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In this paper we analyze the behavior of hydrophobic polyelectrolytes. It has been proposed that this system adopts a pearl-necklace structure reminiscent of the Rayleigh instability of a charged droplet. Using a Poisson-Boltzmann approach,…

Soft Condensed Matter · Physics 2008-04-24 Alexei Chepelianskii , Farshid Mohammad-Rafiee , Elie Raphael

We study the electric double layer near a charged soft surface by using a mean-field approach including non-uniform size effect and solvent polarization. Based on a free energy model, electrostatic potential and number densities of water…

Soft Condensed Matter · Physics 2022-02-10 Jun-Sik Sin , Nam-Hyok Kim , Chung-Sik Sin

The solution of the Poisson--Boltzmann equation for counterions confined between two charged plates is known analytically up to a constant, namely, the ion density in the middle of the channel. This quantity is relevant also because it…

Computational Physics · Physics 2018-09-06 Andrei Bazarenko , Marcello Sega

We report direct experimental evidence that the insulating phase of a disordered, yet strongly interacting two-dimensional electron system (2DES) becomes unstable at low temperatures. As the temperature decreases, a transition from…

Mesoscale and Nanoscale Physics · Physics 2008-01-15 M. Baenninger , A. Ghosh , M. Pepper , H. E. Beere , I. Farrer , D. A. Ritchie

Ionic microgel particles are intriguing systems in which the properties of thermo-responsive polymeric colloids are enriched by the presence of charged groups. In order to rationalize their properties and predict the behaviour of microgel…

Soft Condensed Matter · Physics 2021-01-28 G. Del Monte , F. Camerin , A. Ninarello , N. Gnan , L. Rovigatti , E. Zaccarelli

We study equilibrium statistical mechanics of classical point counter-ions, formulated on 2D Euclidean space with logarithmic Coulomb interactions (infinite number of particles) or on the cylinder surface (finite particle numbers), in the…

Soft Condensed Matter · Physics 2011-03-08 L. Samaj , E. Trizac

The behavior of polyampholytes near a charged planar surface is studied by means of Monte Carlo simulations. The investigated polyampholytes are overall electrically neutral and made up of oppositely charged units (called blocks) that are…

Soft Condensed Matter · Physics 2009-11-11 Rene Messina

Electrophoretic (EP) mobility reversal is commonly observed for strongly charged macromolecules in multivalent salt solutions. This curious effect takes place, e.g., when a charged polymer, such as DNA, adsorbs excess counterions so that…

Soft Condensed Matter · Physics 2023-03-28 Xiang Yang , Sahin Buyukdagli , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

We consider the complexation of highly charged semiflexible polyelectrolytes with oppositely charged macroions. On the basis of scaling arguments we discuss how the resulting complexes depend on the persistence length of the…

Soft Condensed Matter · Physics 2009-11-07 H. Schiessel , R. F. Bruinsma , W. M. Gelbart

We study the ionic equilibria and interactions of neutral semi-permeable spherical shells immersed in electrolyte solutions, including polyions. Although the shells are uncharged, only one type of ions of the electrolyte can permeate them,…

Soft Condensed Matter · Physics 2012-07-24 Vladimir Lobaskin , Artem N. Bogdanov , Olga I. Vinogradova

Though often considered as one of the main driving process of the complexation of species of opposite charges, the release of counterions has never been experimentally directly measured on polyelectrolyte/proteins complexes. We present here…

Chemical Physics · Physics 2009-04-07 Jérémie Gummel , Fabrice Cousin , François Boué

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

The equilibrium electric double layer (EDL) that surrounds the colloidal particles is determinant for the response of a suspension under a variety of static or alternating external fields. An ideal salt-free suspension is composed by the…

Soft Condensed Matter · Physics 2017-09-13 R. Roa , F. Carrique , E. Ruiz-Reina

A novel statistical model for the cooperative binding of monomeric ligands to a linear lattice is developed to study the interaction of ionic surfactant molecules with flexible polyion chain in dilute solution. Electrostatic binding of a…

Soft Condensed Matter · Physics 2015-01-13 T. Nishio , T. Shimizu , Sh. Yoshida , A. Minakata

The build up of polyelectrolyte multilayers (PEMs) was observed by a silicon-on-insulator (SOI) based thin film resistor. Differently charged polyelectrolytes adsorbing to the sensor surface result in defined potential shifts, which…

Soft Condensed Matter · Physics 2007-05-23 Petra A. Neff , Ali Naji , Christof Ecker , Bert Nickel , Regine von Klitzing , Andreas R. Bausch

Recent experiments have reported evidence of dominant electron-hole scattering in the electric conductivity of suspended bilayer graphene near charge neutrality. According to these experiments, plots of the electric conductivity as a…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Mohammad Zarenia , Shaffique Adam , Giovanni Vignale

We present a systematic statistical mechanical analysis of the conformational properties of a stiff polyelectrolyte chain with intrachain attractions that are due to counterion correlations. We show that the mean-field solution corresponds…

Soft Condensed Matter · Physics 2007-05-23 Per Lyngs Hansen , Rudi Podgornik , Daniel Svenšek , V. Adrian Parsegian

We report an investigation of the equilibrium and dynamic properties of polyelectrolyte solutions confined between platinum surfaces with a dynamic Surface Force Apparatus. The polyelectrolyte adsorbs on the surfaces in a dense compact…

Soft Condensed Matter · Physics 2018-03-12 Chloé Barraud , Benjamin Cross , Cyril Picard , Frédéric Restagno , Liliane Léger , Elisabeth Charlaix

The electronic structure of the conjugated polymer, polyaniline, has been studied by resonant and nonresonant X-ray emission spectroscopy using synchrotron radiation for the excitation. The measurements were made on polyaniline and a few…

Materials Science · Physics 2012-01-05 M. Magnuson , J. -H. Guo , S. M. Butorin , A. Agui , C. Såthe , J. Nordgren , A. P. Monkman

In this letter, we study the effects of weak off-diagonal disorder on conjugated polymers with a doubly degenerate ground-state. We find that disorder induces a finite density of neutral solitons in the lattice dimerization of a polymer…

Soft Condensed Matter · Physics 2007-05-23 Marc Thilo Figge , Maxim V. Mostovoy , Jasper Knoester
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