential over a few…
A high resolution inelastic neutron scattering (INS) study of fully deuterated Mn$_{12}$-acetate provides the most accurate spin Hamiltonian parameters for this prototype single molecule magnet so far. The Mn$_{12}$-clusters deviate from…
Dipolar-controlled quantum deflagration going over into quantum detonation in the elongated Mn_12 Ac molecular magnet in a strong transverse field has been considered within the full 3d model. It is shown that within the dipolar window…
Current theories still fail to give a satisfactory explanation of the observed quantum phenomena in the relaxation of the magnetisation of the molecular cluster Mn12 acetate. In the very low temperature regime, Prokof'ev and Stamp recently…
We report experimental studies of crystals of Mn12 molecular magnetic clusters in pulsed magnetic fields with sweep rates up to 4x10^3 T/s. The steps in the magnetization curve are observed at fields that are shifted with respect to the…
We explore the electronic interactions between a thin gold film and a surface layer of the molecular magnet Mn_12-acetate. Magnetoresistance measurements of the gold allow characterization of the interactions by comparison with the…
We present a comprehensive derivation of the magnetization relaxation in a Mn12-acetate crystal based on thermally assisted spin tunneling induced by quartic anisotropy and weak transverse magnetic fields. The overall relaxation rate as…