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We report the results from a computational study of the self-assembly of amphiphilic ditethered nanospheres using molecular simulation. We explore the phase behavior as a function of nanosphere diameter, interaction strength, and…

Mesoscale and Nanoscale Physics · Physics 2009-11-18 Christopher R. Iacovella , Sharon C. Glotzer

Fabrication of diamond structures by self-assembly is a fundamental challenge in making three-dimensional photonic crystals. We simulate a system of model hard particles with attractive patches and show that they can self-assemble into a…

Statistical Mechanics · Physics 2012-01-18 Zhenli Zhang , Aaron S. Keys , Ting Chen , Sharon C. Glotzer

The assembly of colloidal cubic diamond is a challenging process since the shape and interaction parameters and the thermodynamic conditions where this structure is stable are elusive. The simultaneous use of shape-anisotropic particles and…

Soft Condensed Matter · Physics 2024-06-12 Susana Marín-Aguilar , Fabrizio Camerin , Marjolein Dijkstra

We report many different nano-structures which are formed when model nano-particles of different sizes (diameter {\sigma} n ) are allowed to aggregate in a background matrix of semi-flexible self assembled polymeric worm like micellar…

Soft Condensed Matter · Physics 2015-06-23 Shaikh Mubeena , Apratim Chatterji

Concentrated solutions of short blunt-ended DNA duplexes, down to 6 base pairs, are known to order into the nematic liquid crystal phase. This self-assembly is due to the stacking interactions between the duplex terminals that promotes…

Soft Condensed Matter · Physics 2015-05-30 Cristiano De Michele , Tommaso Bellini , Francesco Sciortino

Self-assembly of sphere-forming solution-state amphiphilic diblock copolymers under spherical nanopore confinement is investigated using a simulated annealing technique. For two types of cases of different pore-surface/copolymer…

Soft Condensed Matter · Physics 2023-12-20 Jiaping Wu , Xin Wang , Zheng Wang , Yuhua Yin , Run Jiang , Yao Li , Baohui Li

The fluid phase diagram of trimer particles composed of one central attractive bead and two repulsive beads was determined as a function of simple geometric parameters using flat-histogram Monte Carlo methods. A variety of self-assembled…

Soft Condensed Matter · Physics 2015-05-20 Harold W. Hatch , Jeetain Mittal , Vincent K. Shen

Block copolymers are recognised as a valuable platform for creating nanostructured materials with unique properties. Morphologies formed by block copolymer self-assembly can be transferred into a wide range of inorganic materials, enabling…

Highly periodic structures are often said to convey the beauty of nature. However, most material properties are strongly influenced by the defects they contain. On the mesoscopic scale, molecular self-assembly exemplifies this interplay;…

Using Monte Carlo simulations, we investigate the self-assembly of model nanoparticles inside a matrix of model equilibrium polymers (or matrix of Wormlike micelles) as a function of the polymeric matrix density and the excluded volume…

Soft Condensed Matter · Physics 2018-04-03 Sk. Mubeena , Apratim Chatterji

Quasicrystals are fascinating structures, characterized by strong positional order but lacking the periodicity of a crystal. In colloidal systems, quasicrystals are typically predicted for particles with complex or highly specific…

Soft Condensed Matter · Physics 2022-02-28 Etienne Fayen , Marianne Impéror-Clerc , Laura Filion , Giuseppe Foffi , Frank Smallenburg

One versatile route to the creation of two-dimensional crystal structures on the nanometer to micrometer scale is the self-assembly of colloidal particles at an interface. Here, we explore the crystal phases that can be expected from the…

Soft Condensed Matter · Physics 2020-05-29 Etienne Fayen , Anuradha Jagannathan , Giuseppe Foffi , Frank Smallenburg

The realization of scalable arrangements of nitrogen vacancy (NV) centers in diamond remains a key challenge on the way towards efficient quantum information processing, quantum simulation and quantum sensing applications. Although…

We report the formation of a binary crystal of hard polyhedra due solely to entropic forces. Although the alternating arrangement of octahedra and tetrahedra is a known space-tessellation, it had not previously been observed in…

We present a theoretical description of a mechanism for self assembly in binary soft nanoparticle systems of the type which were studied experimentally by Talapin et al [1]. We focus on, in particular, the conditions for formation of…

Statistical Mechanics · Physics 2021-04-13 Anuradha Jagannathan

We present results of Brownian dynamics simulations of tethered nanospheres and tethered nanorods. Immiscibility between tether and nanoparticle facilitates microphase separation into the bicontinuous, double gyroid structure (first…

Soft Condensed Matter · Physics 2009-01-08 Christopher R. Iacovella , Mark A. Horsch , Sharon C. Glotzer

The phase diagram of model anisotropic particles with four attractive patches in a tetrahedral arrangement has been computed at two different values for the range of the potential, with the aim of investigating the conditions under which a…

Materials Science · Physics 2013-06-26 Eva G. Noya , Carlos Vega , Jonathan P. K. Doye , Ard A. Louis

We present results of molecular simulations that predict the phases formed by the self-assembly of model nanospheres functionalized with a single polymer "tether", including double gyroid, perforated lamella and crystalline bilayer phases.…

Soft Condensed Matter · Physics 2007-05-23 Christopher R. Iacovella , Aaron S. Keys , Mark A. Horsch , Sharon C. Glotzer

Self-assembly processes provide the means to achieve scalable and versatile metamaterials by "bottom-up" fabrication. Despite their enormous potential, especially as a platform for energy materials, self-assembled metamaterials are often…

Applied Physics · Physics 2023-03-09 Jelena Wohlwend , Georg Haberfehlner , Henning Galinski

We systematically explore the self-assembly of semi-flexible polymers in deformable spherical confinement across a wide regime of chain stiffness, contour lengths and packing fractions by means of coarse-grained molecular dynamics…

Soft Condensed Matter · Physics 2021-07-12 Maxime M. C. Tortora , Daniel Jost
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