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Two-dimensional (2D) materials that exhibit spontaneous magnetization, polarization or strain (referred to as ferroics) have the potential to revolutionize nanotechnology by enhancing the multifunctionality of nanoscale devices. However,…

The metallic or insulating nature of the paramagnetic phase of the colossal-magnetoresistance manganites is investigated via a double exchange Hamiltonian with diagonal disorder. Mobility edge trajectory is determined with the transfer…

Strongly Correlated Electrons · Physics 2016-08-31 Qiming Li , Jun Zang , A. R. Bishop , C. M. Soukoulis

We report an infrared reflection spectroscopy study of La$_{1/2}$Ca$_{1/2}$MnO$_3$ over a broad frequency range and temperature interval which covers the transitions from the high temperature paramagnetic to ferromagnetic and, upon further…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , M. Pissas , C. W. Chu

We have studied structural, magnetic and transport properties as a function of temperature and magnetic field in the electron doped manganite YxCa1-xMnO3, for 0<x<0.25. We found that in the paramagnetic regime, the magnetic susceptibility,…

Condensed Matter · Physics 2007-05-23 H. Aliaga , M. T. Causa , A. Butera , B. Alascio , H. Salva , M. Tovar D. Vega , G. Polla , G. Leyva , P. Konig

To understand the collinear-magnetism-driven ferroelectricity in multiferroic Ca3CoMnO6 compound, we have established an elastic diatomic Ising spin-chain model with axial-next-nearest-neighbor interaction to describe its magnetoelectric…

Statistical Mechanics · Physics 2016-03-23 Yan Qi , Qi Yang , Nai-sen Yu , An Du

We show by means of ab-initio calculations that the organic molecular crystal TTF-CA is multiferroic: it has an instability to develop spontaneously both ferroelectric and magnetic ordering. Ferroelectricity is driven by a Peierls…

The relationship between magnetic order and ferroelectric properties has been investigated for MnWO$_4$ with long-wavelength magnetic structure. Spontaneous electric polarization is observed in an elliptical spiral spin phase. The…

Strongly Correlated Electrons · Physics 2009-11-11 K. Taniguchi , N. Abe , T. Takenobu , Y. Iwasa , T. Arima

Multiferroicity and magnetodielectric coupling in metal-organic-frameworks (MOFs) is rare and so far restricted mainly to formate-based systems with perovskite structure. In the course of this work we designed a tetragonal framework…

Materials Science · Physics 2017-10-31 Tathamay Basu , A. Jesche , B. Bredenkotter , M. Grzywa , D. Denysenko , D. Volkmer , A. Loidl , S. Krohns

The phase diagram of half-doped manganite systems of formula A_{0.5}A'_{0.5}MnO_3 is investigated within a single-orbital model incorporating magnetic double-exchange and superexchange, together with intersite Coulomb and electron-lattice…

Strongly Correlated Electrons · Physics 2009-10-31 S. Fratini , D. Feinberg , M. Grilli

The structure and properties of the 1:1 superlattice of LaVO$_{3}$ and SrVO$_{3}$ are investigated with a first-principles density-functional-theory-plus-$U$ (DFT+$U$) method. The lowest energy states are antiferromagnetic charge-ordered…

Materials Science · Physics 2017-03-01 Se Young Park , Anil Kumar , Karin M. Rabe

We show that the symmetry of the spin zigzag chain E phase of the orthorhombic perovskite manganites and nickelates allows for the existence of a finite ferroelectric polarization. The proposed microscopic mechanism is independent of…

Strongly Correlated Electrons · Physics 2007-05-23 I. A. Sergienko , C. Sen , E. Dagotto

Using the density-functional-theory based electronic structure calculations, we study the electronic state of recently discovered mixed-valent manganese oxides $A$Mg$_4$Mn$_6$O$_{15}$ ($A=$ K, Rb, Cs), which are fully spin-polarized…

Strongly Correlated Electrons · Physics 2018-04-18 T. Yamaguchi , K. Sugimoto , Y. Ohta , Y. Tanaka , H. Sato

Experimental evidence show that in the magnetoresistive manganite Ca_(1-x) Y_xMnO_3, ferromagnetic (FM) polarons arises in an antiferromagnetic (AF) background, as a result of the doping with Yttrium. This hypothesis is supported in this…

Condensed Matter · Physics 2009-11-07 H. Aliaga , M. T. Causa , M. Tovar , B. Alascio

Multiferroics, defined for those multifunctional materials in which two or more kinds of fundamental ferroicities coexist, have become one of the hottest topics of condensed matter physics and materials science in recent years. The…

Materials Science · Physics 2015-05-13 K. F. Wang , J. -M. Liu , Z. F. Ren

Multiferroic CuFe1-xAlxO2 (x=0.02) exhibits a ferroelectric ordering accompanied by a proper helical magnetic ordering below T=7K under zero magnetic field. By polarized neutron diffraction and pyroelectric measurements, we have revealed a…

Strongly Correlated Electrons · Physics 2008-03-31 T. Nakajima , S. Mitsuda , S. Kanetsuki , K. Tanaka , K. Fujii , N. Terada , M. Soda , M. Matsuura , K. Hirota

Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any other known material in which the electric polarization is induced by spontaneous…

We report results of a Monte Carlo study of doped, diluted magnetic semiconductors in the low carrier density (insulating) regime. We find that the system undergoes a transition from a paramagnet at high temperatures to a ferromagnet at low…

Materials Science · Physics 2007-05-23 Xin Wan , R. N. Bhatt

Magneto-electric multiferroics exemplified by TbMnO3 possess both magnetic and ferroelectric long-range order. The magnetic order is mostly understood, whereas the nature of the ferroelectricity has remained more elusive. Competing models…

Strongly Correlated Electrons · Physics 2011-10-14 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , J. Herrero-Martin , A. T. Boothroyd , D. Prabhakaran , D. F. McMorrow

We develop a comprehensive theory for magnetoelectricity in magnetically ordered quasi-2D systems whereby in thermal equilibrium an electric field can induce a magnetization $m$ and a magnetic field can induce a polarization. This effect…

Mesoscale and Nanoscale Physics · Physics 2020-10-16 R. Winkler , U. Zülicke

The double exchange (DE) model is systematically applied for studying the coupling between ferroelectric (FE) and magnetic orders in several prototypical types of multiferroic manganites. The model was constructed for the magnetically…

Strongly Correlated Electrons · Physics 2014-11-26 I. V. Solovyev , S. A. Nikolaev