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Ionic liquids (ILs) feature a tailorable and wide range of structural, chemical and electronic properties that make this class of materials suitable to a broad variety of forefront applications in next-generation electronics. Yet, their…

Materials Science · Physics 2022-11-28 Irene Amiehe Essomba , Mauro Boero , Kerstin Falk , Guido Ori

We present a first-principles study of the electronic properties of silicon clathrate nanowires intercalated with various types of alkali or alkaline-earth atoms. We find that the band structure of the nanowires can be tuned by varying the…

Materials Science · Physics 2009-11-11 S. Sirichantaropass , V. M. García-Suárez , C. J. Lambert

In this article, the molecular permanent electric dipole moments and components of static dipole polarizabilities for the electronic ground state of singly charged aluminum monohalides are reported. The coupled-cluster method by considering…

Atomic Physics · Physics 2024-06-18 Ankush Thakur , Renu Bala , H. S. Nataraj , V. S. Prasannaa

We study the electronic structures and dielectric functions of the simple hydrides LiH, NaH, MgH2 and AlH3, and the complex hydrides Li3AlH6, Na3AlH6, LiAlH4, NaAlH4 and Mg(AlH4)2, using first principles density functional theory and GW…

Materials Science · Physics 2007-05-23 M. J. van Setten , V. A. Popa , G. A. de Wijs , G. Brocks

Using a combination of high-level ab initio electronic structure methods with efficient on-the-fly semiclassical evaluation of nuclear dynamics, we performed a massive scan of small polyatomic molecules searching for a long lasting…

Chemical Physics · Physics 2024-09-26 Alan Scheidegger , Jiří Vaníček , Nikolay V. Golubev

It is shown that the consideration of the density of states variation in nanoscale electrochemical systems yields modulations in the rate constant and concomitant electrical currents. The proposed models extend the utility of…

Mesoscale and Nanoscale Physics · Physics 2016-04-22 H. Yamada , P. R. Bandaru

A procedure is described for the precise nonrelativistic evaluation of the dipole polarizabilities of H_2^+ and D_2^+ that avoids any approximation based on the size of the electron mass relative to the nucleus mass. The procedure is…

Atomic Physics · Physics 2007-05-23 J. M. Taylor , A. Dalgarno , J. F. Babb

We present a comprehensive study of the diverse properties of heteronuclear Rydberg molecules, placing a special emphasis on those composed of the light alkali atoms, Li, Na, and K. Electron-atom scattering phase shifts, which determine the…

Atomic Physics · Physics 2019-02-13 Matthew T. Eiles

Recent improvements in experimental techniques for preparing ultracold molecules that contain alkali atoms (e.g., Li, Na, and K) have been reported. Based on these advances in ultracold molecules, new searches for the electric dipole moment…

Atomic Physics · Physics 2020-01-08 A. Sunaga , M. Abe , V. S. Prasannaa , T. Aoki , M. Hada

Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole…

Atomic Physics · Physics 2015-04-08 D. Borsalino , R. Vexiau , M. Aymar , E. Luc-Koenig , O. Dulieu , N. Bouloufa-Maafa

The work presents the detailed analysis of the water dimer properties. Their parameters are investigated on the basis of a multipole interaction potential extended up to the quadrupole--quadrupole and dipole--octupole terms. All main…

Chemical Physics · Physics 2013-05-02 P. V. Makhlaichuk , M. P. Malomuzh , I. V. Zhyganiuk

Alkali metals display unexpected properties at high pressure, including emergence of low symmetry crystal structures, that appear to occur due to enhanced electronic correlations among the otherwise nearly-free conduction electrons. We…

Strongly Correlated Electrons · Physics 2015-06-23 G. Fabbris , J. Lim , L. S. I. Veiga , D. Haskel , J. S. Schilling

The development of advanced electrochemical devices for energy conversion and storage requires fine tuning of electrode reactions, which can be accomplished by altering the electrode/solution interface structure. Particularly, in case of an…

Soft Condensed Matter · Physics 2020-07-02 Yu. A. Budkov , A. V. Sergeev , S. V. Zavarzin , A. L. Kolesnikov

Heavy polar diatomic molecules are the primary tools for searching for the T-violating permanent electric dipole moment of the electron (eEDM). Valence electrons in some molecules experience extremely large effective electric fields due to…

Atomic Physics · Physics 2015-06-11 V. S. Prasannaa , A. C. Vutha , M. Abe , B. P. Das

One of the main objectives of the LHD is to extend the plasma confinement database for helical systems and to demonstrate such extended plasma confinement properties to be sustained in steady state. Among the various plasma parameter…

Plasma Physics · Physics 2015-06-26 Shin Kubo

We analyze the electric dipole moments (PDMs) and static electric dipole polarizabilities of the alkali--alkaline-earth (Alk-AlkE) dimers by employing finite-field coupled-cluster methods, both in the frameworks of non-relativistic and…

Atomic Physics · Physics 2022-06-29 R. Mitra , V. S. Prasannaa , B. K. Sahoo

The static electric dipole polarizability of $\mathrm{Na_N}$ clusters with even N has been calculated in a collective, axially averaged and a three-dimensional, finite-field approach for $2\le N \le 20$, including the ionic structure of the…

Atomic and Molecular Clusters · Physics 2009-10-31 S. Kümmel , T. Berkus , P. -G. Reinhard , M. Brack

Water clusters embedding a nitric acid molecule HNO3(H2O)_{n=1-10} are investigated via electrostatic deflection of a molecular beam. We observe large paraelectric susceptibilities that greatly exceed the electronic polarizability,…

Atomic and Molecular Clusters · Physics 2015-05-14 Ramiro Moro , Jonathon Heinrich , Vitaly V. Kresin

We perform first-principles calculations of the structural, electronic, mechanical, and thermodynamic properties of thorium hydrides (ThH$_{2}$ and Th$_{4}$H$_{15}$) based on the density functional theory with generalized gradient…

Materials Science · Physics 2015-05-14 Bao-Tian Wang , Ping Zhang , Hongzhou Song , Hongliang Shi , Dafang Li , Wei-Dong Li

Calculations of the static electric-dipole scalar and tensor polarizabilities are presented for two alkali atoms, Rb and Cs, for the $nS$, $nP_{1/2, 3/2}$, and $nD_{3/2, 5/2}$ states with large principal quantum numbers up to $n = 50$. The…

Atomic Physics · Physics 2016-09-21 V. A. Yerokhin , S. Y. Buhmann , S. Fritzsche , A. Surzhykov