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The interaction of hydrogen with many transition metal surfaces is characterized by a coexistence of activated with non-activated paths to adsorption with a broad distribution of barrier heights. By performing six-dimensional quantum…

mtrl-th · Physics 2016-09-07 Axel Gross , Matthias Scheffler

Based on first principles calculations we investigate the electronic and magnetic properties of Pt layers in Pd$(001)$/Co/Pt thin film structures exposed to an external electric field. Due to the Co underlayer, the surface Pt layers have…

Materials Science · Physics 2021-02-10 Eszter Simon , Alberto Marmodoro , Sergiy Mankovsky , Hubert Ebert

We analyze non-equilibrium current transport in molecular electronic devices, using as an example devices formed by two terphenyl dithiol molecules attached to gold electrodes. Using a first-principles based self-consistent matrix Green's…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark A. Ratner

Using first-principles calculations we show that the work function of noble metals can be decreased or increased by up to 2 eV upon the adsorption of self-assembled monolayers of organic molecules. We identify the contributions to these…

Other Condensed Matter · Physics 2007-05-23 Paul C. Rusu , Geert Brocks

Chemiresistive materials, which alter their electrical resistance in response to interactions with surrounding chemicals, are valued for their robustness, rapid detection ability and high sensitivity. Recent research has revealed that the…

Chemical Physics · Physics 2024-11-26 Pratyasha Rudra , Swastik Mondal

Electrons on the helium surface display sharp resonant absorption lines related to the transitions between the subbands of quantized motion transverse to the surface. A magnetic field parallel to the surface strongly affects the absorption…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 A. D. Chepelianskii , D. Konstantinov , M. I. Dykman

The interaction between the field emission resonance states and the photodetached electron in an electric field is studied by semiclassical theory. An analytical expression of the photodetachment cross section is derived in the framework.…

Atomic Physics · Physics 2015-05-13 Yan Han , Lifei Wang , Ningyu Yang , Shiyong Ran , Guangcan Yang

As a first step to meet the challenge to calculate the electronic structure and total energy of charged states of atoms and molecules adsorbed on ultrathin-insulating films supported by a metallic substrate using density functional theory…

Materials Science · Physics 2013-11-01 Iván Scivetti , Mats Persson

The dissociative adsorption of methane on variously oxidized Pd, Pt and Pd-Pt surfaces is investigated using density-functional theory, as a step towards understanding the combustion of methane on these materials. For Pd-Pt alloys, models…

We investigate how tilting affects the off-diagonal, dissipationless response of a pair of chirally imbalanced Weyl cones to various external perturbations. The pair of chirally imbalanced Weyl cones can be described as a chiral electron…

Mesoscale and Nanoscale Physics · Physics 2019-07-17 E. C. I. van der Wurff , H. T. C. Stoof

Chemical adsorption of the species at semiconductor surfaces is analyzed showing the existence of the two contributions to adsorption energy: bond creation and charge transfer. It is shown that the energy of quantum surface states is…

Materials Science · Physics 2013-08-20 Stanislaw Krukowski , Pawel Kempisty , Pawel Strak

Oxygen molecule adsorptions on a Pu (100) surface have been studied in detail, using the generalized gradient approximation to density functional theory. Dissociative adsorption with a layer by layer alternate spin arrangement of the…

Materials Science · Physics 2009-11-10 M. N. Huda , A. K. Ray

Multi-valent (MV) battery architectures based on pairing a Mg metal anode with a high-voltage ($\sim$ 3 V) intercalation cathode offer a realistic design pathway toward significantly surpassing the energy storage performance of traditional…

We apply Density Functional Theory (DFT) and the DFT+U technique to study the adsorption of transition metal porphine molecules on atomistically flat Au(111) surfaces. DFT calculations using the Perdew-Burke-Ernzerhof (PBE) exchange…

Recent I/V curve measurements suggest that C60 molecules deposited in gold nanojunctions change their adsorption configuration when a finite voltage in a 2-terminal setting is applied. This is of interest for molecular electronics because a…

Materials Science · Physics 2015-06-25 R. Stadler , S. Kubatkin , T. Bjornholm

We present the results from an extensive atomistic molecular dynamics simulation study of poly(ethylene oxide) (PEO) doped with various amounts of lithium-bis(trifluoromethane)sulfonimide (LiTFSI) salt under the influence of external…

Soft Condensed Matter · Physics 2021-03-10 Alina Wettstein , Diddo Diddens , Andreas Heuer

We investigated the effect of an electric field on the interface magnetic anisotropy of a thin MgO/Fe/MgO layer using density functional theory. The perpendicular magnetic anisotropy energy (MAE) increases not only under electron depletion…

Materials Science · Physics 2015-06-23 Daiki Yoshikawa , Masao Obata , Yusaku Taguchi , Shinya Haraguchi , Tatsuki Oda

The effect of hydrogen adsorption on the magnetic properties of an Fe$_3$ cluster immersed in a Cu(111) surface has been calculated using densifty functional theory and the results used to parametrize an Alexander-Anderson model which takes…

Mesoscale and Nanoscale Physics · Physics 2013-12-16 Pavel F. Bessarab , Valery M. Uzdin , Hannes Jónsson

Nitrogen-doped graphene was recently synthesized and was reported to be a catalyst for hydrogen dissociative adsorption under a perpendicular applied electric field (F). In this work, the diffusion of H atoms on N-doped graphene, in the…

Materials Science · Physics 2012-02-15 Z. M. Ao , A. D. Hernández-Nieves , F. M. Peeters , S. Li

A model of the non-concentric spherical core-shell quantum dot under the influence of an externally applied electric field was proposed. It was established that the energy spectrum of both the electron and the hole depends on the intensity…

Mesoscale and Nanoscale Physics · Physics 2024-12-31 R. Ya. Leshko , I. V. Bilynskyi , O. V. Leshko , M. Yu. Popov , A. O. Ocheretyanyi
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