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The nature of the tetragonal-to-orthorhombic structural transition at $T_s\approx90$ K in single crystalline FeSe is studied using shear-modulus, heat-capacity, magnetization and NMR measurements. The transition is shown to be accompanied…

Superconductivity · Physics 2015-06-22 A. E. Böhmer , T. Arai , F. Hardy , T. Hattori , T. Iye , T. Wolf , H. v. Löhneysen , K. Ishida , C. Meingast

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

Superconductivity · Physics 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

We use inelastic neutron scattering to study spin excitation anisotropy in mechanically detwinned Ba(Fe1-xCox)2As2 with x = 0.048 and 0.054. Both samples exhibit a tetragonal-to-orthorhombic structural transition at Ts, a collinear static…

Superconductivity · Physics 2020-01-08 Long Tian , Panpan Liu , Zhuang Xu , Yu Li , Zhilun Lu , H. C. Walker , U. Stuhr , Guotai Tan , Xingye Lu , Pengcheng Dai

With the proposed Hund's rule correlation picture, i.e. the fluctuating Fe local moments with the As-bridged antiferromagnetic superexchange interactions, the exceptional collapsed tetragonal phase and related phase transitions observed in…

Materials Science · Physics 2011-04-28 Wei Ji , Xun-Wang Yan , Zhong-Yi Lu

We use inelastic neutron scattering to study acoustic phonons and spin excitations in single crystals of NaFeAs, a parent compound of iron pnictide superconductors. NaFeAs exhibits a tetragonal-to-orthorhombic structural transition at…

At ambient pressure CaFe2As2 has been found to undergo a first order phase transition from a high temperature, tetragonal phase to a low temperature orthorhombic / antiferromagnetic phase upon cooling through T ~ 170 K. With the application…

Intrinsic, in-plane anisotropy of electrical resistivity was studied on mechanically detwinned single crystals of SrFe$_2$As$_2$ above and below the temperature of the coupled structural/magnetic transition, $T_{\textrm{TO}}$. Resistivity…

X-ray diffraction pressure studies at room temperature demonstrate that the spinel FeAl$_{2}$O$_{4}$ transforms to a tetragonal phase at ~18 GPa. This tetragonal phase has a highly irregular unit-cell volume versus pressure dependence up to…

Strongly Correlated Electrons · Physics 2018-09-26 W. M. Xu , G. R. Hearne , S. Layek , D. Levy , M. P. Pasternak , G. Kh. Rozenberg , E. Greenberg

Recent investigations of the superconducting iron-arsenide families have highlighted the role of pressure, be it chemical or mechanical, in fostering superconductivity. Here we report that CaFe2As2 undergoes a pressure-induced transition to…

Understanding the microscopic origins of electronic phases in high-transition temperature (high-Tc) superconductors is important for elucidating the mechanism of superconductivity. In the paramagnetic tetragonal phase of BaFe2-xTxAs2 (where…

Superconductivity · Physics 2014-08-13 Xingye Lu , J. T. Park , Rui Zhang , Huiqian Luo , Andriy H. Nevidomskyy , Qimiao Si , Pengcheng Dai

The magnetic order of the localized Eu$^{2+}$ spins in optimally-doped Eu(Fe$_{1-x}$Ir$_{x}$)$_{2}$As$_{2}$ ($\mathit{x}$ = 0.12) with superconducting transition temperature $\mathit{T_{SC}}$ = 22 K was investigated by single-crystal…

Superconductivity · Physics 2015-02-20 W. T. Jin , Wei Li , Y. Su , S. Nandi , Y. Xiao , W. H. Jiao , M. Meven , A. P. Sazonov , E. Feng , Yan Chen , C. S. Ting , G. H. Cao , Th. Brückel

Unlike the ferropnictide superconductors, which crystallize in a tetragonal crystal structure, binary FeAs forms in an orthorhombic crystal structure, where the local atomic environment resembles a highly distorted variant of the FeAs4…

Other Condensed Matter · Physics 2015-03-17 J. R. Jeffries , N. P. Butch , H. Cynn , S. R. Saha , K. Kirshenbaum , S. T. Weir , Y. K. Vohra , J. Paglione

Neutron and X-ray diffraction, magnetic susceptibility, and specific heat measurements have been used to investigate the magnetic and structural phase transitions of the spinel system Fe1+xCr2-xO4(0.0<=x<=1.0). The temperature versus Fe…

We present a combined high-resolution x-ray diffraction and x-ray resonant magnetic scattering (XRMS) study of as-grown BaFe2As2. The structural/magnetic transitions must be described as a two-step process. At T_S = 134.5 K we observe the…

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

In contrast to the simultaneous structural and magnetic first order phase transition $T_{0}$ previously reported, our detailed investigation on an underdoped Ba$_{0.84}$K$_{0.16}$Fe$_{2}$As$_{2}$ single crystal unambiguously revealed that…

The structural properties of the SrFe2As2 and CaFe2As2 compounds have been extensively analyzed by transmission electron microscopy (TEM) from room temperature down to 20K. The experimental results demonstrate that the SrFe2As2 crystal, in…

Superconductivity · Physics 2013-05-29 C. Ma , H. X. Yang , H. F. Tian , H. L Shi , J. B. Lu , Z. W. Wang , L. J. Zeng , G. F. Chen , N. L. Wang , J. Q. Li

The effects of pressure up to $\sim 20$ kbar, on the structural phase transition of SrFe$_2$As$_2$ and lightly Sn-doped BaFe$_2$As$_2$, as well as on the superconducting transition temperature and upper critical field of…

Superconductivity · Physics 2009-11-13 M. S. Torikachvili , S. L. Bud'ko , N. Ni , P. C. Canfield

Raman scattering can detect spontaneous point-group symmetry breaking without resorting to single-domain samples. Here we use this technique to study $\mathrm{BaFe_2As_2}$, the parent compound of the "122" Fe-based superconductors. We show…

Superconductivity · Physics 2015-11-10 Xiao Ren , Lian Duan , Yuwen Hu , Jiarui Li , Rui Zhang , Huiqian Luo , Pengcheng Dai , Yuan Li

Understanding magnetic interactions in the parent compounds of high-temperature superconductors forms the basis for determining their role for the mechanism of superconductivity. For parent compounds of iron pnictide superconductors such as…